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Femtosecond electron microscopy produces real-space images of matter in a series of ultrafast snapshots. Pulses of electrons self-disperse under space-charge broadening, so without compression, the ideal operation mode is a single electron…

Accelerator Physics · Physics 2016-04-21 A. R. Bainbridge , C. W. Barlow-Myers , W. A. Bryan

We present the development of the first ultrafast transmission electron microscope (UTEM) driven by localized photoemission from a field emitter cathode. We describe the implementation of the instrument, the photoemitter concept and the…

The need for ever-faster information processing requires extremely small devices operating at frequencies approaching the terahertz and petahertz regimes. For the diagnostics of such devices, researchers need a spatiotemporal tool that…

Applied Physics · Physics 2024-01-30 Maximilian Mattes , Mikhail Volkov , Peter Baum

Significant progress has been made in spatial resolution using environmental transmission electron microscopes (ETEM), which now enables atomic resolution visualization of structural transformation under variable temperature and gas…

Materials Science · Physics 2015-06-18 Wenpei Gao , Jianbo Wu , Xiaofeng Zhang , Aram Yoon , J. Mabon , W. Swiech , W. L. Wilson , H. Yang , Jian-Min Zuo

Ultrafast Electron Microscopy (UEM) has been demonstrated to be an effective table-top technique for imaging the temporally-evolving dynamics of matter with subparticle spatial resolution on the time scale of atomic motion. However, imaging…

Optics · Physics 2017-08-02 M. Th. Hassan , J. S. Baskin , B. Liao , A. H. Zewail

Instruments to visualize transient structural changes of inhomogeneous materials on the nanometer scale with atomic spatial and temporal resolution are demanded to advance materials science, bioscience, and fusion sciences. One such…

Accelerator Physics · Physics 2017-03-20 X. Shen , R. K. Li , U. Lundström , T. J. Lane , A. H. Reid , S. P. Weathersby , X. J. Wang

Ultrafast transmission electron microscopy (UTEM) has emerged as a versatile technique for the time-resolved imaging of nanoscale dynamics on timescales down to few-hundred attoseconds but the temporal and spatial resolutions are still…

Instrumentation and Detectors · Physics 2024-11-01 Alexander Schröder , Andreas Wendeln , Jonathan T. Weber , Masaki Mukai , Yuji Kohno , Sascha Schäfer

Electrical pulse stimulation drives many important physical phenomena in condensed matter as well as in electronic systems and devices. Often, nanoscopic and mesoscopic mechanisms are hypothesized, but methods to image electrically driven…

Mesoscale and Nanoscale Physics · Physics 2023-06-05 Thomas E Gage , Daniel B Durham , Haihua Liu , Supratik Guha , Ilke Arslan , Charudatta Phatak

The investigation of ultrafast electronic and structural dynamics in low-dimensional systems like nanowires and two-dimensional materials requires femtosecond probes providing high spatial resolution and strong interaction with small volume…

Mesoscale and Nanoscale Physics · Physics 2014-11-18 Melanie Müller , Alexander Paarmann , Ralph Ernstorfer

Femtosecond point-projection microscopy (fs-PPM) is an electron microscopy technique that possesses a combination of high spatio-temporal resolution and sensitivity to local electric fields. This allows it to visualize ultrafast charge…

Applied Physics · Physics 2018-03-06 Faruk Krečinić , Jannik Malter , Alexander Paarmann , Melanie Müller , Ralph Ernstorfer

Scanning transmission electron microscopy (STEM) has advanced rapidly in the last decade thanks to the ability to correct the major aberrations of the probe forming lens. Now atomic-sized beams are routine, even at accelerating voltages as…

Pump-probe electron energy-loss spectroscopy (EELS) with femtosecond temporal resolution will be a transformative research tool for studying non-equilibrium chemistry and electronic dynamics of matter. In this paper, we propose a new…

Accelerator Physics · Physics 2017-11-15 R. K. Li , X. J. Wang

The electronic, optical, and magnetic properties of quantum solids are determined by their low-energy (< 100 meV) many-body excitations. Dynamical characterization and manipulation of such excitations relies on tools that combine…

Mesoscale and Nanoscale Physics · Physics 2018-03-28 E. Pomarico , I. Madan , G. Berruto , G. M. Vanacore , K. Wang , I. Kaminer , F. J. García de Abajo , F. Carbone

In the last decade, the development of Ultrafast Electron Diffraction (UED) and Microscopy (UEM) has enabled the imaging of atomic motion in real time and space. These pivotal table-top tools opened the door for a vast range of applications…

Chemical Physics · Physics 2018-01-16 Mohammed Th. Hassan

Integrating femtosecond (fs) lasers to electron microscopies has enabled direct imaging of transient structures and morphologies of materials in real time and space, namely, ultrafast electron microscopy (UEM). Here we report the…

Transmission electron microscopy (TEM) has reached ~ 50 picometer resolution in a high vacuum, enabling single-atom sensitive imaging of nanomaterials. Extending this capability to gaseous environments would allow for similar visualizations…

Ultrafast electron microscopy provides a movie-like access to structural dynamics of materials in space and time, but fundamental atomic motions or electron dynamics are, so far, too quick to be resolved. Here we report the all-optical…

Optics · Physics 2024-02-27 J. Kuttruff , D. Nabben , A. C. Zimmermann , A. Ryabov , P. Baum

In modern high-gain free-electron lasers, ultra-fast photon pulses designed for studying chemical, atomic and biological systems are generated from a serial of behaviors of high-brightness electron beam at the time-scale ranging from…

Accelerator Physics · Physics 2015-10-22 Guanglei Wang , Meng Zhang , Wei Zhang , Haixiao Deng , Xueming Yang

Watching the motion of electrons on their natural nanometre length- and femtosecond time scales is a fundamental goal and an open challenge of contemporary ultrafast science. Optical techniques and electron microscopy currently mostly…

Optics · Physics 2018-01-23 Jan Vogelsang , Germann Hergert , Dong Wang , Petra Groß , Christoph Lienau

Atomic resolution imaging in transmission electron microscopy (TEM) and scanning TEM (STEM) of light elements in electron-transparent materials has long been a challenge. Biomolecular materials, for example, are rapidly altered when…

Instrumentation and Detectors · Physics 2018-12-05 Fehmi S. Yasin , Tyler R. Harvey , Jordan J. Chess , Jordan S. Pierce , Colin Ophus , Peter Ercius , Benjamin J. McMorran
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