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Recent advances in nanofabrication technology now enable unprecedented control over 2D heterostructures, in which single- or few-atom thick materials with synergetic opto-electronic properties can be combined to develop next-generation…
Noble metal nanoparticles show specific optical properties due to the excitation of localized surface plasmons that make them attractive candidates for highly sensitive bionanosensors. The underlying physical principle is either an…
We address the issue of the second-order coherence of single surface plasmons launched by a quantum source of light into extended gold films. The quantum source of light is made of a scanning fluorescent nanodiamond hosting five…
The optical responses of metals are often dominated by plasmonic resonances - the collective oscillations of interacting electron liquids. Here we unveil a new class of plasmons - quantum metric plasmons (QMPs) - that arise in a wide range…
Strong light-matter interactions enabled by surface plasmons have given rise to a wide range of photonic, optoelectronic and chemical functionalities. In recent years, the interest in this research area has focused on the quantum regime,…
Noble metal nanoparticles exhibit localized plasmon resonance modes that span the visible and near-infrared spectral ranges and have many applications. Modifying the size, shape, and composition of the nanoparticles changes the number of…
Metallic nanostructures can support so-called plasma oscillations (plasmons). Plasmons allow for the concentration of the energy from light, down to sizes well below the conventional diffraction limit known from optics. Plasmonics thus…
We use electronic structure calculations based upon density functional theory to search for ideal plasmonic materials among the alkali noble intermetallics. Importantly, we use density functional perturbation theory to calculate the…
Combining miniaturization and good operating speed is a compelling yet crucial task for our society. Plasmonic waveguides enable the possibility of carrying information at optical operating speed while maintaining the dimension of the…
Quantum plasmonics experiments have on multiple occasions reported the observation of quantum coherence of discrete plasmons, which exhibit remarkable preservation of quantum interference visibility, a seemingly surprising feature for…
Surface plasmon polaritons (SPPs) have recently been recognized as an important future technique for microelectronics. Such SPPs have been studied using classical theory. However, current state-of-the-art experiments are rapidly approaching…
We have shown that alloying a noble metal (gold) with another metal (cadmium), which can contribute two electrons per atom to a free electron gas, can significantly improve the metals optical properties in certain wavelength ranges and make…
We compute the decay rates of emitters coupled to spheroidal nanoantennas made of gold, copper, silver, and aluminum. The spectral position of the localized surface plasmon-polariton resonance, the enhancement factors and the quantum…
Plasmons are usually described in terms of macroscopic quantities such as electric fields and currents. However as fundamental excitations of metals they are also quantum objects with internal structure. We demonstrate that this can induce…
Quantum effects of plasmonic phenomena have been explored through ab-initio studies, but only for exceedingly small metallic nanostructures, leaving most experimentally relevant structures too large to handle. We propose instead an…
Gold nanorod has generated great research interest due to its tunable longitudinal plasmon resonance. However, little progress has been made in the understanding of the effect. A major reason is that, except for metallic spheres and…
Noble metal nanoparticles have been utilized for a vast amount of optical applications. For the applications that used metal nanoparticles as nanosensors and optical labeling, larger radiation damping is preferred (higher optical signal).…
For distances less 10 nm, a total energy transfer occurs from a quantum emitter to a nearby metallic surface, producing evanescent surface waves that are plasmonic in nature. When investigating a metallic nanohole supported on an optically…
Lasing at the nanometre scale promises strong light-matter interactions and ultrafast operation. Plasmonic resonances supported by metallic nanoparticles have extremely small mode volumes and high field enhancements, making them an ideal…
Herein, we investigate the optical properties of quantum plasmonic metasurfaces composed of metallic nano-objects with subnanometer gaps according to the time-dependent density functional theory, a fully quantum mechanical approach. When…