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The symmetry-projected Hartree--Fock ansatz for the electronic structure problem can efficiently account for static correlation in molecules, yet it is often unable to describe dynamic correlation in a balanced manner. Here, we consider a…

Strongly Correlated Electrons · Physics 2015-06-17 Carlos A. Jiménez-Hoyos , R. Rodríguez-Guzmán , Gustavo E. Scuseria

Finding Minimum Energy Configurations (MECs) is essential in fields such as physics, chemistry, and materials science, as they represent the most stable states of the systems. In particular, identifying such MECs in multi-component alloys…

Materials Science · Physics 2025-01-27 Md Rajib Khan Musa , Yichen Qian , Jie Peng , David Cereceda

Using the atomistic tight-binding method in combination with symmetry analysis and extended effective mass theory we derive a phenomenological model for the fine structure of the ground electron and hole states in $[111]$-grown PbX, X=S,Se…

Mesoscale and Nanoscale Physics · Physics 2024-12-02 I. D. Avdeev , M. O. Nestoklon

A Cholesky decomposition (CD)-based implementation of relativistic two-component coupled-cluster (CC) and equation-of-motion CC (EOM-CC) methods using an exact two-component Hamiltonian augmented with atomic-mean-field spin-orbit integrals…

Chemical Physics · Physics 2023-09-19 Chaoqun Zhang , Filippo Lipparini , Stella Stopkowicz , Jürgen Gauss , Lan Cheng

The generator coordinate method (GCM) casts the wavefunction as an integral over a weighted set of non-orthogonal single determinantal states. In principle this representation can be used like the configuration interaction (CI) or shell…

Nuclear Theory · Physics 2015-06-23 Jason L. Stuber

The scalar and vector Laplacians are basic operators in physics and engineering. In applications, they show up frequently perturbed by lower-order terms. The effect of such perturbations on mixed finite element methods in the scalar case is…

Numerical Analysis · Mathematics 2018-11-13 Douglas N. Arnold , Lizao Li

The relativistic coupled-cluster (RCC) theory has been applied recently to a number of heavy molecules to determine their properties very accurately. Since it demands large computational resources, the method is often approximated to…

Atomic Physics · Physics 2020-05-12 V. S. Prasannaa , B. K. Sahoo , M. Abe , B. P. Das

We calculate the decay constants of light and heavy-light pseudoscalar and vector mesons with improved soft-wall holographic wavefuntions, which take into account the effects of both quark masses and dynamical spins. We find that the…

High Energy Physics - Phenomenology · Physics 2018-05-15 Qin Chang , Xiao-Nan Li , Xin-Qiang Li , Fang Su

We calculate the hyperfine structure constant for the Eu isotopes with shell model wave functions. The calculated results are compared with those predicted by the Moskowitz-Lombardi (M-L) empirical formula. It turns out that the two…

Nuclear Theory · Physics 2009-10-30 Tomoko Asaga , Takehisa Fujita , Kaori Ito

We study the electron correlation effects in the calculations of isotope shifts in Na and Mg+ using the relativistic coupled-cluster method. The trends of the correlation effects are explicitly discussed and comparison of the present…

Atomic Physics · Physics 2010-07-29 B. K. Sahoo

In this paper we present an approach aimed at calculating the optical dielectric constant of crystalline insulators both at the Hartree-Fock, and correlated levels. Our scheme employs a real-space methodology, employing Wannier functions as…

Materials Science · Physics 2010-01-14 Priya Sony , Alok Shukla

Density-functional based tight-binding is a powerful method to describe large molecules and materials. Metal-Organic Frameworks (MOFs), materials with interesting catalytic properties and with very large surface areas have been developed…

Point-ion models have been extensively used to determine "hole numbers" at copper and oxygen sites in high-temperature superconducting cuprate compounds from measured nuclear quadrupole frequencies. The present study assesses the…

Superconductivity · Physics 2016-08-31 E. P. Stoll , P. F. Meier , T. A. Claxton

The coupled cluster calculations with accounting for relativistic effects to study spectroscopic and chemical properties of element 120 (E120) are performed. Similar calculations for Ba are also done and they are in a good agreement with…

Chemical Physics · Physics 2013-08-01 L. V. Skripnikov , N. S. Mosyagin , A. V. Titov

We calculate the coupling constants between the light vector mesons and heavy baryons within the framework of the light-cone QCD sum rule in the leading order of heavy quark effective theory. Most resulting sum rules are stable with the…

High Energy Physics - Phenomenology · Physics 2009-11-13 Peng-Zhi Huang , Hua-Xing Chen , Shi-Lin Zhu

The Dirac-Hartree-Fock plus many-body perturbation theory (DHF+MBPT) method has been used to calculate hyperfine structure constants for Fr. Calculated hyperfine structure anomaly for hydrogen-like ion has been shown to be in good agreement…

Atomic Physics · Physics 2018-12-06 E. A. Konovalova , Yu. A. Demidov , M. G. Kozlov , A. E. Barzakh

We study the decay constants of pseudoscalar and vector $B$ meson in the framework of light-cone quark model (LCQM). We apply the variational method to the relativistic Hamiltonian with the Gaussian-type trial wave function to obtain the…

High Energy Physics - Phenomenology · Physics 2018-04-04 Nisha Dhiman , Harleen Dahiya

Starting in 2001, the MILC Collaboration began a large scale calculation of heavy-light meson decay constants using clover valence quarks on ensembles of three flavor configurations. For the coarse configurations, with a=0.12 fm, eight…

High Energy Physics - Lattice · Physics 2008-11-26 MILC Collaboration , C. Bernard , S. Datta , C. DeTar , Steven Gottlieb , E. B. Gregory , U. M. Heller , J. Osborn , R. L. Sugar , D. Toussaint

Quantum-chemical calculations aimed at deriving magnetic coupling constants in exchange-coupled spin clusters commonly utilize a broken-symmetry (BS) approach. This involves calculating several distinct collinear spin configurations,…

Strongly Correlated Electrons · Physics 2023-10-23 Shadan Ghassemi Tabrizi

The central problem in electronic structure theory is the computation of the eigenvalues of the electronic Hamiltonian -- an unbounded, self-adjoint operator acting on a Hilbert space of antisymmetric functions. Coupled cluster (CC)…

Numerical Analysis · Mathematics 2023-01-30 Muhammad Hassan , Yvon Maday , Yipeng Wang