English
Related papers

Related papers: Pushing Configuration-Interaction to the Limit: To…

200 papers

We report no-core solutions for properties of light nuclei with three different approaches in order to assess the accuracy and convergence rates of each method. Full configuration interaction (FCI), Monte Carlo shell model (MCSM) and no…

Nuclear Theory · Physics 2012-11-09 T. Abe , P. Maris , T. Otsuka , N. Shimizu , Y. Utsuno , J. P. Vary

We propose an efficient deterministic method to calculate the full configuration interaction (FCI) ground state energy. This method leverages the sparseness of the Lanczos basis vectors that span the Krylov subspace associated with the…

Chemical Physics · Physics 2024-01-08 Lijun Wang

The statistical description of Giant Molecular Cloud (GMC) properties relies heavily on the performance of automatic identification algorithms, which are often seriously affected by the survey design. The algorithm we designed, SCIMES…

Astrophysics of Galaxies · Physics 2017-01-11 Dario Colombo , Erik Rosolowsky , Adam Ginsburg , Ana Duarte-Cabral , Annie Hughes

Modeling chemical reactions with quantum chemical methods is challenging when the electronic structure varies significantly throughout the reaction, as well as when electronic excited states are involved. Multireference methods such as…

A recent direction in quantum computing for molecular electronic structure sees the use of quantum devices as configuration sampling machines integrated within high-performance computing (HPC) platforms. This appeals to the strengths of…

Quantum Physics · Physics 2026-05-18 Tim Weaving , Angus Mingare , Alexis Ralli , Peter V. Coveney

The multi-configurational self-consistent field theory is considered the standard starting point for almost all multireference approaches required for strongly-correlated molecular problems. The limitation of the approach is generally given…

Chemical Physics · Physics 2015-10-14 Robert E. Thomas , Qiming Sun , Ali Alavi , George H. Booth

This paper presents a parallel \PG{implementation} for the Optimal Transportation Meshfree (OTM) method on large CPU clusters. Communications are handled with the Message Passing Interface (MPI). The Recursive Coordinate Bisection (RCB)…

Computational Engineering, Finance, and Science · Computer Science 2022-06-20 Sandeep Kumar , Pierre Gosselet , Dengpeng Huang , Christian Weißenfels , Peter Wriggers

A multiscale model based on the coupling of the multiconfigurational self-consistent field (MCSCF) method and the classical atomistic polarizable Fluctuating Charges (FQ) force field is presented. The resulting MCSCF/FQ approach is…

We review time-dependent multiconfiguration self-consistent-field (TD-MCSCF) method and time-dependent optimized coupled-cluster (TD-OCC) method for first-principles simulations of high-field phenomena such as tunneling ionization and…

Chemical Physics · Physics 2022-11-21 Takeshi Sato , Himadri Pathak , Yuki Orimo , Kenichi L. Ishikawa

The Configuration Interaction (CI) method is applied to the calculation of the structures of a number of positron binding systems, including e+Be, e+Mg, e+Ca and e+Sr. These calculations were carried out in orbital spaces containing about…

Atomic Physics · Physics 2007-05-23 M. W. J. Bromley , J. Mitroy

We introduce the pCI software package for high-precision atomic structure calculations. The standard method of calculation is based on the configuration interaction (CI) method to describe valence correlations, but can be extended to attain…

Multiplication is an indispensable operation in most of digital signal processing systems. Recently, many systems need to execute different types of algorithms on a multiplier. Therefore, it needs complicated computation and large area…

Hardware Architecture · Computer Science 2019-07-23 Seungbum Baek

We introduce state-averaging into the method of Monte Carlo configuration interaction (SA-MCCI) to allow the stable and efficient calculation of excited states. We show that excited potential curves for H$_{3}$, including a crossing with…

Chemical Physics · Physics 2014-03-03 J. P. Coe , M. J. Paterson

The exponential scaling of complete active space (CAS) and full configuration interaction (CI) calculations limits the ability of quantum chemists to simulate the electronic structures of strongly correlated systems. Herein, we present…

Chemical Physics · Physics 2024-08-01 Kenneth O. Berard , Hongji Gao , Alexander Teplukhin , Xiangmin Jiao , Benjamin G. Levine

In fluid flow simulation, the multi-continuum model is a useful strategy. When the heterogeneity and contrast of coefficients are high, the system becomes multiscale, and some kinds of reduced-order methods are demanded. Combining these…

Numerical Analysis · Mathematics 2023-02-08 Tina Mai , Siu Wun Cheung , Jun Sur Richard Park

We investigate the optimal power allocation and optimal precoding for a multi-cell-processing (MCP) framework with limited cooperation. In particular, we consider two base stations(BSs) which maximize the achievable rate for two users…

Information Theory · Computer Science 2016-01-12 Samah A. M. Ghanem

Maximal Clique Enumeration (MCE) is a fundamental graph mining problem, and is useful as a primitive in identifying dense structures in a graph. Due to the high computational cost of MCE, parallel methods are imperative for dealing with…

Distributed, Parallel, and Cluster Computing · Computer Science 2020-01-31 Apurba Das , Seyed-Vahid Sanei-Mehri , Srikanta Tirthapura

Power distribution systems experience a large-scale integration of Converter-Interfaced Distributed Energy Resources (CIDERs). As acknowledged by recent literature, the interaction of individual CIDER components and different CIDERs through…

Systems and Control · Electrical Eng. & Systems 2022-10-24 Johanna Kristin Maria Becker , Andreas Martin Kettner , Yihui Zuo , Federico Cecati , Sante Pugliese , Marco Liserre , Mario Paolone

A coarse grid correction (CGC) approach is proposed to enhance the efficiency of the matrix exponential and $\varphi$ matrix function evaluations. The approach is intended for iterative methods computing the matrix-vector products with…

Numerical Analysis · Mathematics 2024-04-23 Mike A. Botchev

Self-consistent field theory (SCFT) is one of the most widely-used framework in studying the equilibrium phase behaviors of inhomogenous polymers. For liquid crystalline polymeric systems, the main numerical challenges of solving SCFT…

Numerical Analysis · Mathematics 2024-09-16 Zhijuan He , Kai Jiang , Liwei Tan , Xin Wang