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Hexagonal manganites are multiferroic materials with two highly-dissimilar phase transitions: a ferroelectric transition (from P63/mmc to P63cm) at a temperature higher than 1000 K and an antiferromagnetic transition at TN=65 - 130 K.…

Strongly Correlated Electrons · Physics 2018-02-20 Hasung Sim , Jaehong Jeong , Haeri Kim , S-W Cheong , Je-Geun Park

As the result of the high-temperature improper ferroelectric transition occurring in YMnO3 and other hexagonal manganites a striking domain pattern was observed: an emergence of six domains of alternating polarization from one point in a…

Strongly Correlated Electrons · Physics 2014-01-31 Bruno Mettout , Pierre Toledano , Martin Lilienblum , Manfred Fiebig

We report a detailed high-resolution powder neutron diffraction investigation of the structural behaviour of the multiferroic hexagonal polymorph of YMnO3 between room temperature and 1403 K. The study was aimed at resolving previous…

Materials Science · Physics 2015-05-19 Alexandra S. Gibbs , Kevin S. Knight , Philip Lightfoot

Hexagonal RMnO3 manganites are improper ferroelectrics in which the electric polarization is a by-product of the tripling of the unit cell. In YMnO3, there is a second transition at ~ 920K whose nature remains unexplained. We argue that…

Materials Science · Physics 2014-08-12 A. Cano

The local atomic disorder and the electronic structure in the environment of manganese atoms in LaMnO_3 has been studied by x-ray absorption spectroscopy, over a temperature range (300K to 870K) covering the orbital ordering transition…

Strongly Correlated Electrons · Physics 2009-11-10 Raquel A. Souza , Narcizo M. Souza-Neto , Aline Y. Ramos , Helio C. N. Tolentino , Eduardo Granado

Improper ferroelectrics are described by two order parameters: a primary one, driving a transition to long-range distortive, magnetic or otherwise non-electric order, and the electric polarization, which is induced by the primary order…

The structural phase transition in hexagonal BaMnO$_3$ occurring at $T_c$=130 K was studied in ceramic samples using electron and X-ray diffraction, second harmonic generation as well as by dielectric and lattice dynamic spectroscopies. The…

We report the magnetic susceptibility, specific heat and dielectric constant on high purity polycrystalline samples of three hexagonal manganites: YMnO_3, LuMnO_3 and ScMnO_3. These materials can exhibit a ferroelectric transition at very…

Materials Science · Physics 2007-05-23 D. G. Tomuta , S. Ramakrishnan , G. J. Nieuwenhuys , J. A. Mydosh

In this work we explore the overall structural behaviour of the [(CH3)2NH2][Mn(HCOO)3] multiferroic compound across the temperature range where its ferroelectric transition takes place by means of calorimetry, thermal expansion measurements…

The controversy regarding the ferroelectric behavior of hexagonal InMnO$_3$ is resolved by using a combination of x-ray diffraction (XRD), piezoresponse force microscopy (PFM), second harmonic generation (SHG), and density functional theory…

Materials Science · Physics 2013-05-30 Yu Kumagai , Alexei A. Belik , Martin Lilienblum , Naëmi Leo , Manfred Fiebig , Nicola A. Spaldin

A re-entrant novel phase has been observed in the hexagonal ferroelectric HoMnO3 in the presence of magnetic fields, in the temperature ranges defined by the plateau of the dielectric constant anomaly. The dielectric plateau evolves with…

Strongly Correlated Electrons · Physics 2009-11-10 B. Lorenz , A. P. Litvinchuk , M. M. Gospodinov , C. W. Chu

The ferroelectric phase of the multiferroic hexagonal manganites (h-ReMnO3) has been reported to undergo a series of magnetic transitions involving long-range ordering/reorientation of 4fRe3+ and/or 3dMn3+ spins below room temperature.…

We present results of local spin density approximation pseudopotential calculations for the ferroelectromagnet, yttrium manganite (YMnO3). The origin of the differences between ferroelectric and non-ferroelectric perovskite manganites is…

Materials Science · Physics 2015-06-25 Alessio Filippetti , Nicola A. Hill

We study the interplay of structural and polar distortions in hexagonal YMnO3 and short-period PbTiO3/SrTiO3 superlattices by means of first-principles calculations at constrained electric displacement field D. We find that in YMnO3 the…

Materials Science · Physics 2015-06-05 Massimiliano Stengel , Craig J. Fennie , Philippe Ghosez

Using first-principles calculations, we study theoretically the stable 2H hexagonal structure of BaMnO3. We show that from the stable high temperature P63/mmc structure, the compound should exhibit an improper ferroelectric structural phase…

Materials Science · Physics 2015-06-15 Julien Varignon , Philippe Ghosez

We have investigated dielectric properties in a series of crystals of $R$MnO$_{3}$ ($R$ is a rare earth ion) under magnetic fields and quasihydrostatic pressure. We have found that ferroelectric phase appeared in GdMnO$_3$ crystal below…

Strongly Correlated Electrons · Physics 2009-11-10 H. Kuwahara , K. Noda , J. Nagayama , S. Nakamura

Two magnetic ordering transitions are found in InMnO3, the paramagnetic to antiferromagnetic transition near ~118 K and a lower possible spin rotation transition near ~42 K. Multiple length scale structural measurements reveal enhanced…

Materials Science · Physics 2015-06-22 T. Yu , T. A. Tyson , P. Gao , T. Wu , X. Hong , S. Ghose , Y. -S. Chen

We have identified, for the first time, the change in symmetry at the ferroelectric transition TFE near 1023K of the ferroelectromagnet YMnO3. This transition takes place 300K below the transition to the centrosymmetric state at TIP. Single…

Materials Science · Physics 2007-05-23 Gwilherm Nenert , Yang Ren , Harold T. Stokes , Thomas T. M. Palstra

New metal-ordered manganites RBaMn_{2}O_{6} have been synthesized and investigated in the structures and electromagnetic properties. RBaMn_{2}O_{6} can be classified into three groups from the structural and electromagnetic properties. The…

Strongly Correlated Electrons · Physics 2009-11-07 T. Nakajima , H. Kageyama , H. Yoshizawa , Y. Ueda

Synchrotron X-ray diffraction patterns were measured and analyzed for a polycrystalline sample of the room-temperature ferromagnet Sr3.12Er0.88Co4O10.5 from 300 to 650 K, from which two structural phase transitions were found to occur…

Strongly Correlated Electrons · Physics 2009-11-13 Shintaro Ishiwata , Wataru Kobayashi , Ichiro Terasaki , Kenichi Kato , Masaki Takata
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