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We describe the temporal evolution of the time-resolved photoemission response of the spinless Falicov-Kimball model driven out of equilibrium by strong applied fields. The model is one of the few possessing a metal-insulator transition and…

Strongly Correlated Electrons · Physics 2010-04-23 B. Moritz , T. P. Devereaux , J. K. Freericks

The breakdown of Hooke's law marks the onset of nonlinear behaviour: when displacements become large, restoring forces weaken and conventional proportionality fails. In quantum materials, intense optical excitation can drive the crystal…

Combining quasistatic and time-resolved transport measurements with X-ray and neutron diffraction experiments we study the non-equilibrium states that arise in pure and in Ti substituted Ca$_2$RuO$_4$ under the application of current…

Strongly Correlated Electrons · Physics 2020-08-12 K. Jenni , F. Wirth , K. Dietrich , L. Berger , Y. Sidis , S. Kunkemöller , C. P. Grams , D. I. Khomskii , J. Hemberger , M. Braden

Ultrafast laser excitation of a metal causes correlated, highly nonequilibrium dynamics of electronic and ionic degrees of freedom, which are however only poorly captured by the widely-used two-temperature model. Here we develop an…

Materials Science · Physics 2017-12-06 Pablo Maldonado , Karel Carva , Martina Flammer , Peter M. Oppeneer

High-resolution thermal expansion measurements have been performed for exploring the mysterious "structureless transition" in (TMTTF)$_{2}$X (X = PF$_{6}$ and AsF$_{6}$), where charge ordering at $T_{CO}$ coincides with the onset of…

Strongly Correlated Electrons · Physics 2008-11-24 M. de Souza , P. Foury-Leylekian , A. Moradpour , J. -P. Pouget , M. Lang

Understanding nonequilibrium electron-phonon interactions at the microscopic level and on ultrafast timescales is a central goal of modern condensed matter physics. Combining time- and angle-resolved extreme ultraviolet photoemission…

The electronic and structural properties of a material are strongly determined by its symmetry. Changing the symmetry via a photoinduced phase transition offers new ways to manipulate material properties on ultrafast timescales. However, in…

Strongly Correlated Electrons · Physics 2015-09-25 Simon Wall , Daniel Wegkamp , Laura Foglia , Joyeeta Nag , Richard F. Haglund , Julia Staehler , Martin Wolf

A wide variety of experimental results and theoretical investigations in recent years have convincingly demonstrated that several transition metal oxides and other materials, have dominant states that are not spatially homogeneous. This…

Strongly Correlated Electrons · Physics 2009-11-11 Elbio Dagotto

We use a Langevin approach to treat the finite temperature dynamics of displacement variables in the half-filled spinless Holstein model. Working in the adiabatic regime we exploit the smallness of the adiabatic parameter to simplify the…

Strongly Correlated Electrons · Physics 2019-05-02 Sauri Bhattacharyya , Sankha Subhra Bakshi , Samrat Kadge , Pinaki Majumdar

We relate the phase separation observed in many crystals with pronounced electron correlations to the regions of negative electron compressibility. They were found in several models describing strong electron correlations. At low…

Strongly Correlated Electrons · Physics 2022-10-25 Alexei Sherman

A model of coupled molecular oscillators is proposed to study nonequilibrium thermodynamics of synchronization. We find that synchronization of nonequilibrium oscillators costs energy even when the oscillator-oscillator coupling is…

Biological Physics · Physics 2020-01-29 Dongliang Zhang , Yuansheng Cao , Qi Ouyang , Yuhai Tu

Fluctuations in the energy gap and coupling constants in and between chromophores can play important role in the absorption and energy transfer across a collection of two level systems. In a noisy environment, fluctuations can control…

Chemical Physics · Physics 2024-04-17 Rajesh Dutta , Biman Bagchi

We examine electron-electron mediated relaxation following excitation of a correlated system by an ultrafast electric field pump pulse. The results reveal a dichotomy in the temporal evolution as one tunes through a Mott metal-to-insulator…

Strongly Correlated Electrons · Physics 2013-08-20 B. Moritz , A. F. Kemper , M. Sentef , T. P. Devereaux , J. K. Freericks

Understanding the microscopic spatio-temporal dynamics of nonequilibrium charge carriers in heterosystems promises optimization of process and device design towards desired energy transfer. Hot electron transport is governed by scattering…

We investigate the excitation of phonons in photoexcited antimony and demonstrate that the entire electron-lattice interactions, in particular coherent and incoherent electron-phonon coupling, can be probed simultaneously. Using femtosecond…

We investigate the potential of a quantum Boltzmann equation without momentum conservation for description of strongly correlated electron systems out of equilibrium. In a spirit similar to dynamical mean field theory (DMFT), the momentum…

Strongly Correlated Electrons · Physics 2018-11-07 Michael Wais , Martin Eckstein , Roland Fischer , Philipp Werner , Marco Battiato , Karsten Held

Ultrafast perturbations offer a unique tool to manipulate correlated systems due to their ability to promote transient behaviors with no equilibrium counterpart. A widely employed strategy is the excitation of coherent optical phonons, as…

Superconductivity · Physics 2018-01-24 Michael Schütt , Peter P. Orth , Alex Levchenko , Rafael M. Fernandes

Photoexcitation by ultrashort laser pulses plays a crucial role in controlling reaction pathways, creating nonequilibrium material properties, and offering a microscopic view of complex dynamics at the molecular level. The photo response…

Two-pulse correlation experiments performed using pulses of different intensities on Pd(111) with different CO coverages showed that the CO photodesorption probability depends on whether the strong or the weak pulse arrives first to the…

Phase transitions and the associated symmetry breaking are at the heart of many physical phenomena. Coupled systems with multiple interacting degrees of freedom provide a fertile ground for emergent dynamics that is otherwise inaccessible…