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High-resolution spectroscopy on the $A^2\Pi$ - $X^2\Sigma^+$ electronic system of $^{138}$Ba$^{19}$F is performed using a cold molecular beam produced by a buffer gas source. The hyperfine structure in both $X^2\Sigma^+$ ground and $A^2\Pi$…

The $^1\mathrm{S}_0$-$^3\mathrm{P}_0$ clock transition frequency $\nu_\text{Sr}$ in neutral $^{87}$Sr has been measured relative to the Cs standard by three independent laboratories in Boulder, Paris, and Tokyo over the last three years.…

We have studied possible candidates for laser cooling transitions in $^{169}$Tm in the spectral region 410 -- 420 nm. By means of saturation absorption spectroscopy we have measured the hyperfine structure and rates of two nearly closed…

We demonstrate theoretically the existence of a linear dc Stark shift of the individual substates of an alkali atom in its ground state, dressed by a circularly polarized laser field. It arises from the electroweak nuclear anapole moment…

Atomic Physics · Physics 2008-11-26 Marie-Anne Bouchiat

Using 201Hg+ contained within a linear quadrupole rf ion trap that is part of an atomic clock, we report the first high-resolution spectroscopy on the hyperfine structure of 201Hg+. We measure the absolute ground state hyperfine interval to…

Atomic Physics · Physics 2015-05-13 E. A. Burt , S. Taghavi-Larigani , R. L. Tjoelker

Hyperfine structure (HFS) of atomic energy levels arises due to interactions of atomic electrons with a hierarchy of nuclear multipole moments, including magnetic dipole, electric quadrupole and higher rank moments. Recently, a…

Optical clocks have extremely attractive applications in many fields, including time-frequency metrology, validation of fundamental physical principles, and relativistic geodesy. The 467 nm octupole transition in 171Yb+ ion exhibits…

Atomic Physics · Physics 2025-10-14 Xuanjian Wang , Jian Cao , Hualin Shu , Yi Yuan , Zehao Li , Pengcheng Fang , Qunfeng Chen , Xueren Huang

Hyperfine quenching rates of the lowest-energy metastable $^3P_0$ and $^3P_2$ states of Mg, Ca, Sr, and Yb atoms are computed. The calculations are carried out using ab initio relativistic many-body methods. The computed lifetimes may be…

Atomic Physics · Physics 2009-11-10 Sergey Porsev , Andrei Derevianko

We demonstrate a technique to measure hyperfine structure using a frequency-stabilized diode laser and an acousto-optic modulator locked to the frequency difference between two hyperfine peaks. We use this technique to measure hyperfine…

Atomic Physics · Physics 2007-05-23 Umakant D. Rapol , Anusha Krishna , Vasant Natarajan

Searching for an accurate optical clock which can serve as a better time standard than the present day atomic clock is highly demanding from several areas of science and technology. Several attempts have been made to built more accurate…

Atomic Physics · Physics 2007-09-17 Chiranjib Sur , Rajat K Chaudhuri

Accurate spectroscopic investigations of the heaviest elements are inherently challenging, due to their short lifetimes and low production yields. Success of such measurements requires both dedicated experimental techniques and strong…

We have carried absolute frequency measurements of the $(6s^{2})\,^{1}S_{0}$ $-$ $(6s6p)\,^{3}P_{1}$ transition in $^{171}$Yb (the intercombination line), where the spin-1/2 isotope yields two hyperfine lines. The measurements rely on…

Atomic Physics · Physics 2023-05-23 Daniel M. Jones , Frank van Kann , John J. McFerran

We demonstrate a technique for frequency measurements of UV transitions with sub-MHz precision. The frequency is measured using a ring-cavity resonator whose length is calibrated against a reference laser locked to the $D_2$ line of…

Atomic Physics · Physics 2007-05-23 Ayan Banerjee , Umakant D. Rapol , Dipankar Das , Anusha Krishna , Vasant Natarajan

We have measured and analyzed the hyperfine structure of two lines, one at 583nm and one at 401nm, of the only stable fermionic isotope of atomic erbium as well as determined its isotope shift relative to the four most-abundant bosonic…

We demonstrated transferring the stability of one highly stable clock laser operating at 729 nm to another less stable laser operating at 698 nm. The two different wavelengths were bridged using an optical frequency comb. The improved…

Atomic Physics · Physics 2012-01-17 A. Yamaguchi , N. Shiga , S. Nagano , Y. Li , H. Ishijima , H. Hachisu , M. Kumagai , T. Ido

Hyperfine spectra of $^\text{27-32}$Al ($Z=13$) have been measured at the ISOLDE-CERN facility via collinear laser spectroscopy using the $3s^23p\ ^2\text{P}^\text{o} _{3/2}\rightarrow 3s^24s\ ^2\text{S}_{1/2}$ atomic transition. For the…

We have measured the frequency splitting between the $(2S, F=1/2)$ and $(2S, F=3/2)$ hyperfine sublevels in atomic deuterium by an optical differential method based on two-photon Doppler-free spectroscopy on a cold atomic beam. The result…

Atomic Physics · Physics 2009-11-10 N. Kolachevsky , P. Fendel , S. G. Karshenboim , T. W. Hänsch

We implement imaging spectroscopy of the optical clock transition of lattice-trapped degenerate fermionic Sr in the Mott-insulating regime, combining micron spatial resolution with submillihertz spectral precision. We use these tools to…

Atomic Physics · Physics 2018-03-14 G. Edward Marti , Ross B. Hutson , Akihisa Goban , Sara L. Campbell , Nicola Poli , Jun Ye

We have observed the rotational ground-state (J = 1-0) transitions of DCO+, HN13C and DNC with the IRAM 30m telescope toward the dark cloud LDN 1512 which has exceptionally narrow lines permitting hyperfine splitting to be resolved in part.…

Astrophysics of Galaxies · Physics 2015-05-14 Floris van der Tak , Holger Müller , Michael Harding , Jürgen Gauss

We report on hyperfine-resolved laser spectroscopy of the A$^2\Pi \leftarrow $X$^2\Sigma^+$ transition of MgF, relevant for laser cooling. We recorded 25 rotational transitions with an absolute accuracy of better than 20 MHz, assigned 56…

Atomic Physics · Physics 2022-04-13 M. Doppelbauer , S. C. Wright , S. Hofsäss , B. G. Sartakov , G. Meijer , S. Truppe
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