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We demonstrate, numerically, the possibility of manipulating the spin states of molecular nanomagnets with shaped microwave pulses designed with quantum optimal control theory techniques. The state-to-state or full gate transformations can…

Quantum Physics · Physics 2021-12-01 Alberto Castro , Adrian Garcia Carrizo , David Zueco , Fernando Luis

Experiments in coherent spectroscopy correspond to control of quantum mechanical ensembles guiding them from initial to final target states. The control inputs (pulse sequences) that accomplish these transformations should be designed to…

Quantum Physics · Physics 2009-11-07 Navin Khaneja , Timo Reiss , Burkhard Luy , Steffen J. Glaser

The SpinQuest experiment at Fermilab employs a dynamically polarized solid ammonia target to probe the spin structure of the proton, requiring stable, optimized microwave-driven Dynamic Nuclear Polarization (DNP) under high radiation…

Instrumentation and Detectors · Physics 2026-04-28 Vibodha Bandara , Jordan D. Roberts , Dustin Keller

Microwave control of trapped ions can provide an implementation of high-fidelity two-qubit gates free from errors induced by photon scattering. Furthermore, microwave conductors may be embedded into a scalable trap structure, providing the…

We present three designs for planar superconducting microwave resonators for electron spin resonance (ESR) experiments. We implement finite element simulations to calculate the resonance frequency and quality factors as well as the…

Mesoscale and Nanoscale Physics · Physics 2019-08-21 Stefan Weichselbaumer , Petio Natzkin , Christoph W. Zollitsch , Mathias Weiler , Rudolf Gross , Hans Huebl

For many applications of pulsed radiation, the time-history of the radiation intensity must be optimized to induce a desired time-history of conditions. This optimization is normally performed using multi-physics simulations of the system.…

Computational Physics · Physics 2019-03-14 Damian C. Swift , George B. Zimmerman

Magnetic Resonance Fingerprinting (MRF) is a method to extract quantitative tissue properties such as T1 and T2 relaxation rates from arbitrary pulse sequences using conventional magnetic resonance imaging hardware. MRF pulse sequences have…

The past decade has demonstrated increasing interests in using optimal control based methods within coherent quantum controllable systems. The versatility of such methods has been demonstrated with particular elegance within nuclear…

Quantum Physics · Physics 2015-05-18 Ivan I. Maximov , Niels Chr. Nielsen , Julien Salomon , Gabriel Turinici

Nitrogen-vacancy centers possessing nuclear spins are promising candidates for a novel nuclear spin gyroscope. Preparation of a nuclear spin state is a crucial step to implement a sensor that utilizes a nuclear spin. In a low magnetic…

Spins of single donor atoms are attractive candidates for large scale quantum information processing in silicon, since quantum computation can be realized through the manipulation of electron and/or nuclear spins. We here report on…

Materials Science · Physics 2007-05-23 A. Ferretti , M. Fanciulli , A. Ponti , A. Schweiger

Spin-echo instruments are typically used to measure diffusive processes and the dynamics and motion in samples on ps and ns timescales. A key aspect of the spin-echo technique is to determine the polarisation of a particle beam. We present…

Materials Science · Physics 2018-02-05 Anton Tamtögl , Benjamin Davey , David J. Ward , Andrew P. Jardine , John Ellis , William Allison

We develop energy efficient, continuous microwave schemes to couple electron and nuclear spins, using phase or amplitude modulation to bridge their frequency difference. These controls have promising applications in biological systems,…

Quantum Physics · Physics 2019-01-14 J. Casanova , E. Torrontegui , M. B. Plenio , J. J. García-Ripoll , E. Solano

We optimize the pulse shape and polarization of time-dependent electric fields to maximize the production of electron-positron pairs via strong field quantum electrodynamics processes. The pulse is parametrized in Fourier space by a…

High Energy Physics - Phenomenology · Physics 2017-08-02 François Fillion-Gourdeau , Florian Hebenstreit , Denis Gagnon , Steve MacLean

We investigate the maximum signal to noise ratio per unit time that can be achieved for a spin 1/2 particle subjected to a periodic pulse sequence. Optimal control techniques are applied to design the control field and the position of the…

Quantum Physics · Physics 2015-06-22 M. Lapert , E. Assémat , S. J. Glaser , D. Sugny

We propose a methodology to design optimal pulses for achieving quantum optimal control on molecular systems. Our approach constrains pulse shapes to linear combinations of a fixed number of experimentally relevant pulse functions. Quantum…

Quantum Physics · Physics 2015-10-28 Ruben D. Guerrero , Carlos A. Arango , Andres Reyes

In this work, we demonstrate the use of frequency-tunable superconducting NbTiN coplanar waveguide microresonators for multi-frequency pulsed electron spin resonance (ESR) experiments. By applying a bias current to the center pin, the…

Quantum Physics · Physics 2017-07-19 A. T. Asfaw , A. J. Sigillito , A. M. Tyryshkin , T. Schenkel , S. A. Lyon

We present simulations and analytic calculations of the electromagnetic microwave fields of coplanar waveguide (CPW) resonators in the vicinity of highly conducting metallic samples. The CPW structures are designed with the aim of…

Mesoscale and Nanoscale Physics · Physics 2015-06-23 Conrad Clauss , Martin Dressel , Marc Scheffler

Response functions of resonant circuits create ringing artefacts if their input changes rapidly. When physical limits of electromagnetic spectroscopies are explored, this creates two types of problems. Firstly, simulation: the system must…

Systems and Control · Electrical Eng. & Systems 2023-07-19 Uluk Rasulov , Anupama Acharya , Marina Carravetta , Guinevere Mathies , Ilya Kuprov

Nuclear magnetic resonance signal dynamics as described by the Bloch equations are highly complex and often are without closed form solutions. This is especially the case for quantitative magnetic resonance fingerprinting (MRF) scans in…

Medical Physics · Physics 2020-10-05 Nikolai J. Mickevicius , Andrew S. Nencka , Eric S. Paulson

We establish a testbed system for the development of high-sensitivity Electron Spin Resonance (ESR) techniques for small samples at cryogenic temperatures. Our system consists of a Niobium Nitride thin-film planar superconducting…

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