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First-order structural phase transition is a common phenomenon in materials that qualitatively alters their physical properties. Yet, the abrupt first-order nature is usually unexplained by realistic computations, implying an omission of…

Strongly Correlated Electrons · Physics 2026-03-16 Xingchen Shen , Wei Ku

The corrosion behavior of NiCr alloys in molten FLiNaK salt is governed by complex Cr-F chemical interactions, necessitating a fundamental understanding for enhancing alloy performance in harsh environments. However, significant gaps remain…

Materials Science · Physics 2025-06-23 Hamdy Arkoub , Daniel Flynn , Adri C. T. van Duin , Miaomiao Jin

Oxide heterostructures have shown rich physics phenomena, particularly in the conjunction of exotic insulator-metal transition (IMT) at the interface between polar insulator LaAlO3 and non-polar insulator SrTiO3 (LaAlO3/SrTiO3).…

The discovery of ambient-pressure nickelate high-temperature superconductivity provides a new platform for probing the underlying superconducting mechanisms. However, the thermodynamic metastability of Ruddlesden-Popper nickelates…

Superconductivity · Physics 2026-03-05 Wei Lv , Zihao Nie , Heng Wang , Haoliang Huang , Guangdi Zhou , Qikun Xue , Zhuoyu Chen

The oxidation kinetics of hematite {\alpha}-Fe$_2$O$_3$(0001) surfaces are vital for its applications in catalysis, environmental remediation, and industrial processes. Despite prior studies, the roles of temperature, oxygen partial…

Materials Science · Physics 2026-05-21 Nishant Kumar , Matthias Blatnik , Jan Čechal

Layered chalcogenides including Bi2Te3, Sb2Te3, Bi-Sb-Te ternary alloys and heterostructures are known as great thermoelectric, topological insulators and recently highlighted as plasmonic building blocks beyond noble metals. Here, we…

Elucidating the catalytic descriptor that accurately characterizes the structure-activity relationships of typical catalysts for various important heterogeneous catalytic reactions is pivotal for designing high-efficient catalytic systems.…

Chemical Physics · Physics 2025-10-23 Zhen Zhu , Shan Gao , Jing Zhang , Xuxin Kang , Shunfang Li , Xiangmei Duan

The hexagonal perovskite BaNiO3, prepared via non-ceramic approaches, is known to act as a good catalyst for the oxygen-evolution reaction (OER) in alkaline media. Here we report our observation that BaNiO3 synthesized via KOH flux growth…

The rational design of transition metal dichalcogenide electrocatalysts for efficiently catalyzing hydrogen evolution reaction (HER) is believed to lead to the generation of a renewable energy carrier. To this end our work has made three…

The synthesis of high-quality Ruddlesden-Popper (RP) nickelates remains challenging due to variations in oxygen content and the prevalence of intergrown RP phases. Precisely controlling the stoichiometry and characterizing the resulting…

High-transition-temperature ($T_{C}$) superconductivity is recently discovered in Ruddlesden-Popper (RP) nickelate films with extraordinarily strong oxidation. While investigating phase diagrams is essential for uncovering the…

We developed a facile and scalable 3-step hydrothermal, electrodeposition, and annealing technique to synthesize a variety of nanowire heterostructures. The heterojunction catalysts of CP-ZnO-MoS2 and CP-ZnO-ZnS-MoS2 both saw an increase in…

Materials Science · Physics 2025-03-10 Lee Kendall , Dawn Ford , Giovanni Zangari , Stephen McDonnell

Metal-support interfaces fundamentally govern the catalytic performance of heterogeneous systems through complex interactions. Here, utilizing operando transmission electron microscopy, we uncovered a type of looping metal-support…

Materials Science · Physics 2025-07-08 Yue Pan , Shiyu Zhen , Xiaozhi Liu , Mengshu Ge , Jianxiong Zhao , Lin Gu , Dan Zhou , Liang Zhang , Dong Su

Molybdenum disulfide (MoS2) has emerged as a promising, cost-effective catalyst for hydrogen production via water splitting. We investigate the structural and electrocatalytic properties of MoS2 thin films deposited on different substrates…

Nontrivial topology in type-II Dirac semimetal NiTe$_2$ leading to topologically protected surface states give rise to fascinating phenomena holding great promise for next-generation electronic and spintronic devices. Key parameters $-$…

Strongly Correlated Electrons · Physics 2025-06-13 Neeraj Bhatt , Asif Ali , Deepali Sharma , Sakshi Bansal , Manasi Mandal , Ravi Prakash Singh , Ravi Shankar Singh

The honeycomb lattice iridate Na$_2$IrO$_3$ shows frustrated magnetism and can potentially display Kitaev-like exchange interactions. Recently, it was shown that the electronic properties of the surface of crystalline Na$_2$IrO$_3$ can be…

Materials Science · Physics 2018-09-25 Aastha Vasdev , Lalit Yadav , Suman Kamboj , Kavita Mehlawat , Yogesh Singh , Goutam Sheet

Tricobalt tetraoxide (Co3O4) is an important catalyst and Co3O4(110) is a frequently exposed surface in Co3O4 nanomaterials. We employed Density-functional theory with on-site Coulomb repulsion U term to study the atomic structures,…

Materials Science · Physics 2015-06-04 Jia Chen , Annabella Selloni

Nickelate films have recently attracted broad attention due to the observation of superconductivity in the infinite layer phase of $Nd_{0.8}Sr_{0.2}NiO_2$ (obtained by reducing Sr doped $NdNiO_3$ films) and their similarity to the cuprates…

Superconductivity · Physics 2021-12-15 Gad Koren , Anna Eyal , Leonid Iomin , Yuval Nitzav

The recent discovery of high-temperature superconductivity in high-pressurized La$_3$Ni$_2$O$_{7-\delta}$ has garnered significant attention. Using density functional theory, we investigate the magnetic properties of…

Materials Science · Physics 2024-12-30 Xiao-Sheng Ni , Yuyang Ji , Lixin He , Tao Xie , Dao-Xin Yao , Meng Wang , Kun Cao

Electrocatalytic hydrogenation of nitrobenzene (Ph-NO2) reaction (EHNR) has been considered as a potential alternative to the traditional thermocatalytic process in the production of high-value aniline (Ph-NH2). However, due to the absence…

Chemical Physics · Physics 2024-03-26 Yuchen Wang , Yaoyu Liu , Zhiyue Zhao , Zhikeng Zheng , Alina M. Balu , Rafael Luque , Kai Yan