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Using thermodynamic measurements, neutron diffraction, nuclear magnetic resonance, and muon spin relaxation, we establish putative quantum spin-liquid behavior in Ba$_3$InIr$_2$O$_9$, where unpaired electrons are localized on mixed-valence…

Muon spin rotation and relaxation experiments in the pyrochlore iridate Eu2Ir2O7 yield a well-defined muon spin precession frequency below the metal-insulator/antiferromagnetic transition temperature TM = 120 K, indicative of long-range…

Strongly Correlated Electrons · Physics 2015-03-19 Songrui Zhao. J. M. Mackie , D. E. MacLaughlin , O. O. Bernal , J. J. Ishikawa , Y. Ohta , S. Nakatsuji

We report results of magnetic susceptibility, specific heat, and muon spin relaxation ($\mu$SR) measurements on the polycrystalline Ba$_6$Nd$_2$Ti$_4$O$_{17}$, a disorder-free triangular-lattice antiferromagnet. The absence of long-range…

Strongly Correlated Electrons · Physics 2024-11-21 C. Y. Jiang , B. L. Chen , K. W. Chen , J. C. Jiao , Y. Wang , Q. Wu , N. Y. Zhang , M. Y. Zou , P. -C. Ho , O. O. Bernal , L. Shu

Frustrated magnets offer a plethora of exotic magnetic ground states, including quantum spin liquids (QSLs), in which enhanced quantum fluctuations prevent a long-range magnetic ordering of the strongly correlated spins down to lowest…

Collective behaviour of electrons, frustration induced quantum fluctuations and entanglement in quantum materials underlie some of the emergent quantum phenomena with exotic quasi-particle excitations that are highly relevant for…

Here, we report both ac and dc magnetization, thermodynamic and electric properties of hexagonal Ba$_3$NiIr$_2$O$_9$. The Ni$^{2+}$ (spin-1) forms layered triangular-lattice and interacts antiferromagnetically while Ir$^{5+}$ is believed to…

Strongly Correlated Electrons · Physics 2021-07-14 Shobha Gondh , Manju Mishra Patidar , Kranti Kumar , M. P. Saravanan , V. Ganesan , A. K. Pramanik

The synergistic interplay between spin correlations, spin-orbit coupling, and competing exchange interactions provides a promising route to realize exotic quantum states with nontrivial excitations in rare-earth based frustrated magnets.…

Strongly Correlated Electrons · Physics 2026-05-25 J. Khatua , D. Tay , T. Shiroka , M. Pregelj , K. Kargeti , S. K. Panda , G. B. G. Stenning , P. Manuel , M. D. Le , D. T. Adroja , P. Khuntia

The hexagonal polymorph of Ba$_3$Tb(BO$_3$)$_3$ contains Tb$^{3+}$ ions on a quasi-2D triangular lattice, resulting in geometric magnetic frustration. Powder samples of Ba$_3$Tb(BO$_3$)$_3$ have been investigated using specific heat, powder…

Strongly Correlated Electrons · Physics 2025-02-21 Nicola Kelly , Manh Duc Le , Denis Sheptyakov , Camilla Tacconis , Cheng Liu , Gavin Stenning , Peter Baker , Siân Dutton

Muon-spin relaxation results on the pyrochlore iridate Nd$_2$Ir$_2$O$_7$ are reported. Spontaneous coherent muon-spin precession below the metal-insulator transition (MIT) temperature of about 33 K is observed, indicating the appearance of…

Strongly Correlated Electrons · Physics 2013-09-03 Hanjie Guo , Kazuyuki Matsuhira , Ikuto Kawasaki , Makoto Wakeshima , Yukio Hinatsu , Isao Watanabe , Zhu-an Xu

We report the synthesis of single crystals of a novel layered iridate Ba$_{21}$Ir$_9$O$_{43}$, and present the crystallographic, transport and magnetic properties of this material. The compound has a hexagonal structure with two iridium…

