Related papers: Cs nDJ Rydberg-atom macrodimers formed by long-ran…
We demonstrate the single-photon Rydberg excitation of cesium atoms in a magneto-optical trap (MOT). We excite atoms directly from ${{6S}_{1/2}}$ ground state to ${{nP}_{3/2}}(n=70-100)$ Rydberg state with a narrow-linewidth 319 nm…
The general formalism of the multipolar expansion of electrostatic interactions is applied to the calculation the potential energy between an excited atom (without fine structure) and a ground state diatomic molecule at large separations.…
The passage of cold cesium 49S$_{1/2}$ Rydberg atoms through an electric-field-induced multi-level avoided crossing with nearby hydrogen-like Rydberg levels is employed to prepare a cold, dipolar Rydberg atom gas. When the electric field is…
We investigate the phenomenon of optical bistability in a driven ensemble of Rydberg atoms. By performing two experiments with thermal vapors of rubidium and cesium, we are able to shed light onto the underlying interaction mechanisms…
Atoms with a highly excited electron, called Rydberg atoms, can form unusual types of molecular bonds. The bond differs from the well known ionic and covalent bonds not only by its binding mechanism, but also by its bond length ranging up…
We consider three level atoms driven by two resonant light fields in a ladder scheme where the upper level is a highly excited Rydberg state. We show that the dipole--dipole interactions between Rydberg excited atoms prevents the formation…
We explore the fluorescence signals from a pair of atoms driven towards Rydberg states on a three-level ladder transition. The dipole--dipole interactions between Rydberg excited atoms significantly distort the dark state and…
We predict the existence of a class of ultracold giant molecules formed from trapped ultracold Rydberg atoms and polar molecules. The interaction which leads to the formation of such molecules is the anisotropic charge-dipole interaction…
Rydberg states of excitons are promising quantum objects to engineer giant nonlinearities in a solid-state system. For this purpose, a deeper understanding of the dynamics of Rydberg excitons and of their potential for coherent manipulation…
We report on the realization of a $^{133}$Cs optical tweezer array in a cryogenic blackbody radiation (BBR) environment. By enclosing the array within a 4K radiation shield, we measure long Rydberg lifetimes, up to $406 (36)\,\mu$s for the…
Neutral atom qubits with Rydberg-mediated interactions are a leading platform for developing large-scale coherent quantum systems. In the majority of experiments to date, the Rydberg states are not trapped by the same potential that…
Vibrational properties of ultralong Rydberg Cs$_2$ molecules are investigated on corresponding potential curves obtained by perturbation theory. The Rydberg Cs$_2$ molecules are associated by a Rydberg Cs($nS/nP$) atom $(n=30-70)$ and a…
We present a pulsed four-wave mixing (FWM) scheme via a Rydberg state to create, store and retrieve collective Rydberg polaritons. The storage medium consists of a gas of thermal Rb atoms confined in a 220 {\mu}m thick cell, which are…
Rydberg atoms provide a powerful platform for exploring strongly interacting quantum systems, both in free space and in structured electromagnetic environments, with growing applications in quantum technology. Accurately modeling their…
We demonstrate a single-photon Rydberg excitation spectroscopy of cesium (Cs) atoms in a room-temperature vapor cell. Cs atoms are excited directly from 6S1/2 ground state to nP3/2 (n = 70 - 100) Rydberg states with a 318.6 nm ultraviolet…
Ensembles of atoms interacting via their Rydberg levels, known as "superatoms" for their ability to encode qubits and to emit single photons, attract increasing attention as building blocks for quantum network nodes. Assessing their…
Collisional and thermal ionization of sodium nS and nD Rydberg atoms with n=8-20 has been studied. The experiments were performed using a two-step pulsed laser excitation in an effusive atomic beam at atom density of about 2 10^{10}…
Optically trapped Rydberg atoms are a suitable platform to explore quantum many-body physics mediated by long-range atom--atom interactions that can be engineered through externally applied light fields. However, this approach is limited to…
We have observed resonant energy transfer between cold Rydberg atoms in spatially separated cylinders. Resonant dipole-dipole coupling excites the 49s atoms in one cylinder to the 49p state while the 41d atoms in the second cylinder are…
Dipole-dipole interactions between helium atoms in Rydberg-Stark states with principal quantum number $n=53$ and approximately linear Stark energy shifts, resulting from induced electric dipole moments of approximately 7900 D, have been…