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We investigate the influence of static disorder and thermal excitations on excitonic energy transport in the light-harvesting apparatus of photosynthetic systems by solving the Schr\"{o}dinger equation and taking into account the coherent…

Biological Physics · Physics 2012-09-07 Shi-Jie Xiong , Ye Xiong , Yang Zhao

Two distinct approaches, the Frenkel-Dirac time-dependent variation and the Haken-Strobl model, are adopted to study energy transfer dynamics in single-ring and double-ring light-harvesting systems in purple bacteria. It is found that…

Chemical Physics · Physics 2015-06-05 Jun Ye , Kewei Sun , Yang Zhao , Yunjin Yu , Chee Kong Lee , Jianshu Cao

Exciton transport in molecular aggregates is a fundamental process governing the performance of organic optoelectronics and light-harvesting systems. While most theoretical studies have emphasized long-time transport behavior, recent…

Chemical Physics · Physics 2026-03-25 Siwei Wang , Guangming Liu , Hsing-Ta Chen

This paper considers the propagation of excitons in linear chains of QDs with a side defect, located on a dielectric substrate. This configuration is suitable for spatially selective excitation of the system by pulsed optical radiation…

Mesoscale and Nanoscale Physics · Physics 2026-02-17 Aleksey Vlasov , Pavel Golovinski

Polarons, which arise from the self-trapping interaction between electrons and lattice distortions in a solid, have been known and extensively investigated for nearly a century. Nevertheless, the study of polarons continues to be an active…

We present a comprehensive study of exciton wave packet evolution in disordered lossless polaritonic wires. Our simulations reveal signatures of ballistic, diffusive, and subdiffusive exciton dynamics under strong light-matter coupling and…

Quantum Physics · Physics 2023-09-27 Gustavo J. R. Aroeira , Kyle Kairys , Raphael F. Ribeiro

The role of noise in the transport properties of quantum excitations is a topic of great importance in many fields, from organic semiconductors for technological applications to light-harvesting complexes in photosynthesis. In this paper we…

Quantum Physics · Physics 2016-11-22 Stefano Iubini , Octavi Boada , Yasser Omar , Francesco Piazza

We enlarge our results from the study of the hopping mechanism of the oscillation excitation transport in 1D model of one biology-like macromolecular chain to the case of a system composed from two 1D parallel macromolecular chains with…

Mesoscale and Nanoscale Physics · Physics 2016-01-12 D. Čevizović , S. Petković , S. Galović , A. Chizhov , A. Reshetnyak

In this work, we systematically investigate the spectral and transport properties of exciton-polaritons under the explicit influence of intermolecular vibrational coupling, which introduces dynamic disorder. In the context of a…

Chemical Physics · Physics 2025-12-03 Guangming Liu , Hsing-Ta Chen

Molecular aggregates can under certain conditions transport electronic excitation energy over large distances due to dipole-dipole interactions. Here, we explore to what extent thermal motion of entire monomers can guide or enhance this…

Chemical Physics · Physics 2020-12-22 R. Pant , S. Wüster

Excitation energy transport can be significantly enhanced by strong light-matter interactions. In the present work, we explore intriguing features of coherent transient exciton wave packet dynamics on a lossless disordered polaritonic wire.…

Quantum Physics · Physics 2024-02-26 Gustavo J. R. Aroeira , Kyle T. Kairys , Raphael F. Ribeiro

We numerically study excitation transfer in an artificial LH1-RC complex -- an $N$-site donor ring coupled to a central acceptor -- driven by a narrowband optical mode and evolved under a Lindblad master equation with loss and dephasing. In…

Optics · Physics 2025-09-27 Stephon Alexander , Roger Andrews , Oliver Fox , Sarben Sarkar

Disordered quantum networks, as those describing light-harvesting complexes, are often characterized by the presence of antenna structures where the light is captured and inner structures (reaction centers) where the excitation is…

Mesoscale and Nanoscale Physics · Physics 2015-08-10 Giulio G. Giusteri , G. Luca Celardo , Fausto Borgonovi

Collective optical excitations in dipole-coupled nanorings of sub-wavelength spaced quantum emitters exhibit extreme sub-radiance and field confinement facilitating an efficient and low-loss ring-to-ring energy transfer. We show that energy…

Following the ideas of Davydov's soliton theory, we study the bio-energy transport in protein molecules. By using a quantum Brownian motion model for a phonon dressed vibrational exciton, we calculate the time-dependence on the mean square…

Biological Physics · Physics 2019-04-01 Theja N. De Silva , Peighton Bolt

Molecular materials have been studied as a potential platform for highly efficient transport such as exciton transport and quantum information spreading. However, one detrimental factor to transport efficiency is the inherent disorder of…

Quantum Physics · Physics 2024-09-12 Weijun Wu , Ava N. Hejazi , Gregory D. Scholes

Recent ultrafast optical experiments show that excitons in large biological light-harvesting complexes are coupled to molecular vibration modes. These high-frequency vibrations will not only affect the optical response, but also drive the…

Quantum Physics · Physics 2015-02-12 Arend G. Dijkstra , Chen Wang , Jianshu Cao , Graham R. Fleming

In recent years it has become clear that the transport of excitons and charge carriers in molecular systems can be enhanced by coherent coupling with photons, giving rise to the formation of hybrid excitations known as polaritons. Such…

Materials Science · Physics 2023-01-19 M. Balasubrahmaniyam , Arie Simkovich , Adina Golombek , Guy Ankonina , Tal Schwartz

The non-equilibrium dynamics of matter excited by light may produce electronic phases that do not exist in equilibrium, such as laser-induced high-transition-temperature superconductivity. Here we simulate the dynamics of a metal driven at…

Strongly Correlated Electrons · Physics 2022-12-05 John Sous , Benedikt Kloss , Dante M. Kennes , David R. Reichman , Andrew J. Millis

The transport of excitations governs fundamental properties of matter. Particularly rich physics emerges in the interplay between disorder and environmental noise, even in small systems such as photosynthetic biomolecules.…

Quantum Physics · Physics 2018-02-14 Nils Trautmann , Philipp Hauke
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