Related papers: Filming non-radiative population transfer: Time-re…
Future ultrafast x-ray light sources might image ultrafast coherent electron motion in real-space and in real-time. For a rigorous understanding of such an imaging experiment, we extend the theory of non-resonant x-ray scattering to the…
We propose a novel way to image dynamical properties of nonstationary electron systems using ultrafast resonant x-ray scattering. Employing a rigorous theoretical analysis within the framework of quantum electrodynamics, we demonstrate that…
An application of resonant inelastic x-ray scattering technique for studying of optical scale excitations in electron-correlated materials is discussed. Examples are given including data obtained for 3d transition metal, lanthanide, and…
The elastic scattering of twisted electrons by diatomic molecules is studied within the framework of the non-relativistic first Born approximation. In this process, the coherent interaction of incident electrons with two molecular centers…
We propose an approach to probe coherent spin-state dynamics of molecules using circularly polarized hard x-ray pulses. For the dynamically aligned nitric oxide molecules in a coherent superposition spin-orbit coupled electronic state that…
The scattering of 1D matter wave bright solitons on attractive potentials enables one to populate bound states, a feature impossible with noninteracting wave packets. Compared to noninteracting states, the populated states are renormalized…
Oxygen resonant inelastic X-ray scattering has become a prominent tool for unveiling the electronic structure of solids, especially redox mechanisms in Li-rich cathode materials. A number of studies have observed a strong absorption feature…
Whereas atom-molecule collisions have been studied with complete quantum state resolution, interactions between two state-selected molecules have proven much harder to probe. Here, we report the measurement of state-resolved inelastic…
Scattering theory traditionally deals with the asymptotic behaviour of a system far removed from the actual scattering event. Here we present an experimental study of the one-dimensional scattering of a non-interacting condensate of 87-Rb…
Free-electron laser hard X-ray light sources can provide high fluence, femtosecond pulses, enabling the time-resolved probing of structural dynamics and elementary relaxation processes in molecules. Traditional X-ray elastic scattering from…
Molecular iodine was photoexcited by a strong 800 nm laser, driving several channels of multiphoton excitation. The motion following photoexcitation was probed using time-resolved X-ray scattering, which produces a scattering map…
Nonadiabatic dynamics around an avoid crossing or a conical intersection play a crucial role in the photoinduced processes of most polyatomic molecules. The present work shows that the topological phase in conical intersection makes the…
The coherence of a hyperfine-state superposition of a trapped $^{9}$Be$^+$ ion in the presence of off-resonant light is experimentally studied. It is shown that Rayleigh elastic scattering of photons that does not change state populations…
The physics of radioactive ion beams implies the description of weakly-bound nuclear systems. One key aspect concerns the coupling to low-lying collective-type excited states, which for these systems might not be stable levels, but particle…
In this work, we irradiate a superconducting artificial molecule composed of two coupled tunable transmons with microwave light while monitoring its state via joint dispersive readout. Performing high-power spectroscopy, we observe and…
The ultrafast non-radiative relaxation of a molecular ensemble coupled to a cavity mode is considered theoretically and by real-time quantum dynamics. For equal coupling strength of single molecules to the cavity mode, the non-radiative…
We have embedded an artificial atom, a superconducting transmon qubit, in a 1D open space and investigated the scattering properties of an incident microwave coherent state. By studying the statistics of the reflected and transmitted…
Observing the motion of the nuclear wavepackets during a molecular reaction, in both space and time, is crucial for understanding and controlling the outcome of photoinduced chemical reactions. We have imaged the motion of a vibrational…
Inclusive quasi-elastic electron scattering off nuclei is investigated at high momentum transfer (Q^2>1 (GeV/c)^2) and x>1 adopting a consistent treatment of nucleon-nucleon correlations in initial and final states. It is shown that in case…
We investigate theoretically a nuclear excitation mechanism involving absorption of non-resonant photons leveraged by the coupling to the atomic shell. The nuclear non-resonant photoexcitation is assisted by electron recombination which…