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Luminescence properties of carbon nanotubes are strongly affected by exciton diffusion, which plays an important role in various nonradiative decay processes. Here we perform photoluminescence microscopy on hundreds of individual…

Mesoscale and Nanoscale Physics · Physics 2015-03-23 A. Ishii , M. Yoshida , Y. K. Kato

Direct measurements of the diffusion length of excitons in air-suspended single-walled carbon nanotubes are reported. Photoluminescence microscopy is used to identify individual nanotubes and to determine their lengths and chiral indices.…

Mesoscale and Nanoscale Physics · Physics 2010-06-17 S. Moritsubo , T. Murai , T. Shimada , Y. Murakami , S. Chiashi , S. Maruyama , Y. K. Kato

Pump-dependent photoluminescence imaging and 2nd order photon correlation studies have been performed on individual single-walled carbon nanotubes (SWCNTs) at room temperature that enable the extraction of both the exciton diffusion…

Mesoscale and Nanoscale Physics · Physics 2015-07-10 Xuedan Ma , Oleskiy Roslyak , Juan G. Duque , Xiaoying Pang , Stephen K. Doorn , Andrei Piryatinski , David H. Dunlap , Han Htoon

Simultaneous photoluminescence and photocurrent measurements on individual single-walled carbon nanotubes reveal spontaneous dissociation of excitons into free electron-hole pairs. Correlation of luminescence intensity and photocurrent…

Mesoscale and Nanoscale Physics · Physics 2014-03-19 Y. Kumamoto , M. Yoshida , A. Ishii , A. Yokoyama , T. Shimada , Y. K. Kato

Single walled carbon nanotubes as emerging quantum-light sources may fill a technological gap in silicon photonics due to their potential use as near infrared, electrically driven, classical or non-classical emitters. Unlike in…

Single-walled carbon nanotubes are a promising material as quantum light sources at room temperature and as nanoscale light sources for integrated photonic circuits on silicon. Here we show that integration of dopant states in carbon…

Mesoscale and Nanoscale Physics · Physics 2018-08-24 A. Ishii , X. He , N. F. Hartmann , H. Machiya , H. Htoon , S. K. Doorn , Y. K. Kato

One- and two-photon luminescence excitation spectroscopy showed a series of distinct excitonic states in single-walled carbon nanotubes. The energy splitting between one- and two-photon-active exciton states of different wavefunction…

Materials Science · Physics 2007-05-23 J. Maultzsch , R. Pomraenke , S. Reich , E. Chang , D. Prezzi , A. Ruini , E. Molinari , M. S. Strano , C. Thomsen , C. Lienau

Spatiotemporal dynamics of excitons in isolated semiconducting single-walled carbon nanotubes are studied using transient absorption microscopy. Differential reflection and transmission of an 810-nm probe pulse after excitation by a 750-nm…

Mesoscale and Nanoscale Physics · Physics 2013-01-08 Brian A. Ruzicka , Rui Wang , Jessica Lohrman , Shenqiang Ren , Hui Zhao

We study the excitonic recombination dynamics in an ensemble of (9,4) semiconducting single-wall carbon nanotubes by high sensitivity time-resolved photo-luminescence experiments. Measurements from cryogenic to room temperature allow us to…

Other Condensed Matter · Physics 2015-06-25 S. Berger , C. Voisin , G. Cassabois , C. Delalande , Philippe Roussignol , X. Marie

Condensed-matter emitters offer enriched cavity quantum electrodynamical effects due to the coupling to external degrees of freedom. In the case of carbon nanotubes a very peculiar coupling between localized excitons and the one-dimensional…

The bright exciton emission of semiconducting carbon nanotubes is appealing for optoelectronic and quantum photonic devices as well as fundamental studies of light-matter interaction in one-dimensional nanostructures. The photophysics of…

Mesoscale and Nanoscale Physics · Physics 2017-05-09 Ibrahim Sarpkaya , Zhengyi Zhang , William Walden-Newman , Xuesi Wang , James Hone , Chee Wei Wong , Stefan Strauf

We have studied emission properties of high-density excitons in single-walled carbon nanotubes through nonlinear photoluminescence excitation spectroscopy. As the excitation intensity was increased, all emission peaks arising from different…

Mesoscale and Nanoscale Physics · Physics 2009-11-13 Y. Murakami , J. Kono

At low temperature the photoluminescence of single-wall carbon nanotubes show a large variety of spectral profiles ranging from ultra narrow lines in suspended nanotubes to broad and asymmetrical line-shapes that puzzle the current…

Single-molecule chemical reactions with individual single-walled carbon nanotubes were observed through near-infrared photoluminescence microscopy. The emission intensity within distinct submicrometer segments of single nanotubes changes in…

Electroluminescence from individual carbon nanotubes within split-gate devices is investigated. By characterizing the air-suspended nanotubes with photoluminescence spectroscopy, chirality is identified and electroluminescence peaks are…

Mesoscale and Nanoscale Physics · Physics 2017-05-10 N. Higashide , M. Yoshida , T. Uda , A. Ishii , Y. K. Kato

Photoluminescent carbon nanotubes are expected to become versatile room-temperature single-photon sources that have applications in quantum information processing. Quantum emission from carbon nanotubes is often induced by localization of…

Mesoscale and Nanoscale Physics · Physics 2021-11-18 Zhen Li , Keigo Otsuka , Daiki Yamashita , Daichi Kozawa , Yuichiro K. Kato

To provide physical insight into the recently observed photoluminescence saturation behaviors in single-walled carbon nanotubes implying the existence of an upper limit of exciton densities, we have performed a time-dependent theoretical…

Mesoscale and Nanoscale Physics · Physics 2015-05-13 Ajit Srivastava , Junichiro Kono

We investigate electric-field induced redshifts of photoluminescence from individual single-walled carbon nanotubes. The shifts scale quadratically with field, while measurements with different excitation powers and energies show that…

Mesoscale and Nanoscale Physics · Physics 2014-10-23 M. Yoshida , Y. Kumamoto , A. Ishii , A. Yokoyama , Y. K. Kato

We present direct experimental observation of exciton-phonon bound states in the photoluminescence excitation spectra of isolated single walled carbon nanotubes in aqueous suspension. The photoluminescence excitation spectra from several…

Materials Science · Physics 2009-11-11 Flavio Plentz , Henrique B. Ribeiro , Ado Jorio , Marcos A. Pimenta , Michael S. Strano

The efficiencies of photonic devices are primarily governed by radiative quantum efficiency, which is a property given by the light emitting material. Quantitative characterization for carbon nanotubes, however, has been difficult despite…

Mesoscale and Nanoscale Physics · Physics 2022-04-19 H. Machiya , D. Yamashita , A. Ishii , Y. K. Kato
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