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Modulation of electronic properties of materials by electric fields is central to the operation of modern semiconductor devices, providing access to complex electronic behaviors and greater freedom in tuning the energy bands of materials.…

Materials Science · Physics 2024-01-09 Ashwin Ramasubramaniam , Doron Naveh

The picosecond thermal response of a normal octadecanethiol self-assembled monolayer on a gold surface was studied using pump-probe, broadband-infrared, background-suppressed and vibrational sum frequency generation spectroscopy. The…

Materials Science · Physics 2014-05-27 Hiroki Fujiwara

Negative piezoelectrics contract in the direction of applied electric field, which are opposite to normal piezoelectrics and rare in dielectric materials. The raising of low dimensional ferroelectrics, with unconventional mechanisms of…

Materials Science · Physics 2023-12-19 Ziwen Wang , Shuai Dong

Piezoelectricity offers precise and robust conversion between electricity and mechanical force. Here we report the first experimental evidence of piezoelectricity in a single layer of molybdenum disulfide (MoS2) crystal as a result of…

Materials Science · Physics 2014-09-01 Hanyu Zhu , Yuan Wang , Jun Xiao , Ming Liu , Shaomin Xiong , Zi Jing Wong , Ziliang Ye , Xiaobo Yin , Xiang Zhang

We have modeled the layer-by-layer assembly process of flexible polyelectrolytes on flat surfaces. The multilayer has a three-zone structure. An exponential growth is found for the first several layers, followed by a linear growth for…

Soft Condensed Matter · Physics 2007-05-23 Qiang Wang

Since 2022, large apparent strains (>1%) with highly asymmetrical strain-electric field (S-E) curves have been reported in various thin piezoceramic materials, attributed to a bidirectional electric-field-induced bending (electrobending)…

Materials Science · Physics 2025-03-05 Yi Cheng , Shuo Tian , Bin Li , Yejing Dai

We examine the interactions between polyelectrolytes (PEs) and uncharged substrates at conditions corresponding to a dielectric discontinuity between the aqueous solution and the substrate. To this end, we vary the relevant system…

Soft Condensed Matter · Physics 2024-12-03 Hossein Vahid , Alberto Scacchi , Maria Sammalkorpi , Tapio Ala-Nissila

In this work, we demonstrate the tunability of electronic properties of Si/SiO2 substrate by molecular and ionic surface modifications. The change in the electronic properties such as the work function (WF) and electron affinity (EA), were…

We study mixtures of charged surfactants, which alone in solution form uni- and multilamellar vesicles, and oppositely charged polyelectrolytes (PEs). The phase behavior is investigated at fixed surfactant concentration as a function of the…

Soft Condensed Matter · Physics 2007-05-23 Laurence Ramos , Edith Vivares

Using first-principles calculations we show that the work function of noble metals can be decreased or increased by up to 2 eV upon the adsorption of self-assembled monolayers of organic molecules. We identify the contributions to these…

Other Condensed Matter · Physics 2007-05-23 Paul C. Rusu , Geert Brocks

Low-dimensional (LD) transition metal dichalcogenides (TMDs) in the form of nanoflakes, which consist of one or several layers, are the subject of intensive fundamental and applied research. Due to the size-induced transition from a bulk to…

Polar metals characterized by the simultaneous coexistence of ferroelectric distortions and metallicity have attracted tremendous attention. Developing such materials at low dimensions remains challenging since both conducting electrons and…

Materials Science · Physics 2020-03-24 Tao Xu , Jingtong Zhang , Yuquan Zhu , Jie Wang , Takahiro Shimada , Takayuki Kitamura , Tong-Yi Zhang

Molecular self-assembly has been extensively used for surface modification of metals and oxides for a variety of applications, including molecular and organic electronics. One of the goals of this research is to learn how the electronic…

Materials Science · Physics 2009-11-13 M. F. Calhoun , J. Sanchez , D. Olaya , M. E. Gershenson , V. Podzorov*

We report piezoelectric response in liquid phase exfoliated MoS2 nanosheets with desired structure and morphology. The piezoelectric effect in liquid phase exfoliated few layers of MoS2 flakes is interesting as it may allow the scalable…

Materials Science · Physics 2023-06-07 Jyoti Shakya , Gayathri H N , Arindam Ghosh

We report how the electron transport through a solid-state metal/Gly-Gly-His tripeptide (GGH) monolayer/metal junction and the metal/GGH work function are modified by the GGH complexation with Cu2+ ions. Conducting AFM is used to measure…

Ferroelectricity is usually found in compound materials composed by different elements. Here, based on first-principles calculations, we reveal the first example of spontaneous electrical polarization and ferroelectricity in stable…

Materials Science · Physics 2017-06-20 Chengcheng Xiao , Fang Wang , Shengyuan A. Yang , Yunhao Lu

Piezoelectrics are materials that linearly deform in response to an applied electric field. As a fundamental prerequisite, piezoelectric material must possess a non centrosymmetric crystal structure. For more than a century, this remains…

The adsorption of highly \textit{oppositely} charged flexible polyelectrolytes onto a charged spherical surface is investigated by means of Monte Carlo simulations in a fashion which resembles the layer-by-layer deposition technique…

Soft Condensed Matter · Physics 2007-05-23 Rene Messina , Christian Holm , Kurt Kremer

We compute the electronic structure of two-dimensional (2D) materials decorated with self-assembled organic monolayers using density functional theory. We find that 2D materials are strongly impacted by near-field electrostatic effects…

Materials Science · Physics 2021-09-22 Qunfei Zhou , Bukuru Anaclet , Trevor Steiner , Michele Kotiuga , Pierre Darancet

Sb and Bi monolayers, as single-elemental ferroelectric materials with similar atomic structure, hold intrinsic piezoelectricity theoretically, which makes them highly promising for applications in functional nano-devices such as sensors…

Materials Science · Physics 2023-09-22 Yunfei Hong , Junkai Deng , Qi Kong , Xiangdong Ding , Jun Sun , Jefferson Zhe Liu
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