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We report the synthesis and characterization of molecular rectifying diodes on silicon using sequential grafting of self-assembled monolayers of alkyl chains bearing a pi group at their outer end (Si/sigma-pi/metal junctions). We…

Materials Science · Physics 2010-05-14 S. Lenfant , D. Guerin , F. Tran Van , C. Chevrot , S. Palacin , J. P. Bourgoin , O. Bouloussa , F. Rondelez , D. Vuillaume

The self-assembled monolayers of alkane thiolates on Ag (111) surfaces and nanoparticles are studied using molecular dynamics. Reactive force fields allow simulations of very large systems such as nanoparticles of 10 nm. Stable (sqrt(7) X…

Chemical Physics · Physics 2024-01-11 Adam Lahouari , Jean-Philip Piquemal , Johannes Richardi

Hybrid ferromagnetic metal/organic interfaces (spinterfaces) exhibit unique properties, including spin filtering. In parallel, chiral organic molecules can themselves induce efficient spin filtering, leading to unexpectedly high spin…

We use density functional theory and Monte Carlo lattice simulations to investigate the structure of ZrO$_{2}$ monolayers on Si(001). Recently, we have reported on the experimental growth of amorphous ZrO$_{2}$ monolayers on silicon and…

Materials Science · Physics 2019-06-27 Mehmet Dogan , Sohrab Ismail-Beigi

A two PDEs-based model is developed for studies of a morphological and compositional evolution of a thermodynamically stable alloy surface in a strong electric field, assuming different and anisotropic diffusional mobilities of the two…

Materials Science · Physics 2015-06-18 Mikhail Khenner , Mahdi Bandegi

We have used scanning probe microscopy to investigate self-assembled monolayers of chemically synthesized peptides. We find that the peptides form a dense uniform monolayer, above which is found a sparse additional layer. Using scanning…

Soft Condensed Matter · Physics 2009-10-31 David J. Bergeron , Wilfried Clauss , Denis L. Pilloud , P. Leslie Dutton , Alan T. Johnson

Monolayer group-IV monochalcogenides (MX, M = Ge, Sn, Pb; X = S, Se, Te) are a family of novel two-dimensional (2D) materials that have atomic structures closely related to that of the staggered black phosphorus lattice. The structure of…

Materials Science · Physics 2020-06-16 Kai Chang , Stuart S. P. Parkin

Bio-conjugated nanomaterials play a promising role in the development of novel supramolecular structures, molecular machines, and biosensing devices. In this study, lipid-conjugated gold nanoparticles were synthesized and allowed to form a…

Materials Science · Physics 2012-07-24 Subhasish Chatterjee , Markrete Krikorian , Harry D. Gafney , Bonnie Gersten

Mean-field theory is used to model polyelectrolyte adsorption and the possibility of overcompensation of charged surfaces. For charged surfaces that are also chemically attractive, the overcharging is large in high salt conditions,…

Soft Condensed Matter · Physics 2009-11-10 Adi Shafir , David Andelman

Ultrahigh electrostrains (greater than 1%) in several piezoceramic systems have been reported since 2022, which attract more and more interest in the field of piezoelectricity; however, the mechanism is still unclear. Here, we have directly…

Applied Physics · Physics 2023-12-07 Shuo Tian , Bin Li , Yejing Dai

Competing electronic phases in two-dimensional transition metal dichalcogenides constitute a fertile platform for uncovering emergent ground states and elucidating the control parameters that govern the correlated electron phases. Among…

Other Condensed Matter · Physics 2026-03-05 Ishita Pushkarna , Árpád Pásztor , Greta Lupi , Adolfo O. Fumega , Christoph Renner

The recently experimentally synthesized monolayer $\mathrm{MoSi_2N_4}$ and $\mathrm{WSi_2N_4}$ (\textcolor[rgb]{0.00,0.00,1.00}{Science 369, 670-674 (2020})) lack inversion symmetry, which allows them to become piezoelectric. In this work,…

Materials Science · Physics 2020-12-29 San-Dong Guo , Yu-Tong Zhu , Wen-Qi Mu , Lei Wang , Xing-Qiu Chen

In this paper, a consistent theory is developed for size-dependent piezoelectricity in dielectric solids. This theory shows that electric polarization can be generated as the result of coupling to the mean curvature tensor, unlike previous…

General Physics · Physics 2013-05-15 Ali R. Hadjesfandiari

Electromechanical coupling through piezoelectric polymer chains allows the emission of organic molecules in active nanowires to be tuned. This effect is evidenced by highly bendable arrays of counter-ion dye-doped nanowires made of a…

The effect of structural constriction on molecular mobility is investigated by broadband dielectric spectroscopy (BDS) within three types of molecular arrangements: monomers, oligomers and self-assembled monolayers (SAMs). While disordered…

We present calculations on the deformation of two- and three-layer electret systems. The electrical field is coupled with the stress-strain equations by means of the Maxwell stress tensor. In the simulations, two-phase systems are…

Materials Science · Physics 2007-05-23 Enis Tuncer , Michael Wegener , Reimund Gerhard-Multhaupt

Self-assembled monolayers (SAMs) have been used to improve both the positive and negative bias-stress stability of amorphous indium gallium zinc oxide (IGZO) bottom gate thin film transistors (TFTs). N-hexylphosphonic acid (HPA) and…

We have investigated the electronic structure of charged bilayer and trilayer phoshporene using first-principles, density-functional-theory calculations. We find that the effective dielectric constant for an external electric field applied…

Mesoscale and Nanoscale Physics · Physics 2017-08-09 Bukyoung Jhun , Cheol-Hwan Park

Temperature dependent structural changes in a nearly pure monoclinic phase composition (x=0.525) of Pb(Zr_xTi_1-x)O_3 (PZT) have been investigated using Rietveld analysis of high-resolution synchrotron powder x-ray diffraction data and…

We use first-principles calculations to investigate the band structure evolution of W$X_2$/Mo$X_2$ ($X$ = S, Se) heterobilayers under a perpendicular electric field. We characterize the extent to which the type-II band alignment in these…

Mesoscale and Nanoscale Physics · Physics 2016-12-28 Dennis Huang , Efthimios Kaxiras
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