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Exploring an upper limit of magnetic anisotropy in two-dimensional materials, such as graphene and transition metal dichalcogenides, is at the heart of spintronics research. Herein, an atomic-scale perpendicular magnetic anisotropy up to an…

Materials Science · Physics 2016-08-10 Dorj Odkhuu

Spin-polarized transport through bistable magnetic adatoms or single-molecule magnets (SMMs), which exhibit both uniaxial and transverse magnetic anisotropy, is considered theoretically. The main focus is on the impact of transverse…

Mesoscale and Nanoscale Physics · Physics 2014-07-22 Maciej Misiorny , Józef Barnaś

The cause for the preferred spin orientation in magnetic systems containing spin-1/2 transition-metal ions was explored by studying the origin of the easy-plane anisotropy of the spin-1/2 Cu2+ ions in CuCl2.2H2O, LiCuVO4, CuCl2 and CuBr2 on…

Strongly Correlated Electrons · Physics 2015-06-22 Jia Liu , Hyun-Joo Koo , Hongjun Xiang , Reinhard K. Kremer , Myung-Hwan Whangbo

We have obtained analytical expressions for the q-dependent static spin susceptibility of monolayer transition metal dichalcogenides, considering both the electron-doped and hole-doped cases. Our results are applied to calculate…

Mesoscale and Nanoscale Physics · Physics 2016-05-24 H. Hatami , T. Kernreiter , U. Zülicke

Materials with large magnetocrystalline anisotropy and strong electric field effects are highly needed to develop new types of memory devices based on electric field control of spin orientations. Instead of using modified transition metal…

Materials Science · Physics 2017-08-02 Xuelei Sui , Tao Hu , Jianfeng Wang , Bing-Lin Gu , Wenhui Duan , Mao-sheng Miao

Using density functional theory, we investigate the electronic and magnetic properties of $3d$ transition-metal adatoms adsorbed on a monolayer of Mn on W(110). Mn/W(110) has a noncollinear cycloidal spin-spiral ground state with an angle…

Materials Science · Physics 2020-04-15 Mara Gutzeit , Soumyajyoti Haldar , Stefan Heinze

In intercalated transition metal dichalcogenide $Fe_xTaS_2$ (0.2 $\leq$ x $\leq$ 0.4) single crystals, large magnetic anisotropy is observed. Transport property measurements indicate that heavy Fe-doping leads to a large anisotropy of…

Strongly Correlated Electrons · Physics 2017-05-10 G. Wu , B. L. Kang , Y. L. Li , T. Wu , N. Z. Wang , X. G. Luo , Z. Sun , L. J. Zou , X. H. Chen

Both quantum and classical behavior of single atomic spins on surfaces is determined by the local anisotropy of adatoms and their coupling to the immediate electronic environment. Yet adatoms seldom reside on surfaces alone and it is…

Materials Science · Physics 2015-11-04 P. Ruiz-Díaz , O. V. Stepanyuk , V. S. Stepanyuk

We show that in the metallic phase of a two dimensional electron gas the spin-orbit coupling due to structure inversion asymmetry leads to a characteristic anisotropy in the magnetoconductance. Within the assumption that the metallic phase…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 P. Schwab , R. Raimondi

Transition metal dichalcogenides have been the primary materials of interest in the field of valleytronics for their potential in information storage, yet the limiting factor has been achieving long valley decoherence times. We explore the…

Mesoscale and Nanoscale Physics · Physics 2018-10-17 Christopher J. Ciccarino , Thomas Christensen , Ravishankar Sundararaman , Prineha Narang

We investigate via exact diagonalization of finite clusters the electronic structure and magnetism of M$_2$O$_9$ dimers in the mixed-valence hexagonal perovskites A$_3$B'M$_2$O$_9$ for various different fillings of 4$d$ and 5$d$…

Strongly Correlated Electrons · Physics 2021-01-04 Ying Li , Alexander A. Tsirlin , Tusharkanti Dey , Philipp Gegenwart , Roser Valenti , Stephen M. Winter

We propose an experiment, which would allow to pinpoint the role of spin-orbit coupling in the metal-nonmetal transition observed in a number of two-dimensional systems at low densities. Namely, we demonstrate that in a parallel magnetic…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 Guang-Hong Chen , M. E. Raikh , Yong-Shi Wu

We investigate the dynamics of Fe adatoms and dimers deposited on the Cu(111) metallic surface in the presence of spin-orbit coupling, within time-dependent density functional theory. The \textit{ab initio} results provide…

Mesoscale and Nanoscale Physics · Physics 2017-10-03 Filipe S. M. Guimarães , Manuel dos Santos Dias , Benedikt Schweflinghaus , Samir Lounis

Magnetic anisotropy (MA) is one of the most important material properties for modern spintronic devices. Conventional manipulation of the intrinsic MA, i.e. magnetocrystalline anisotropy (MCA), typically depends upon crystal symmetry.…

We consider layered decorated honeycomb lattices at two-thirds filling, as realized in some trinuclear organometallic complexes. Localized $S=1$ moments with a single-spin anisotropy emerge from the interplay of Coulomb repulsion and spin…

Strongly Correlated Electrons · Physics 2017-11-15 J. Merino , A. C. Jacko , A. L. Khosla , B. J. Powell

Using an ab initio density functional theory (DFT) based electronic structure method, we study the effects of adatoms on the electronic properties of monolayer transition metal dichalcogenide (TMD) Molybdenum-disulfide (MoS2). We consider…

Mesoscale and Nanoscale Physics · Physics 2014-04-08 Jiwon Chang , Stefano Larentis , Emanuel Tutuc , Leonard F. Register , Sanjay K. Banerjee

We put forward a scheme to study the anisotropic magnetic couplings in Sr2IrO4 by mapping fully relativistic constrained noncollinear density functional theory including an on-site Hubbard U correction onto a general spin model Hamiltonian.…

It is shown that the spin-orbit coupling due to structure inversion asymmetry leads to a characteristic anisotropy in the magnetoconductance of two-dimensional metals. Relevance for recent experiments is discussed.

Mesoscale and Nanoscale Physics · Physics 2009-11-07 R. Raimondi , M. Leadbeater , P. Schwab , E. Caroti , C. Castellani

The properties of quantum systems interacting with their environment, commonly called open quantum systems, can be strongly affected by this interaction. While this can lead to unwanted consequences, such as causing decoherence in qubits…

We analyze magnetic phases of monolayers of transition metal dichalcogenides that are two-valley materials with electron-electron interactions. The exchange inter-valley scattering makes two-valley systems less stable to the spin…

Strongly Correlated Electrons · Physics 2019-07-31 Dmitry Miserev , Jelena Klinovaja , Daniel Loss
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