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Structural changes in a glass due to deformation are subtle and difficult to quantify using conventional imaging and diffraction techniques. Additionally, transmission electron microscopy (TEM) sample preparation using energetic ions often…

The nonlinear rheological properties of dense suspensions are discussed within simplified models, suggested by a recent first principles approach to the model of Brownian particles in a constant-velocity-gradient solvent flow. Shear…

Soft Condensed Matter · Physics 2015-06-24 Matthias Fuchs , Michael E. Cates

Glasses have liquid-like structure, but exhibit solid-like properties. A central question concerns the relation between the structure and mechanical properties of glasses, but structural changes remain difficult to resolve. We use a novel…

Soft Condensed Matter · Physics 2013-04-04 D. V. Denisov , M. T. Dang , B. Struth , G. H. Wegdam , P. Schall

The glass transition remains one of the great unsolved mysteries of contemporary condensed matter physics. When crystallization is bypassed by rapid cooling, a supercooled liquid, retaining amorphous particle arrangment, results. The…

Materials Science · Physics 2016-10-12 Nicholas B. Weingartner , Zohar Nussinov

We propose a dynamical theory of low-temperature shear deformation in amorphous solids. Our analysis is based on molecular-dynamics simulations of a two-dimensional, two-component noncrystalline system. These numerical simulations reveal…

Statistical Mechanics · Physics 2009-10-30 M. L. Falk , J. S. Langer

Plastic deformation in metallic glasses at room temperature leads to the development of shear bands due to shear localization. In many experiments, shear bands have shown local density variations along their path, with a distinct imbalance…

Disordered Systems and Neural Networks · Physics 2024-07-22 Harald Rösner , Arabinda Bera , Alessio Zaccone

We report experiments on hard sphere colloidal glasses that reveal a type of shear banding hitherto unobserved in soft glasses. We present a scenario that relates this to an instability arising from shear-concentration coupling, a mechanism…

Soft Condensed Matter · Physics 2015-05-19 R. Besseling , L. Isa , P. Ballesta , G. Petekidis , M. E. Cates , W. C. K. Poon

Concentrated particulate suspensions, commonplace in the pharmaceutical, cosmetic and food industries, display intriguing rheology. In particular, the dramatic increase in viscosity with strain rate (shear thickening and jamming) which is…

Soft Condensed Matter · Physics 2011-01-13 M. I. Smith , R. Besseling , M. E. Cates , V. Bertola

A wide range of materials can exist in microscopically disordered solid forms, referred to as amorphous solids or glasses. Such materials -- oxide glasses and metallic glasses, to polymer glasses, and soft solids such as colloidal glasses,…

Soft Condensed Matter · Physics 2021-08-20 Anshul D. S. Parmar , Srikanth Sastry

Molecular dynamics simulations of shear band development over 1000% strain in simple shear are used to test whether the local plastic strain rate is proportional to exp(-1/chi), where chi is a dimensionless quantity related to the "disorder…

Materials Science · Physics 2007-06-14 Yunfeng Shi , Michael B. Katz , Hui Li , Michael L. Falk

The transport of slightly deformable chiral objects in a uniform shear flow is investigated. Depending on the equilibrium configuration one finds up to four different asymptotic states that can be distinguished by a lateral drift velocity…

Soft Condensed Matter · Physics 2012-07-06 Peter Talkner , Gert-Ludwig Ingold , Peter Hanggi

Using molecular dynamics simulation, we examine the dynamics of crystal, polycrystal, and glass in a Lennard-Jones binary mixture composed of small and large particles in two dimensions. The crossovers occur among these states as the…

Soft Condensed Matter · Physics 2010-05-04 Hayato Shiba , Akira Onuki

Computer simulations of yielding of glasses under shear have typically been performed under constant volume, strain controlled protocols. However, volumetric effects, such as the dilatancy associated with plastic rearrangements, and the…

Soft Condensed Matter · Physics 2026-02-10 Krishna K Tiwari , Srikanth Sastry

In two-dimensional Lennard-Jones glasses, mechanical probing reveals that local yield surfaces are dominated by regions with a positive second derivative of the yield stress with respect to the loading angle. Each feature corresponds to a…

Soft Condensed Matter · Physics 2026-03-19 Spencer Fajardo , Paul Desmarchelier , Sylvain Patinet , Michael L. Falk

The influence of alternating shear orientation and strain amplitude of cyclic loading on yielding in amorphous solids is investigated using molecular dynamics simulations. The model glass is represented via a binary mixture that was rapidly…

Soft Condensed Matter · Physics 2020-12-08 Nikolai V. Priezjev

In this paper we study the mechanical properties and pore structure in a three-dimensional molecular dynamics model of porous glass under athermal quasistatic shear. The vitreous samples are prepared by rapid thermal quench from a high…

Soft Condensed Matter · Physics 2021-06-08 Sucharita Niyogi , Bhaskar Sen Gupta

We study shear yielding and steady state flow of glassy materials with molecular dynamics simulations of two standard models: amorphous polymers and bidisperse Lennard-Jones glasses. For a fixed strain rate, the maximum shear yield stress…

Soft Condensed Matter · Physics 2009-11-10 Joerg Rottler , Mark O. Robbins

We use a custom shear cell coupled to an optical microscope to investigate at the particle level the yielding transition in concentrated emulsions subjected to an oscillatory shear deformation. By performing experiments lasting thousands of…

Soft Condensed Matter · Physics 2014-08-27 E. D. Knowlton , D. J. Pine , L. Cipelletti

It has been a long-standing materials science challenge to establish structure-property relations in amorphous solids. Here we introduce a rotation-variant local structure representation that enables different predictions for different…

Materials Science · Physics 2022-03-15 Zhao Fan , Evan Ma

When amorphous solids are strained they display elastic deformation at small strain, however, beyond a critical strain they yield and begin to flow plastically. The origin of this plasticity lies in the irreversible rearrangement of…

Soft Condensed Matter · Physics 2019-09-19 Atharva Pandit , Antina Ghosh , Vijayakumar Chikkadi