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Hund's coupling is shown to generally favor, in a doped half-filled Mott insulator, an increase in the compressibility culminating in a Fermi-liquid instability towards phase separation. The largest effect is found about the frontier…

Strongly Correlated Electrons · Physics 2017-04-20 Luca de' Medici

Atomic physics has a profound impact on the physical properties of correlated electron materials. This article describes a prime example of this phenomenon. We provide a non-technical introduction to the physics of Hund metals, a broad…

Strongly Correlated Electrons · Physics 2024-11-26 Antoine Georges , Gabriel Kotliar

We analyze multi-orbital Hubbard models describing Hund's metals, focusing on the ubiquitous occurrence of a charge instability, signalled by a divergent/negative electronic compressibility, in a range of doping from the half-filled Mott…

Strongly Correlated Electrons · Physics 2020-11-25 Maria Chatzieleftheriou , Maja Berović , Pablo Villar Arribi , Massimo Capone , Luca de' Medici

Motivated by the recent discovery of superconductivity in infinite-layer nickelates RE$_{1-\delta}$Sr$_\delta$NiO$_2$ (RE$=$Nd, Pr), we study the role of Hund's coupling $J$ in a quarter-filled two-orbital Hubbard model which has been on…

Strongly Correlated Electrons · Physics 2021-05-18 Siheon Ryee , Myung Joon Han , Sangkook Choi

Strong electronic correlations are often associated with the proximity of a Mott insulating state. In recent years however, it has become increasingly clear that the Hund's rule coupling (intra-atomic exchange) is responsible for strong…

Strongly Correlated Electrons · Physics 2013-03-20 Antoine Georges , Luca de' Medici , Jernej Mravlje

Hund's coupling plays a decisive role in shaping electron correlations of multi-orbital systems, giving rise to a class of materials--Hund's metals--that combine local-moment physics with metallic transport. Here we derive an effective…

Strongly Correlated Electrons · Physics 2025-11-27 Johan Carlström

Strong correlation effects caused by Hund's coupling have been actively studied during the past decade. Hund's metal, strongly correlated while far from the Mott insulating limit, was studied as a representative example. However, recently,…

Strongly Correlated Electrons · Physics 2024-04-01 Ina Park , Bo Gyu Jang , Dong Wook Kim , Ji Hoon Shim , Gabriel Kotliar

To clarify the nature of correlations in Hund metals and its relationship with Mott physics we analyze the electronic correlations in multiorbital systems as a function of intraorbital interaction U, Hund's coupling JH and electronic…

Strongly Correlated Electrons · Physics 2015-09-02 L. Fanfarillo , E. Bascones

Hund metals are multi-orbital systems with moderate Coulomb interaction, $U$, and sizeable Hund's rule coupling, $J<U$, that aligns the spins in different orbitals. They show strong correlation effects, like very low Fermi-liquid coherence…

Strongly Correlated Electrons · Physics 2018-12-27 Katharina M. Stadler , Gabriel Kotliar , Andreas Weichselbaum , Jan von Delft

We show that electron correlations lead to a bad metallic state in chalcogenides FeSe and FeTe despite the intermediate value of the Hubbard repulsion $U$ and Hund's rule coupling $J$. The evolution of the quasi particle weight $Z$ as a…

Materials Science · Physics 2013-05-24 N. Lanatà , H. U. R. Strand , G. Giovannetti , B. Hellsing , L. de' Medici , M. Capone

We study the interplay between Mott physics, driven by Coulomb repulsion U, and Hund physics, driven by Hund's coupling J, for a minimal model for Hund metals, the orbital-symmetric three-band Hubbard-Hund model (3HHM) for a lattice filling…

Strongly Correlated Electrons · Physics 2021-09-09 K. M. Stadler , G. Kotliar , S. -S. B. Lee , A. Weichselbaum , J. von Delft

We show how in multi-band materials, the Hund's coupling plays a crucial role in tuning the degree of electronic correlation. While in half-filled systems it enhances the correlations, in all other cases it pushes the boundary for the Mott…

Strongly Correlated Electrons · Physics 2011-06-02 Luca de' Medici

The recently proposed theoretical concept of a Hund's metal is regarded as a key to explain the exotic magnetic and electronic behavior occuring in the strongly correlated electron systems of multiorbital metallic materials. However, a…

We show that in multi-band metals the correlations are strongly affected by the Hund's rule coupling, which depending on the filling promotes metallic, insulating or bad-metallic behavior. The quasiparticle coherence and the proximity to a…

Strongly Correlated Electrons · Physics 2015-03-19 Luca de' Medici , Jernej Mravlje , Antoine Georges

We propose a way to identify strongly Hund-correlated materials by unveiling a key signature of Hund correlations at the two-particle level. The defining feature is the {\it sign} of the response of the {\it frozen spin ratio} (the…

Strongly Correlated Electrons · Physics 2023-08-28 Siheon Ryee , Sangkook Choi , Myung Joon Han

We analyze a simple model containing the physical ingredients of a Hund's metal, the local spin fluctuations with power-law correlators, $(\Omega_0/|\Omega|)^\gamma$, with $\gamma$ greater than one, interacting with electronic…

Superconductivity · Physics 2018-11-07 Tsung-Han Lee , Andrey Chubukov , Hu Miao , Gabriel Kotliar

We study LiFeP, LiFeAs and NaFeAs in their paramagnetic metallic phase including dynamical electronic correlations within a density functional theory + slave-spin mean-field framework. The three compounds are found to lie next to the…

Superconductivity · Physics 2021-09-29 Pablo Villar Arribi , Luca de' Medici

We analyze the electronic properties of interacting crystal field split three band systems. Using a rotationally invariant slave boson approach we analyze the behavior of the electronic mass renormalization as a function of the intralevel…

Strongly Correlated Electrons · Physics 2019-05-22 Jorge I. Facio , Pablo S. Cornaglia

FeSe has been extensively explored as a quantum material, primarily due to the observed highest superconducting transition temperature among Fe-based unconventional superconductors. Nonetheless, the electronic structure and the electron…

Strongly Correlated Electrons · Physics 2023-10-31 Byungkyun Kang , Maengsuk Kim , Chul Hong Park , Anderson Janotti

We combine transport, angle-resolved photoemission spectroscopy and scanning tunneling spectroscopy to investigate several low energy manifestations of the Hund coupling in a canonical FeSC family Li(Fe,Co)As. We determine the doping…

Superconductivity · Physics 2021-06-17 H. Miao , Y. L. Wang , J. -X. Yin , J. Zhang , S. Zhang , M. Z. Hasan , R. Yang , X. C. Wang , C. Q. Jin , T. Qian , H. Ding , H. -L. Lee , G. Kotliar
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