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Polymeric ionic liquids are emerging polyelectrolyte materials for modern electrochemical applications. In this paper, we propose a self-consistent field theory of the polymeric ionic liquid on a charged conductive electrode. Taking into…

Soft Condensed Matter · Physics 2022-02-02 Yury A. Budkov , Nikolai N. Kalikin , Andrei L. Kolesnikov

Relevant information about the nature of the dynamics of ions in electrolytes can be obtained by studying the nonlinear dependence on an applied electric field. Here we use molecular dynamics (MD) simulations to study the field effects for…

Soft Condensed Matter · Physics 2025-03-21 Alina Wettstein , Diddo Diddens , Andreas Heuer

Vesicles self-assembled from amphiphilic diblock copolymers exhibit a wide diversity of behavior upon electroporation, due to competitions between edge, surface and bending energies that drive the system, while different viscous dissipation…

Soft Condensed Matter · Physics 2009-11-07 Harry Bermudez , Helim Aranda-Espinoza , Daniel A. Hammer , Dennis E. Discher , .

In this work, we carry out a study of the conserved quantities and dynamical structure of the four-dimensional modified axion electrodynamics theory described by the axion-photon coupling. In the first part of the analysis, we employ the…

High Energy Physics - Theory · Physics 2021-12-22 Omar Rodríguez-Tzompantzi

We investigate electro-osmosis in aqueous solutions of polyelectrolytes using mean-field equations. A solution of positively charged polyelectrolytes is confined between two negatively charged planar surfaces, and an electric field is…

Soft Condensed Matter · Physics 2015-06-16 Yuki Uematsu , Takeaki Araki

Polymer chains decorated with a fraction of monomers capable of forming reversible bonds form transient polymer networks that are important in soft and biological systems. If chains are flexible and the attractive monomers are all of the…

Soft Condensed Matter · Physics 2023-10-18 Lorenzo Rovigatti , Francesco Sciortino

Morphology of polymer electrolytes membranes (PEM), e.g., Nafion, inside PEM fuel cell catalyst layers has significant impact on the electrochemical activity and transport phenomena that determine cell performance. In those regions, Nafion…

Materials Science · Physics 2015-01-27 Daiane Damasceno Borges , Gerard Gebel , Alejandro A. Franco , Kourosh Malek , Stefano Mossa

We consider the statistical mechanics of a system of topologically linked polymers, such as for instance a dense solution of polymer rings. If the possible topological states of the system are distinguished using the Gauss linking number as…

Statistical Mechanics · Physics 2010-01-05 Franco Ferrari

The venerable theory of electrokinetic phenomena rests on the hypothesis of a dilute solution of point-like ions near a weakly charged surface, whose potential relative to the bulk is of order the thermal voltage ($kT/e \approx 25$ mV at…

Fluid Dynamics · Physics 2009-09-29 Martin Z. Bazant , Mustafa Sabri Kilic , Brian D. Storey , Armand Ajdari

Environmental oxidation has a great impact in tuning the physical, chemical and electronic properties of two-dimensional (2D) monolayers which can affect their practical applications in nanoscale engineering devices under ambient…

Materials Science · Physics 2025-11-18 Soumendra Kumar Das , Prasanjit Samal , Brahmananda Chakraborty , Sridhar Sahu

The Electron-Ion Collider~(EIC), a forthcoming powerful high-luminosity facility, represents an exciting opportunity to explore new physics. In this article, we study the potential of the EIC to probe the coupling between axion-like…

High Energy Physics - Phenomenology · Physics 2024-03-01 Reuven Balkin , Or Hen , Wenliang Li , Hongkai Liu , Teng Ma , Yotam Soreq , Mike Williams

Porous electrodes are found in energy storage devices such as supercapacitors and pseudocapacitors. However, the effect of electrode-pore-size distribution over their energy storage properties remains unclear. Here, we develop a model for…

Chemical Physics · Physics 2021-12-03 Filipe Henrique , Pawel J. Zuk , Ankur Gupta

Polyelectrolytes, such as polyacrylic acid (PAA), can effectively mitigate $\mathrm{CaCO_3}$ scale formation. Despite their success as antiscalants, the underlying mechanism of $\mathrm{Ca^{2+}}$ binding to polyelectrolyte chains remains…

Soft Condensed Matter · Physics 2024-03-21 Sriteja Mantha , Alec Glisman , Decai Yu , Eric Wasserman , Scott Backer , Zhen-Gang Wang

Pair potentials that are bounded at the origin provide an accurate description of the effective interaction for many systems of dissolved soft macromolecules (e.g., flexible dendrimers). Using numerical free-energy calculations, we…

Soft Condensed Matter · Physics 2014-10-29 C. Speranza , S. Prestipino , G. Malescio , P. V. Giaquinta

Recent advances in experimental and computational techniques have allowed for an accurate description of the adsorption of ionic liquids on metallic electrodes. It is now well established that they adopt a multi-layered structure, and that…

Materials Science · Physics 2016-03-15 Benjamin Rotenberg , Mathieu Salanne

Lithium iron phosphate (LiFePO$_4$) is the prototypical two-phase battery material, whose complex patterns of lithium ion intercalation provide a testing ground for theories of electrochemical thermodynamics. Using a depth-averaged (a-b…

Chemical Physics · Physics 2018-08-21 Daniel A. Cogswell , Martin Z. Bazant

Applications of nanoparticles in biology require that the nanoparticles remain stable in solutions containing high concentrations of proteins and salts, as well as in cell culture media. In this work, we developed simple protocols for the…

Soft Condensed Matter · Physics 2009-07-07 B. Chanteau , J. Fresnais , J. -F. Berret

The action principle by Low [Proc. R. Soc. Lond. A 248, 282--287] for the classic Vlasov-Maxwell system contains a mix of Eulerian and Lagrangian variables. This renders the Noether analysis of reparametrization symmetries inconvenient,…

Plasma Physics · Physics 2020-04-30 Eero Hirvijoki , Joshua W. Burby , David Pfefferlé , Alain J. Brizard

This paper presents a new technique to study the adsorption and desorption of ions and electrons on insulating surfaces in the presence of strong electric fields in cryoliquids. The experimental design consists of a compact cryostat coupled…

The interaction of ultra-intense lasers with solid foils can be used to accelerate ions to high energies well exceeding 60 MeV. The non-linear relativistic motion of electrons in the intense laser radiation leads to their acceleration and…