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The momentum-space signatures of excitons can be experimentally accessed through time-resolved (pump-probe) photoelectron spectroscopy. In this work, we develop a computational framework for exciton photoemission orbital tomography (exPOT)…

Magnetoelectroluminescence (MEL) of organic semiconductor has been experimentally tuned by adopting blended emitting layer consisting of both hole and electron transporting materials. A theoretical model considering intermolecular quantum…

Materials Science · Physics 2015-05-14 B. F. Ding , Y. Yao , X. Y. Sun , Z. Y. Sun , X. D. Gao , Z. T. Xie , Z. J. Wang , X. M. Ding , Y. Z. Wu , X. F. Jin , C. Q. Wu , X. Y. Hou

The optical dielectric function of ZnGeN$_2$ is calculated from the interband transitions using the energy bands calculated in the quasiparticle self-consistent (QS)$G\hat W$ method using two different levels of approximation: the…

Materials Science · Physics 2024-03-22 Ozan Dernek , Walter R. L. Lambrecht

Environmental dielectric screening effects on exciton transition energies in single-walled carbon nanotubes (SWNTs) have been studied quantitatively in the range of dielectric constants from 1.0 to 37 by immersing SWNTs bridged over…

We have investigated excitons in highly-aligned single-walled carbon nanotubes (SWCNTs) through optical spectroscopy at low temperature (1.5 K) and high magnetic fields ($\textbf{\textit{B}}$) up to 55 T. SWCNT/polyacrylic acid films were…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 J. Shaver , S. A. Crooker , J. A. Fagan , E. K. Hobbie , N. Ubrig , O. Portugall , V. Perebeinos , Ph. Avouris , J. Kono

We present evidence of all optical trion generation and emission in undoped single walled carbon nanotubes (SWCNTs). Luminescence spectra, recorded on individual SWCNTs over a large CW excitation intensity range, show trion emission peaks…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 Silvia Santos , Bertrand Yuma , Stéphane Berciaud , Jonah Shaver , Mathieu Gallart , Pierre Gilliot , Laurent Cognet , Brahim Lounis

Statistics of photons emitted by mobile excitons in individual carbon nanotubes are investigated. Photoluminescence spectroscopy is used to identify the chiralities and suspended lengths of air-suspended nanotubes, and photon correlation…

Mesoscale and Nanoscale Physics · Physics 2017-11-28 A. Ishii , T. Uda , Y. K. Kato

The development of high-performance electron sources requires theoretical frameworks that accurately link the microscopic electronic properties of cathode materials to their macroscopic photoemission observables. Here, we present a…

Materials Science · Physics 2026-02-16 Richard Schier , Chen Wang , Jonas Dube , Julius Kühn , Alice Galdi , Thorsten Kamps , Caterina Cocchi

We demonstrate a class of model nano-electromechanical systems (NEMS) based on multiwalled carbon nanotubes (MWNTs) which has longer inner cores coaxially oscillating inside their respective shorter outer shell holders and can operate at…

Materials Science · Physics 2007-09-26 Quan-shui Zheng , Zhiping Xu , Adrian Neild , Tuck Wah Ng

The nonlocal correlation mechanism between excitonic pairs is considered for a two dimensional exciton system. On the base of the unitary decomposition of the usual electron operator, we include the electron phase degrees of freedom into…

Strongly Correlated Electrons · Physics 2015-08-04 V. Apinyan , T. K. Kopeć

We show that the photoluminescence intensity of single-walled carbon nanotubes is much stronger in tubes with large chiral angles - armchair tubes - because exciton resonances make the luminescence of zigzag tubes intrinsically weak. This…

Materials Science · Physics 2009-11-11 Stephanie Reich , Christian Thomsen , John Robertson

We report that dark excitons can have a large contribution to the emission intensity in carbon nanotubes due to an efficient exciton conversion from a dark state to a bright state. Time-resolved photoluminescence measurements are used to…

Mesoscale and Nanoscale Physics · Physics 2019-12-11 A. Ishii , H. Machiya , Y. K. Kato

In many field electron emission experiments on single-walled carbon nanotubes (SWCNTs), the SWCNT stands on one of two well-separated parallel plane plates, with a macroscopic field FM applied between them. For any given location "L" on the…

"Metallic" carbon nanotubes exhibit quasiparticle gaps when isolated from a screening environment. The gap-opening mechanism is expected to be of electronic origin, but the precise nature is debated. In this work, we show that hybrid…

Mesoscale and Nanoscale Physics · Physics 2018-11-14 Maria Hellgren , Jacopo Baima , Anissa Acheche

We propose a new formalism and an effective computational framework to study self-trapped excitons (STE) in insulators and semiconductors from first principles. Using the many-body Bethe-Salpeter equation in combination with perturbation…

Materials Science · Physics 2023-11-22 Yunfei Bai , Yaxian Wang , Sheng Meng

The distribution of rates of carrier multiplication (CM) following photon absorption is calculated for semiconductor nanocrystals (NCs). The NC electronic structure is described using a screened pseudopotential method known to give reliable…

Materials Science · Physics 2015-05-13 Eran Rabani , Roi Baer

We introduce a new simplified method for computing the electron field emission current in short carbon nanotubes using ab-initio computation in periodic simulation cells. We computed the evolution of the wave functions using Time-Dependent…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 Sherif Tawfik , Salah El Sheikh , Noha Salem

This paper reviews both experimental and theoretical work on nanostructures showing high quantum yields due to the phenomenon of multiple exciton generation. It outlines the aims and barriers to progress in identifying further such…

Mesoscale and Nanoscale Physics · Physics 2018-06-06 Nicholas Siemons , Alessio Serafini

An analytical expression is obtained for the biexciton binding energy as a function of the inter-exciton distance and binding energy of constituent quasi-one-dimensional excitons in carbon nanotubes. This allows one to trace biexciton…

Mesoscale and Nanoscale Physics · Physics 2015-05-20 I. V. Bondarev

Using Coulomb correlation parameters appropriate for $\pi$-conjugated polymers (PCPs), and a nearest neighbor hopping integral that is arrived at by fitting the energy spectra of three zigzag semiconducting single-walled carbon nanotubes…

Materials Science · Physics 2007-05-23 Zhendong Wang , Hongbo Zhao , Sumit Mazumdar
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