Ba3IrTi2O9 crystallizes in a hexagonal structure consisting of a layered triangular arrangement of Ir4+ (Jeff=1/2). Magnetic susceptibility and heat capacity data show no magnetic ordering down to 0.35K inspite of a strong magnetic coupling…

Strongly Correlated Electrons · Physics 2012-10-29 Tusharkanti Dey , A. V. Mahajan , P. Khuntia , M. Baenitz , B. Koteswararao , F. C. Chou

Muon spin relaxation experiments have been performed in the pyrochlore iridate Pr_2Ir_2O_7 for temperatures in the range 0.025-250 K. Kubo-Toyabe relaxation functions are observed up to > 200 K, indicating static magnetism over this…

Strongly Correlated Electrons · Physics 2009-11-13 D. E. MacLaughlin , Y. Ohta , Y. Machida , S. Nakatsuji , G. M. Luke , K. Ishida , R. H. Heffner , Lei Shu , O. O. Bernal

In order to characterize thermal excitations in a frustrated spin liquid, we have examined the magnetothermodynamics of a model geometrically frustrated magnet. Our data demonstrate a crossover in the nature of the spin excitations between…

Condensed Matter · Physics 2009-11-07 Y. K. Tsui , J. Snyder , P. Schiffer

We present a muon spin relaxation study on the Ising pyrochlore Nd$_2$Zr$_2$O$_7$ which develops an "all-in-all-out" magnetic order below 0.4~K. At 20~mK far below the ordering transition temperature, the zero-field muon spin relaxation…

Materials Science · Physics 2016-09-07 J. Xu , C. Balz , C. Baines , H. Luetkens , B. Lake

The three-dimensional frustrated spin lattice in MgCrGaO4, where Cr3+ ions occupy a pyrochlore-like network, exemplifies a quantum magnet with competing interactions, macroscopic degeneracy, and exotic low-energy excitations. Using…

Strongly Correlated Electrons · Physics 2026-03-17 U. Jena , S. Kundu , Suheon Lee , Q. Faure , F. Damay , S. Rols , Adam Berlie , S. Petit , Kwang-Yong Choi , P. Khuntia

We present an experimental investigation of the magnetic ground state in Ba$_4$NbIr$_3$O$_{12}$, a fractional valent trimer iridate. X-ray absorption and photoemission spectroscopy show that the Ir valence lies between 3+ and 4+ while Nb is…

The title compound Ba3RuTi2O9 crystallizes with a hexagonal unit cell. It contains layers of edge shared triangular network of Ru4+ (S=1) ions. Magnetic susceptibility chi(T) and heat capacity data show no long range magnetic ordering down…

Strongly Correlated Electrons · Physics 2013-06-14 Tusharkanti Dey , A. V. Mahajan

The triangular-lattice system $\alpha$-RuI$_3$ is isostructural to the widely-studied $\alpha$-RuCl$_3$ compound which was identified as a potential Kitaev system but exhibits, instead of spin liquid behaviour, a magnetically ordered…

Strongly Correlated Electrons · Physics 2024-06-07 Hank C. H. Wu , Benjamin M. Huddart , Francis L. Pratt , Danrui Ni , Robert J. Cava , Stephen J. Blundell

A detailed zero and transverse field (ZF&TF) muon spin rotation (muSR) investigation of magnetism and the magneto-electric coupling in Cu2OSeO3 is reported. An internal magnetic field B_int(T=0) = 85.37(25) mT was found, in agreement with a…

Strongly Correlated Electrons · Physics 2015-05-28 A. Maisuradze , Z. Guguchia , B. Graneli , H. M. Ronnow , H. Berger , H. Keller

In the garnet structure compound Yb3Ga5O12, the Yb3+ ions (ground state effective spin S' = 1/2) are situated on two interpenetrating corner sharing triangular sublattices such that frustrated magnetic interactions are possible. Previous…

Condensed Matter · Physics 2009-11-10 J. A. Hodges , P. Bonville , M. Rams , K. Krolas
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