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The dissolution of NaCl in water is one of the most common everyday processes, yet it remains poorly understood at the molecular level. Here we report the results of an extensive density functional theory study in which the initial stages…

Chemical Physics · Physics 2013-12-18 Jiří Klimeš , David R. Bowler , Angelos Michaelides

We investigate salt crystallization in porous media that can lead to their disintegration. For sodium sulfate we show for the first time experimentally that when anhydrous crystals are wetted with water, there is very rapid growth of the…

Soft Condensed Matter · Physics 2009-06-16 Noushine Shahidzadeh Bonn , Francois Bertrand , Daniel Bonn

Charged colloids can form ordered structures like Wigner crystals or glasses at very low concentrations due to long-range electrostatic repulsions. Here, we combine small-angle x-ray scattering (SAXS) and optical experiments with…

Soft Condensed Matter · Physics 2025-03-19 Hanna Anop , Laura Dal Compare , Frederic Nallet , Achille Giacometti , Eric Grelet

Specifically, we examine concentrations from [NaCl]=1m to [NaCl]=6m, where 6.1m represents the solubility threshold of NaCl in H2O. For the water model, we employ the flexible TIP4P/$\epsilon_{Flex}$ model, which offers an enhanced…

Statistical Mechanics · Physics 2024-10-25 Raúl Fuentes-Azcatl

Aqueous solutions of LiCl are probably the most studied electrolyte solutions related to the complexity of liquid water at low temperatures. Despite the large amount of available experimental data hardly any computational studies were…

Soft Condensed Matter · Physics 2020-04-29 Philip H. Handle

The aggregation of binary colloids of same size and balanced charges is studied by Brownian dynamics simulations for dilute suspensions. It is shown that, under appropriate conditions, the formation of colloidal crystals is dominated by…

Soft Condensed Matter · Physics 2015-06-12 D. Bochicchio , A. Videcoq , R. Ferrando

We report the detection of NaCl, KCl, and their $^{37}$Cl and $^{41}$K isotopologues toward the disk around Orion SrcI. About 60 transitions of these molecules were identified. This is the first detection of these molecules in the…

Astrophysics of Galaxies · Physics 2019-02-20 Adam Ginsburg , Brett McGuire , Richard Plambeck , John Bally , Ciriaco Goddi , Melvyn Wright

HCl, a 'textbook' example of a polar covalent molecule, is a well-known compound of hydrogen and chlorine. Inspired by the discovery of unexpected stable stoichiometries of sodium chlorides, we performed systematic searches for all stable…

Materials Science · Physics 2015-08-07 Qingfeng Zeng , Shuyin Yu , Duan Li , Gilles Frapper , Artem R. Oganov

We have prepared a series of polycrystalline samples La$_{0.5}$Sr$_{0.5}$CoO$_{3-\delta}$} with $0 < \delta \le 0.21$ and characterized their oxygen content, crystal structure, and magnetic properties. While the fully oxygenated samples are…

Materials Science · Physics 2007-05-23 Ryan P. Haggerty , Ram Seshadri

We present a first-principles study on the dielectric properties of an NaCl crystal and ultrathin NaCl films under a finite external electric field. Our results show that the high-frequency dielectric constant of the films is not affected…

Materials Science · Physics 2009-11-10 Tomoya Ono , Kikuji Hirose

The reaction of alkali (Na, Cs) clusters with water clusters embedded in helium nanodroplets is studied using femtosecond photo-ionization as well as electron impact ionization. Unlike Na clusters, Cs clusters are found to completely react…

Atomic and Molecular Clusters · Physics 2011-12-19 S. Mueller , S. Krapf , Th. Koslowski , M. Mudrich , F. Stienkemeier

The crystal structures of the NaxCoO2 phases based on three-layer NaCoO2, with x=0.32, x=0.51, x=0.60, x=0.75 and x=0.92, determined by powder neutron diffraction, are reported. The structures have triangular CoO2 layers interleaved by…

Strongly Correlated Electrons · Physics 2009-11-11 L. Viciu , J. W. G. Bos , H. W. Zandbergen , Q. Huang , M. L. Foo , S. Ishiwata , A. P. Ramirez , M. Lee , N. P. Ong , R. J. Cava

It is shown that structuring at the microlevel, a previously not described in detail phenomenon, is the intrinsic property of water and aqueous solutions. At room conditions water (including "ultrapure" one) and aqueous solutions are…

Soft Condensed Matter · Physics 2018-09-05 Tatiana Yakhno , Vladimir Yakhno

This paper aims to study Na doping in Bi-2212 superconducting ceramics. Na-doped Bi-2212 samples powders with a Bi2-uSr2-vCa1-wCu2-xNayOz stoichiometry are prepared by means of thermal treatments. The intended Na substitution level, y, is…

Superconductivity · Physics 2007-05-23 S. Rahier , S. Stassen , R. Cloots , M. Ausloos

In recent experiments on sodium chloride clusters structural transitions between nanocrystals with different cuboidal shapes were detected. Here we presents results for the thermodynamics and dynamics of one of these clusters, (NaCl)35Cl-.…

Condensed Matter · Physics 2007-05-23 Jonathan Doye , David Wales

Water hydrogen bonding is extremely versatile; approximately 20 ice structures and several types of clathrate hydrate structures have been identified. These crystalline water structures form at temperatures below room temperature and/or at…

Alkali halide (100) crystal surfaces are anomalous, being very poorly wetted by their own melt at the triple point. We present extensive simulations for NaCl, followed by calculations of the solid-vapor, solid-liquid, and liquid-vapor free…

Other Condensed Matter · Physics 2007-05-23 T. Zykova-Timan , D. Ceresoli , U. Tartaglino , E. Tosatti

As a nontrivial solid state of matter, the glassy-crystal state embraces physical features of both crystalline and amorphous solids, where a long-range ordered periodic structure formed by the mass centers of constituent molecules…

Dating from experiments more than 20 years ago, it has been realized that the crystallization of hard colloidal particles in the vicinity of dynamical arrest has several anomalies, that render the conventional nucleation and growth model…

Disordered Systems and Neural Networks · Physics 2011-02-25 Davide Cellai , Andrzej Z. Fima , Aonghus Lawlor , Kenneth A. Dawson

In this paper we report the structural and property (magnetic and electrical transport) measurements of nanocrystals of half-doped $\mathrm{La_{0.5}Ca_{0.5}MnO_3}$(LCMO) synthesized by chemical route, having particle size down to an average…

Strongly Correlated Electrons · Physics 2009-11-13 Tapati Sarkar , Barnali Ghosh , A. K. Raychaudhuri , Tapan Chatterji