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Multi-dimensional coherent spectroscopy (MDCS)1,2 is a powerful method for optical spectroscopy that has become an important tool for studying ultrafast dynamics in a wide range of systems. It is an optical analog of multidimensional…
Dual-frequency comb spectroscopy has emerged as a disruptive technique for measuring wide-spanning spectra with high resolution, yielding a particularly powerful technique for sensitive multi-component gas analysis. We present a…
Frequency combs, broadband light sources whose spectra consist of coherent, discrete modes, have become essential in many fields. Miniaturizing frequency combs would be a significant advance in these fields, enabling the deployment of…
We propose and characterize experimentally a new source of optical frequency combs for performing multi-heterodyne spectrometry. This comb modality is based on a frequency shifting loop seeded with a CW monochromatic laser. The comb lines…
Photonic integrated circuits utilize planar waveguides to process light on a chip, encompassing functions like generation, routing, modulation, and detection. Similar to the advancements in the electronics industry, photonics research is…
Chip-scale optical frequency combs can provide broadband spectroscopy for diagnosing complex organic molecules. They are also promising as miniaturized laser spectrometers in applications ranging from atmospheric chemistry to geological…
We report the upgrade and operation of a frequency-comb-assisted high-resolution mid-infrared molecular spectrometer allowing us to combine high spectral purity, SI-traceability, wide tunability and high sensitivity. An optical frequency…
We introduce a novel ultra-broadband ultraviolet and visible frequency comb light source covering more than 240 THz by resonant dispersive wave emission in a gas-filled hollow-core fiber waveguide. The light source allows tuning from ~340…
Multi-spectral frequency combs provide frontier architectures for laser standoff spectroscopy, optical clockwork, and high-capacity optical communications. Frequency microcombs, aided by their high-quality resonances and inherent…
Dual-comb spectroscopy is a powerful technique for real-time, broadband optical sampling of molecular spectra which requires no moving components. Recent developments with microresonator-based platforms have enabled frequency combs at the…
Optical spectroscopy and imaging of microscopic samples have opened up a wide range of applications throughout the physical, chemical, and biological sciences. High chemical specificity may be achieved by directly interrogating the…
The optical frequency comb has made a significant impact in precision spectroscopy and on our ability to probe atomic, molecular and, recently, nuclear transitions to further our understanding of their fundamental properties and how their…
Two frequency combs can be used to measure the full complex response of a sample in a configuration which can be alternatively viewed as the equivalent of a dispersive Fourier transform spectrometer, infrared time domain spectrometer, or a…
Frequency metrology lies at the heart of precision measurement. Optical frequency combs provide a coherent link uniting the microwave and optical domains in the electromagnetic spectrum, with profound implications in timekeeping, sensing…
Optical-frequency combs enable measurement precision at the 20th digit, and accuracy entirely commensurate with their reference oscillator. A new direction in experiments is the creation of ultracompact frequency combs by way of nonlinear…
Nonlinear nanophotonic waveguides have opened a route to compact frequency combs for precision metrology, spectroscopy and astronomy, yet broadband comb access to the visible remains challenging on CMOS-compatible platforms. Silicon nitride…
The development of broadband microresonator frequency combs at visible wavelengths is pivotal for the advancement of compact and fieldable optical atomic clocks and spectroscopy systems. Yet, their realization necessitates resonators with…
The femtosecond laser frequency comb has enabled the 21st century revolution in optical synthesis and metrology. A particularly compelling technique that relies on the broadband coherence of two laser frequency combs is dual-comb…
Mid-infrared femtosecond optical frequency combs were produced by difference frequency generation of the spectral components of a near-infrared comb in a 3-mm-long MgO:PPLN crystal. We observe strong pump depletion and 9.3 dB parametric…
Laser frequency combs are coherent light sources that simultaneously provide pristine frequency spacings for precision metrology and the fundamental basis for ultrafast and attosecond sciences. Recently, nonlinear parametric conversion in…