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Self- and cross-correlation dynamics of deeply supercooled liquids were recently identified using photon correlation spectroscopy and spin relaxometry on the one hand, and using dielectric investigations on the other. These results fueled a…

Soft Condensed Matter · Physics 2021-03-09 K. Moch , P. Münzner , R. Böhmer , C. Gainaru

We discuss a novel approach, the point-to-set correlation functions, that allows to determine relevant static and dynamic length scales in glass-forming liquids. We find that static length scales increase monotonically when the temperature…

Disordered Systems and Neural Networks · Physics 2013-07-04 Walter Kob , Sandalo Roldan-Vargas , Ludovic Berthier

Rigidity plays an important role on the relaxation properties of glass forming melts, yet it is usually determined from the average co-ordination number through the chemical composition. A discussion is presented on how viscoelasticity can…

Soft Condensed Matter · Physics 2019-06-06 J. Quetzalcoatl Toledo-Marin , Gerardo G. Naumis

In an attempt to quantitatively characterize the recently observed slow dynamics in the isotropic and nematic phase of liquid crystals, we investigate the single-particle orientational dynamics of rodlike molecules across the…

Soft Condensed Matter · Physics 2009-11-13 Biman Jana , Dwaipayan Chakrabarti , Biman Bagchi

The structure, thermodynamics and slow activated dynamics of the equilibrated metastable regime of glass-forming fluids remains a poorly understood problem of high theoretical and experimental interest. We apply a highly accurate…

Soft Condensed Matter · Physics 2024-08-21 Subhashish Chaki , Baicheng Mei , Kenneth S. Schweizer

We introduce a new and robust approach for characterizing spatially and temporally heterogeneous behavior within a system based on the evolution of dynamic fuctuations once averaged over different space lengths and time scales. We apply it…

Disordered Systems and Neural Networks · Physics 2018-07-04 J. Ariel Rodriguez Fris , Eric R. Weeks , Francesco Sciortino , Gustavo A. Appignanesi

Particles in structural glasses rattle around temporary equilibriumpositions, that seldom change through a process which is much faster than the relaxation time, known as particle jump. Since the relaxation of the system is due to the…

Soft Condensed Matter · Physics 2015-11-03 Massimo Pica Ciamarra , Raffaele Pastore , Antonio Coniglio

Thermodynamic effects of local structure fluctuations in glassformers are analyzed in terms of energy basins and inter-basin hopping. Depending on the time-scale of measurement, one observes short-time thermodynamic properties related to a…

Statistical Mechanics · Physics 2007-05-23 Alexander Z. Patashinski , Mark A. Ratner

We study the relaxation process in a simple glass-former - the KA lattice gas model. We show that, for this model, structural relaxation is due to slow percolation of regions of co-operatively moving particles, which leads to heterogeneous…

Statistical Mechanics · Physics 2009-11-13 Pinaki Chaudhuri , Srikanth Sastry , Walter Kob

Granular simulations are used to probe the particle scale dynamics at short, intermediate, and long time scales for gravity driven, dense granular flows down an inclined plane. On approach to the angle of repose, where motion ceases, the…

Soft Condensed Matter · Physics 2009-11-11 L. E. Silbert

If a hierarchy of interatomic interactions exists in a solid, low-frequency modes can be found from viewing this solid as a mechanical network. In this case, the low-frequency modes are determined by the network rigidity. We study the…

Disordered Systems and Neural Networks · Physics 2008-05-12 Kostya Trachenko , Martin T Dove

We develop a framework for understanding the difference between strong and fragile behavior in the dynamics of glass-forming liquids from the properties of the potential energy landscape. Our approach is based on a master equation…

Disordered Systems and Neural Networks · Physics 2015-05-30 Sumilan Banerjee , Chandan Dasgupta

Using video microscopy, we measure local spatial constraints in disordered binary colloidal samples, ranging from dilute fluids to jammed glasses, and probe their spatial and temporal correlations to local dynamics during the glass…

Soft Condensed Matter · Physics 2019-07-03 Xiunan Yang , Hua Tong , Wei-Hua Wang , Ke Chen

We present a detailed investigation of the wave vector dependence of collective atomic motion in Au49Cu26.9Si16.3Ag5.5Pd2.3 and Pd42.5Cu27Ni9.5P21 supercooled liquids close to the glass transition temperature. Using x-ray photon correlation…

The slow dynamics for a colloidal suspension of particles interacting with a hard-core repulsion complemented by a short-ranged attraction is discussed within the frame of mode-coupling theory for ideal glass transitions for parameter…

Soft Condensed Matter · Physics 2007-05-23 Matthias Sperl

Atomistic deformation simulations in the nominally elastic regime are performed for a model binary glass with strain rates as low as $10^{4}$/sec (corresponding to 0.01 shear strain per 1$\mu$sec). A robust elasticity is revealed that…

Soft Condensed Matter · Physics 2020-11-21 P. M. Derlet , R. Maass

We analyze data from confocal microscopy experiments of a colloidal suspension to validate predictions of rapid sporadic events responsible for structural relaxation in a glassy sample. The trajectories of several thousand colloidal…

Soft Condensed Matter · Physics 2011-12-08 J. Ariel Rodriguez Fris , Gustavo A. Appignanesi , Eric R. Weeks

It is experimentally shown that, depending on the carrier-concentration of the system $n$, the dynamics of electron-glasses either \textit{slows down }with increasing temperature or it is \textit{independent} of it. This also correlates…

Strongly Correlated Electrons · Physics 2007-11-28 Z. Ovadyahu

We investigate by Molecular-Dynamics simulations the fast mobility - the rattling amplitude of the particles temporarily trapped by the cage of the neighbors - in mildly supercooled states of dense molecular (linear trimers) and atomic…

Fluid Dynamics · Physics 2016-05-04 S. Bernini , F. Puosi , D. Leporini

We present a derivation of a recently proposed theory for the time dependence of density fluctuations in stationary states of strongly interacting, athermal, self-propelled particles. The derivation consists of two steps. First, we start…

Soft Condensed Matter · Physics 2016-01-13 Grzegorz Szamel