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We explore the impact of a magnetic field on the ferroelectric domain pattern in polycrystalline hexagonal ErMnO3 at cryogenic temperatures. Utilizing piezoelectric force microscopy measurements at 1.65 K, we observe modifications of the…

Materials Science · Physics 2024-03-21 J. Schultheiß , L. Puntigam , M. Winkler , S. Krohns , D. Meier , H. Das , D. M. Evans , I. Kézsmárki

Structural, magnetic and electric properties of a metal-ordered perovskite YBaMn2O6 have been studied by means of powder X-ray diffraction, DSC, magnetic susceptibility, and electric resistivity. It is found that this material undergoes a…

Strongly Correlated Electrons · Physics 2009-11-07 T. Nakajima , H. Kageyama , Y. Ueda

Magnetically-driven ferroelectric atomic displacements of the order of 10$^{-3} Angstrom have been observed in orthorhombic (perovskite like) YMnO$_3$ by a single-crystal synchrotron x-ray diffraction. The refined polar structure shows the…

Strongly Correlated Electrons · Physics 2011-08-12 D. Okuyama , S. Ishiwata , Y. Takahashi , K. Yamauchi , S. Picozzi , K. Sugimoto , H. Sakai , M. Takata , R. Shimano , Y. Taguchi , T. Arima , Y. Tokura

We observe a seemingly complex magnetic field dependence of dielectric constant of hexagonal YbMnO3 near the spin ordering temperature. After rescaling, the data taken at different temperatures and magnetic fields collapse on a single curve…

Materials Science · Physics 2008-12-01 U. Adem , M. Mostovoy , N. Bellido , A. A. Nugroho , Ch. Simon , T. T. M. Palstra

While defects are unavoidable in crystals and often detrimental to material performance, they can be a key ingredient for inducing functionalities when tailored. Here, we demonstrate that an A-site-deficient perovskite Y$_{1/3}$TaO$_3$…

We have studied the influence of antiferromagnetic ordering on the local dielectric moments of the MnO_5 and LuO_7 polyhedra by measuring neutron powder diffraction patterns of LuMnO_3 at temperatures near T_N. We show that the coupling is…

Strongly Correlated Electrons · Physics 2009-11-10 Bas B. Van Aken , Thomas T. M. Palstra

Structural features of ferroic domains are fundamentally important for the understanding of microstructure and physical properties of ferroic materials, and they are also of technological significance for information storage and electronic…

Materials Science · Physics 2012-05-22 J. Q. Li , J. Li , H. X. Yang , H. F. Tian , S-W. Cheong , C. Ma , S. Zhang , Y. G. Zhao

Coexistence of mutually influencing ferroelectric and magnetic ordering at low temperature in hexagonal phase of rare-earth manganites gives rise to interesting physical phenomena. Here, we report a detailed analysis of powder neutron…

Materials Science · Physics 2014-05-13 A. K. Singh , S. D. Kaushik , V. Siruguri , S. Patnaik

High harmonic generation from Pr$_{0.8}$Ca$_{0.2}$MnO$_{3}$ was investigated across a high-temperature paramagnetic phase and a low-temperature ferromagnetic phase. As the temperature decreases, the harmonic intensity gradually increases in…

Strongly Correlated Electrons · Physics 2025-01-27 A. Nakano , K. Uchida , Y. Tomioka , M. Takaya , Y. Okimoto , K. Tanaka

Several rare earth magnetic pyrochlore materials are well modeled by a spin-1/2 quantum Hamiltonian with anisotropic exchange parameters Js. For the Er2Ti2O7 material, the Js were recently determined from high-field inelastic neutron…

Strongly Correlated Electrons · Physics 2014-04-11 J. Oitmaa , R. R. P. Singh , A. G. R. Day , B. V. Bagheri , M. J. P. Gingras

Pure SrTiO3 in bulk form is known to be an incipient ferroelectric where the quantum fluctuations of lattice positions prevent long range ferroelectric ordering at a finite temperature. We show evidence and identify the origin of…

Strongly Correlated Electrons · Physics 2016-10-19 Vinay Kumar Shukla , Soumik Mukhopadhyay

We argue that the homogeneous distribution of spins in the spin-spiral state of orthorhombic manganites is deformed by the relativistic spin-orbit interaction. The thus induced spin-spiral inhomogeneity gives rise to the ferroelectric…

Materials Science · Physics 2011-02-10 I. V. Solovyev

The floating-zone method with different growth ambiances has been used to selectively obtain hexagonal or orthorhombic DyMnO$_{3}$ single crystals. The crystals were characterized by X-ray powder diffraction of ground specimen and a…

Strongly Correlated Electrons · Physics 2009-11-13 S Harikrishnan , S Roessler , C M Naveen Kumar , H L Bhat , U K Roessler , S Wirth , F Steglich , Suja Elizabeth

Ferroelectricity has been found to occur in several insulating systems, such as TbMnO$_3$ (TMO) and Ni$_3$V$_2$O$_8$ (NVO) which have more than one phase with incommensurately modulated long-range magnetic order. Here we give a…

Materials Science · Physics 2009-11-11 A. Brooks Harris

Single crystal synthesis, structure, electric polarization and heat capacity measurements on hexagonal InMnO3 show that this small R ion in the RMnO3 series is ferroelectric (space group P63cm). Structural analysis of this system reveals a…

Materials Science · Physics 2015-06-15 T. Yu , P. Gao , T. Wu , T. A. Tyson , R. Lalancette

Trimerization-polarization domains in ferroelectric hexagonal YMnO$_3$ were resolved in all three spatial dimensions by piezoresponse force microscopy. Their topology is dominated by electrostatic effects with a range of 100 unit cells and…

Materials Science · Physics 2015-05-27 Tobias Jungk , Ákos Hoffmann , Manfred Fiebig , Elisabeth Soergel

Detailed structural measurements were conducted on a new perovskite, ScMnO3, and on orthorhombic LuMnO3. Complementary density functional theory (DFT) calculations were carried out, and predict that ScMnO3 possesses E-phase magnetic order…

Strongly Correlated Electrons · Physics 2015-06-19 T. Yu , T. A. Tyson , H. Y. Chen , A. M. M. Abeykoon , Y. -S. Chen , K. H. Ahn

A complex magnetic order of the multiferroic compound Co3TeO6 has been revealed by neutron powder diffraction studies on ceramics and crushed single crystals. The compound adopts a monoclinic structure (s.g. C2/c) in the studied temperature…

Materials Science · Physics 2011-11-28 S. A. Ivanov , R. Tellgren , C. Ritter , P. Nordblad , R. Mathieu , G. Andre , N. V. Golubko , E. D. Politova , M. Weil

Nominally pure undoped parent manganite LaMnO_3 exhibits a puzzling behavior inconsistent with a simple picture of an A-type antiferromagnetic insulator (A-AFI) with a cooperative Jahn-Teller ordering. We do assign its anomalous properties…

Strongly Correlated Electrons · Physics 2015-05-19 A. S. Moskvin

Domain walls (DWs) in ferroic materials, across which the order parameter abruptly changes its orientation, can host emergent properties that are absent in the bulk domains. Using a broadband ($10^6-10^{10}$ Hz) scanning impedance…

Mesoscale and Nanoscale Physics · Physics 2018-03-30 Xiaoyu Wu , Urko Petralanda , Lu Zheng , Yuan Ren , Rongwei Hu , Sang-Wook Cheong , Sergey Artyukhin , Keji Lai