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Using a combination of single-crystal neutron scattering and reverse Monte Carlo refinements, we study the magnetic structure of paramagnetic MnO at a temperature (160\,K) substantially below the Curie-Weiss temperature…

We show that the improper ferroelectric phase transition in the multiferroic hexagonal manganites displays the same symmetry-breaking characteristics as those proposed in early-universe theories. We present an analysis of the Kibble-Zurek…

Materials Science · Physics 2021-03-09 S. M. Griffin , M. Lilienblum , K. Delaney , Y. Kumagai , M. Fiebig , N. A. Spaldin

Identification of novel multiferroic materials with high-ordering temperatures remains at the forefront of condensed matter physics research. In this regard, the antiferromagnetic RCrO$_3$ compounds (like GdCrO$_3$) constitute a promising…

Experimental and theoretical studies of unusual polar, dielectric and magnetic properties of room temperature multiferroics, such as perovskites Pb(Fe$_{1/2}$Nb$_{1/2}$)O$_3$ (PFN) and Pb(Fe$_{1/2}$Ta$_{1/2}$)O$_3$ (PFT), are very…

Neutron scattering techniques have been used to study the relaxor ferroelectric 0.68PbMg1/3Nb2/3O3-0.32PbTiO3 denoted in this paper as 0.68PMN-0.32PT. On cooling, these relaxor ferroelectrics have a long-range ordered ferroelectric phase…

Materials Science · Physics 2007-05-23 S. N. Gvasaliya , B. Roessli , R. A. Cowley , S. Kojima , S. G. Lushnikov

Deterministic polarization reversal in ferroelectric and multiferroic films is critical for their exploitation in nanoelectronic devices. While ferroelectricity has been studied for nearly a century, major discrepancies in the reported…

Like most perovskites, SrRuO$_3$ exhibits structural phase transitions associated with rotations of the RuO$_6$ octahedra. The application of moderate magnetic fields in the ferromagnetically ordered state allows one to fully control these…

Materials Science · Physics 2017-12-27 S. Kunkemöller , D. Brüning , A. Stunault , A. A. Nugroho , T. Lorenz , M. Braden

The subtle interplay of randomness and quantum fluctuations at low temperatures gives rise to a plethora of unconventional phenomena in systems ranging from quantum magnets and correlated electron materials to ultracold atomic gases.…

Disordered Systems and Neural Networks · Physics 2014-01-15 L. Demko , S. Bordacs , T. Vojta , D. Nozadze , F. Hrahsheh , C. Svoboda , B. Dora , H. Yamada , M. Kawasaki , Y. Tokura , I. Kezsmarki

We have investigated the effects of substituting In for Mn on the antiferromagnetic phase transition in YMnO3 using magnetic, dielectric, and specific heat measurements. We prepared a set of isostructural phase pure hexagonal…

Materials Science · Physics 2015-05-14 A. Dixit , Andrew E. Smith , M. A. Subramanian , G. Lawes

Cu3Nb2O8 is an unusual multiferroic compound that undergoes a series of magnetic ordering at low temperatures. Concurrent development of electric polarization has been reported at TN1 ~25 K corresponding to a non-collinear helicoidal…

Strongly Correlated Electrons · Physics 2015-06-22 G. Sharma , J. Saha , S. D. Kaushik , V. Siruguri , S. Patnaik

Room-temperature ferrimagnetism was discovered for the anti-site-disordered perovskite Ca2MnOsO6 with Tc = 305 K. Ca2MnOsO6 crystallizes into an orthorhombic structure with a space group of Pnma, in which Mn and Os share the…

We have investigated the temperature-dependent changes in the near-$E$$_F$ occupied and unoccupied states of Pr$_{0.67}$Ca$_{0.33}$MnO$_3$ which shows the presence of ferromagnetic and antiferromagnetic phases. The temperature-dependent…

Strongly Correlated Electrons · Physics 2009-11-11 M. K. Dalai , P. Pal , B. R. Sekhar , N. L. Saini , R. K. Singhal , K. B. Garg , B. Doyle , S. Nannarone , C. Martin , F. Studer

We show that the transition in AMnO3 from the orthorhombic perovskite phase to the hexagonal phase is promoted by inducing disorder on the A-site. The gap between the orthorhombic and the hexagonal phase is widened for disordered, mixed…

Strongly Correlated Electrons · Physics 2007-05-23 Jan-Willem Bos , Bas B. van Aken , Thomas T. M. Palstra

The temperature dependent local structure of TbMn2O5 was determined by x-ray absorption spectroscopy. An anomalous Tb-O distribution is found. At high temperature it is broad but resolves into two distinct peaks below approximately 180 K.…

Strongly Correlated Electrons · Physics 2009-11-13 T. A. Tyson , M. Deleon , S. Yoong , S. -W. Cheong

We study the finite-temperature transition in a model XY antiferromagnet on a pyrochlore lattice, which describes the pyrochlore material Er2Ti2O7. The ordered magnetic structure selected by thermal fluctuations is six-fold degenerate.…

Strongly Correlated Electrons · Physics 2014-04-15 M. E. Zhitomirsky , P. C. W. Holdsworth , R. Moessner

We revealed the anomalous temperature behavior of the giant dielectric permittivity and unusual frequency dependences of the pyroelectric response of the fine-grained ceramics prepared by the spark plasma sintering of the ferroelectric…

The low temperature phase of single crystals of Nd$_{0.5}$Ca$_{0.5}$MnO$_3$ and Gd$_{0.5}$Ca$_{0.5}$MnO$_3$ manganites is investigated by squid magnetometry. Nd$_{0.5}$Ca$_{0.5}$MnO$_3$ undergoes a charge-ordering transition at…

Materials Science · Physics 2016-08-31 R. Mathieu , P. Nordblad , A. R. Raju , C. N. R. Rao

We report inelastic neutron scattering results on the spin dynamics in the 50 % hole-doped manganites, Pr{1/2}Sr{1/2}MnO3 and Nd{1/2}Sr{1/2}MnO3. In the paramagnetic phase, these systems exhibit a ridge-type diffuse scattering, indicating a…

Strongly Correlated Electrons · Physics 2007-05-23 H. Kawano , R. Kajimoto , H. Yoshizawa , Y. Tomioka , H. Kuwahara , Y. Tokura

The perovskite oxide EuTiO3 (ETO) has attracted increased scientific interest due to its potential multiferroic properties and magnetic activity above and below its structural phase transition at TS=282K. Various experiments have indirectly…

We report an infrared reflection spectroscopy study of La$_{1/2}$Ca$_{1/2}$MnO$_3$ over a broad frequency range and temperature interval which covers the transitions from the high temperature paramagnetic to ferromagnetic and, upon further…

Strongly Correlated Electrons · Physics 2009-11-10 A. P. Litvinchuk , M. N. Iliev , M. Pissas , C. W. Chu