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1$T$-TaS$_2$ is the only insulating transition-metal dichalcogenide (TMD) with an odd number of electrons per unit cell. This insulating state is non-magnetic, making it a potential spin-liquid candidate. The unusual electronic behavior…

Strongly Correlated Electrons · Physics 2024-06-28 Amir Dalal , Jonathan Ruhman , Jörn W. F. Venderbos

Two-dimensional layered transition metal dichalcogenide (TMDC) materials often exhibit exotic quantum matter phases due to the delicate coupling and competitions between the charge, lattice, orbital, and spin degrees of freedom.…

Mesoscale and Nanoscale Physics · Physics 2018-02-07 Seho Yi , Zhenyu Zhang , Jun-Hyung Cho

We investigate the low-temperature charge-density-wave (CDW) state of bulk TaS$_2$ with a fully self-consistent DFT+U approach, over which the controversy has remained unresolved regarding the out-of-plane metallic band. By examining the…

Strongly Correlated Electrons · Physics 2021-05-19 Dongbin Shin , Nicolas Tancogne-Dejean , Jin Zhang , Mahmut Sait Okyay , Angel Rubio , Noejung Park

Here we report a comprehensive inelastic light scattering studies on 1T-TaS2 with different thickness. This compound is well known for its rich charge density wave phases. Along with that it has been one of the promising candidates for a…

Strongly Correlated Electrons · Physics 2025-05-06 Vivek Kumar , Birender Singh , Pradeep Kumar

Combination of low-dimensionality and electron correlation is vital for exotic quantum phenomena such as the Mott-insulating phase and high-temperature superconductivity. Transition-metal dichalcogenide (TMD) 1T-TaS2 has evoked great…

We investigate the interplay of the electron-electron and electron-phonon interactions in the electronic structure of an exotic insulating state in the layered dichalcogenide 1T-TaS2, where the charge-density-wave (CDW) order coexists with…

Materials Science · Physics 2017-07-12 Doohee Cho , Yong-Heum Cho , Sang-Wook Cheong , Ki-Seok Kim , Han Woong Yeom

1T-tantalum disulphide (1T-TaS2) is a promising material to realize quantum spin liquid state and fractional excitations. Here, we take a closer look on the temperature dependent magnetic susceptibility of 1T-TaS2 at low magnetic fields to…

Strongly Correlated Electrons · Physics 2022-07-28 Sudip Pal , S. B. Roy

Low-dimensional electron systems, as realized naturally in graphene or created artificially at the interfaces of heterostructures, exhibit a variety of fascinating quantum phenomena with great prospects for future applications. Once…

Strongly Correlated Electrons · Physics 2016-08-03 T. Ritschel , J. Trinckauf , K. Koepernik , B. Büchner , M. v. Zimmermann , H. Berger , Y. I. Joe , P. Abbamonte , J. Geck

We present the zero-temperature phase diagram of the one-dimensional t2g-orbital Hubbard model, obtained using the density-matrix renormalization group and Lanczos techniques. Emphasis is given to the case for the electron density n=5…

Strongly Correlated Electrons · Physics 2009-11-11 Jose Xavier , Hiroaki Onishi , Takashi Hotta , Elbio Dagotto

Strong electron-electron interaction can induce Mott insulating state, which is believed to host unusual correlated phenomena such as quantum spin liquid when quantum fluctuation dominates and unconventional superconductivity through…

Strongly Correlated Electrons · Physics 2025-04-24 Qiang Gao , Haiyang Chen , Wen-shin Lu , Yang-hao Chan , Zhenhua Chen , Yaobo Huang , Zhengtai Liu , Peng Chen

Recently, many exotic electronic states, such as quantum spin liquid (QSL) and superconductivity (SC), have been extensively discovered and introduced in layered transition metal dichalcogenides 1T-TaS2 by controlling their complex…

Materials Science · Physics 2022-12-08 Geng Yanyan , Lei Le , Dong Haoyu , Guo Jianfeng , Mi Shuo , Li Yan , Huang Li , Pang Fei , Xu Rui , Zhou Weichang , Liu Zheng , Ji Wei , Cheng Zhihai

Two-dimensional layered transition-metal-dichalcogenide compound 1T-TaS2 shows the rare coexistence of charge density wave (CDW) and electron correlation driven Mott transition. In addition, atomic-cluster spins on the triangular lattice of…

Strongly Correlated Electrons · Physics 2022-07-28 Sudip Pal , Kranti Kumar , Rohit Sharma , A Banerjee , S B Roy , Je-Geun Park , A. K. Nigam , Sang-Wook Cheong

The magnetic properties of NiTa$_2$O$_6$ were investigated by magnetic susceptibility, specific heat, electron paramagnetic resonance, neutron powder diffraction and pulse field magnetization measurements. Accompanying \textit{ab initio}…

Strongly Correlated Electrons · Physics 2015-06-18 J. M. Law , H. -J. Koo , M. -H. Whangbo , E. Bruecher , V. Pomjakushin , R. K. Kremer

The layered transition metal dichalcogenide compounds 1T-TaS2 and 4H-TaS2 are well known for their exotic properties, which include charge density wave, superconductivity, Mott transition, etc., and lately quantum spin liquid. Here, we…

The low-temperature metallic phase of 1T-TaS2 may originate from current- and voltage-driven destabilization of the commensurate charge density wave (CDW) in a strongly correlated Mott insulator, alongside the robust yet rarely realized…

We have investigated the effect of the magnetic field (B) on the very low-temperature equilibrium heat capacity ceq of the quasi-1 D organic compound (TMTTF)2Br, characterized by a commensurate Spin Density Wave (SDW) ground state. Below…

Disordered Systems and Neural Networks · Physics 2007-10-11 S. Sahling , J. C. Lasjaunias , R. Mélin , P. Monceau , G. Reményi

Coexistence of localized and extended excitations is central to the macroscopic properties of correlated materials. For 5d transition metal compounds, electron correlations alone generally do not lead to a metal-insulator (Mott) transition,…

The charge density wave (CDW) transition temperature in the quasi-one dimensional (Q1D) organic material of (Per)$_2$Au(mnt)$_2$ is relatively low (TCDW = 12 K). Hence in a mean field BCS model, the CDW state should be completely suppressed…

Strongly Correlated Electrons · Physics 2009-11-10 D. Graf , J. S. Brooks , E. S. Choi , S. Uji , J. C. Dias , M. Almeida , M. Matos

This study investigates the electronic states and physical quantities of an organic charge-transfer complex HMTSF-TCNQ, which undergoes a charge-density-wave (CDW) phase transition at temperature $T_c\simeq 30$ K. A first-principles…

Materials Science · Physics 2021-11-03 S. Ozaki , I. Tateishi , H. Matsuura , M. Ogata , K. Hiraki

Competing and intertwined orders including inhomogeneous patterns of spin and charge are observed in many correlated electron materials, such as high-temperature superconductors. Introducing a new development of the constrained-path…

Strongly Correlated Electrons · Physics 2023-02-24 Bo Xiao , Yuan-Yao He , Antoine Georges , Shiwei Zhang
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