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Collective modes of doped two-dimensional crystalline materials, namely graphene, MoS$_2$ and phosphorene, both monolayer and bilayer structures, are explored using the density functional theory simulations together with the random phase…

Mesoscale and Nanoscale Physics · Physics 2018-02-06 Zahra Torbatian , Reza Asgari

We report a combined theoretical/experimental study of dynamic screening of excitons in media with frequency-dependent dielectric functions. We develop an analytical model showing that interparticle interactions in an exciton are screened…

Mesoscale and Nanoscale Physics · Physics 2017-03-16 Andrey R. Klots , Benjamin Weintrub , Dhiraj Prasai , Daniel Kidd , Kalman Varga , Kirill A. Velizhanin , Kirill I. Bolotin

We show how to calculate the optical functions of a nanoplatelet, taking into account the effect of a dielectric confinement on excitonic states. Real density matrix approach is employed to obtain analytical and semi-analytical relations…

Excitonic effects play a particularly important role in the optoelectronic behavior of two-dimensional (2D) semiconductors. To facilitate the interpretation of experimental photoabsorption and photoluminescence spectra we provide…

Mesoscale and Nanoscale Physics · Physics 2018-01-04 M. Szyniszewski , E. Mostaani , N. D. Drummond , V. I. Fal'ko

We present a theory of excitonic processes in gate controlled graphene quantum dots. The dependence of the energy gap on shape, size and edge for graphene quantum dots with up to a million atoms is predicted. Using a combination of…

Mesoscale and Nanoscale Physics · Physics 2015-05-19 A. D. Guclu , P. Potasz , P. Hawrylak

The formation and disassociation of excitons plays a crucial role in any photovoltaic or photocatalytic application. However, excitonic effects are seldom considered in materials discovery studies due to the monumental computational cost…

Materials Science · Physics 2021-03-16 Tathagata Biswas , Arunima K. Singh

In 2D materials, the quantum confinement and van der Waals-type interlayer interactions largely govern the fundamental electronic and optical properties, and the dielectric screening plays a dominant role in the excitonic properties. This…

Mesoscale and Nanoscale Physics · Physics 2021-02-19 Guowei Zhang , Shenyang Huang , Fanjie Wang , Hugen Yan

Experimental evidence of strong coupling between excitons confined in a quantum well and the photonic modes of a two-dimensional dielectric lattice is reported. Both resonant scattering and photoluminescence spectra at low temperature show…

We have developed a theory of exciton-polariton band structure of resonant three-dimensional photonic crystals for arbitrary dielectric contrast and effective mass of the exciton that is excited in one of the compositional materials. The…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 E. L. Ivchenko , A. N. Poddubny

We study the coherent light-matter interactions of GaAs quantum wells associated with excitons, biexcitons and many-body effects. For most polarization configurations, excitonic features dominate the phase-resolved two-dimensional…

Other Condensed Matter · Physics 2011-12-13 Alan D. Bristow , Denis Karaiskaj , Xingcan Dai , Richard. P. Mirin , Steven T. Cundiff

Optical responses of atomically thin 2D materials are greatly influenced by electron-hole interactions. It is by far established that exciton signatures can be well-identified in the optical absorption spectrum of quasi-2D materials.…

Mesoscale and Nanoscale Physics · Physics 2023-10-30 Yu-Tzu Chang , Yang-Hao Chan

A major obstacle for computing optical spectra of solids is the lack of reliable approximations for capturing excitonic effects within time-dependent density-functional theory. We show that the trustful prediction of strongly bound…

We present an analytical investigation of the optical absorption spectrum of monolayer molybdenumdisulfide. Based on the density matrix formalism, our approach gives insights into the microscopic origin of excitonic transitions, their…

Materials Science · Physics 2014-03-24 Gunnar Berghäuser , Ermin Malic

Excitonic effects play a particularly important role in the optoelectronic behavior of two-dimensional semiconductors. To facilitate the interpretation of experimental photoabsorption and photoluminescence spectra we provide (i)…

Mesoscale and Nanoscale Physics · Physics 2017-08-23 E. Mostaani , M. Szyniszewski , C. H. Price , R. Maezono , M. Danovich , R. J. Hunt , N. D. Drummond , V. I. Fal'ko

Exciton problem is solved in the two-dimensional Dirac model with allowance for strong electron-hole attraction. The exciton binding energy is assumed smaller than but comparable to the band gap. The exciton wavefunction is found in the…

Mesoscale and Nanoscale Physics · Physics 2020-10-28 N. V. Leppenen , L. E. Golub , E. L. Ivchenko

The exciton binding energy, the energy required to dissociate an excited electron-hole pair into free charge carriers, is one of the key factors to the optoelectronic performance of organic materials. However, it remains unclear whether…

Chemical Physics · Physics 2015-12-08 Jui-Che Lee , Jeng-Da Chai , Shiang-Tai Lin

The anisotropic nature of the new two-dimensional (2D) material phosphorene, in contrast to other 2D materials such as graphene and transition metal dichalcogenide (TMD) semiconductors, allows excitons to be confined in a…

The optical excitation spectra and excitonic resonances are investigated in systematically functionalized SiC with Fluorine and/or Chlorine utilizing density functional theory in combination with many-body perturbation theory. The latter is…

Materials Science · Physics 2017-11-22 L. B. Drissi , F. Z. Ramadan , S. Lounis

Various properties of interlayer excitons in double-layer transition metal dichalcogenides quantum dots are analyzed using a low-energy effective Hamiltonian with Coulomb interaction. We solve the single-particle Hamiltonian with and…

Mesoscale and Nanoscale Physics · Physics 2024-08-15 Xiang Liu , Zheng Tao , Wenchen Luo , Tapash Chakraborty

Many-body interactions between quasiparticles (electrons, excitons, and phonons) have led to the emergence of new complex correlated states and are at the core of condensed matter physics and material science. In low-dimensional materials,…