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MeV ultrafast electron diffraction (UED) is a widely used technology for ultrafast structural dynamic studies of matters in numerous areas. The development of laser wakefield accelerator (LWFA) envisions great potential of advanced…

Accelerator Physics · Physics 2024-04-22 Yu Fang , Fei Li , Jianfei Hua , Bo Guo , Linyi Zhou , Bing Zhou , Zhihao Chen , Jianyi Liu , Zheng Zhou , Yipeng Wu , Yingchao Du , Renkai Li , Wei Lu

The temporal resolution of MeV ultrafast electron diffraction (UED) is fundamentally constrained by the electron bunch length at the sample, motivating the development of new electron sources capable of producing femtosecond scale bunches.…

Ultrafast electron diffraction and phonon-diffuse scattering (UED(S)) experiments make use of photo-induced changes to electron scattering intensity across 2D detectors to report on a very wide range of dynamic structural phenomena in…

Instrumentation and Detectors · Physics 2026-04-20 Laurenz Kremeyer , David Cai , Malik Lahlou , Sebastian Hammer , Raphael Schwenzer , Bradley J. Siwick

We study the non-equilibrium structural dynamics of the incommensurate and nearly-commensurate charge-density wave phases in 1T-TaS$_2$. Employing ultrafast low-energy electron diffraction (ULEED) with 1 ps temporal resolution, we…

We demonstrate ultralow phase noise 10-GHz microwave signal generation from a free-running mode-locked Er-fiber laser with -142 and -157 dBc/Hz single-sideband absolute phase noise at 10- and 100-kHz offset frequencies, respectively. The…

Optics · Physics 2013-11-05 Kwangyun Jung , Junho Shin , Jungwon Kim

We demonstrate a remarkably effective single-stage compression technique for ultrafast pulses in the visible electromagnetic spectrum using second-harmonic pulses at 515 nmderived from a 1030 nm Yb-based femtosecond regenerative amplifier.…

We demonstrate an active carrier-envelope phase (CEP) stabilization scheme for optical waveforms generated by difference-frequency mixing of two spectrally detuned and phase-correlated pulses. By performing ellipsometry with spectrally…

Ultrafast Electron Microscopy (UEM) has been demonstrated to be an effective table-top technique for imaging the temporally-evolving dynamics of matter with subparticle spatial resolution on the time scale of atomic motion. However, imaging…

Optics · Physics 2017-08-02 M. Th. Hassan , J. S. Baskin , B. Liao , A. H. Zewail

Since the discovery of electron-wave duality, electron scattering instrumentation has developed into a powerful array of techniques for revealing the atomic structure of matter. Beyond detecting local lattice variations in equilibrium…

Visualizing ultrafast dynamics at the atomic scale requires time-resolved pump-probe characterization with femtosecond temporal resolution. For single-shot ultrafast electron diffraction (UED) with fully relativistic electron bunch probes,…

In the last decade, the development of Ultrafast Electron Diffraction (UED) and Microscopy (UEM) has enabled the imaging of atomic motion in real time and space. These pivotal table-top tools opened the door for a vast range of applications…

Chemical Physics · Physics 2018-01-16 Mohammed Th. Hassan

Compression of UV femtosecond laser pulses focused into a gas cell filled with xenon is reported numerically. With a large negative Kerr index and normal dispersion, xenon promotes temporal modulational instability (MI) which can be…

Optics · Physics 2010-02-03 L. Berge , C. Koehler , S. Skupin

Two nominally identical ultra-stable cryogenic microwave oscillators are compared. Each incorporates a dielectric-sapphire resonator cooled to near 6 K in an ultra-low vibration cryostat using a low-vibration pulse-tube cryocooler. The…

Instrumentation and Detectors · Physics 2012-05-15 John G. Hartnett , Nitin R. Nand , Chuan Lu

A dc electron gun, generating picosecond pulses with up to $8\times10^{6}$ electrons per pulse, was developed. Its applicability for future time-resolved-diffraction experiments on state- and conformer-selected laser-aligned or oriented…

Chemical Physics · Physics 2016-02-25 Nele L. M. Müller , Sebastian Trippel , Karol Długołecki , Jochen Küpper

In this work, non-destructive virtual diagnostics are applied to retrieve the electron beam time of arrival and energy in a relativistic ultrafast electron diffraction (UED) beamline using independently-measured machine parameters. This…

We review the conventional phase-locking technique in the long-term stabilization of the mode-locked fiber laser and investigate the phase noise limitation of the conventional technique. To break the limitation, we propose an improved…

Optics · Physics 2014-03-12 Dong Hou , Bo Ning , Shuangyou Zhang , Jiutao Wu , Jianye Zhao

A source of ultrashort pulses of light in the 2 {\mu}m region was constructed using supercontinuum broadening from an erbium mode-locked laser. The output spectrum spanned 1000 nm to 2200 nm with an average power of 250 mW. A pulse width of…

Optics · Physics 2017-07-26 Andrew Klose , Gabriel Ycas , Daniel L. Maser , Scott A. Diddams

We demonstrate compression of 95 keV, space-charge-dominated electron bunches to sub-100 fs durations. These bunches have sufficient charge (200 fC) and are of sufficient quality to capture a diffraction pattern with a single shot, which we…

This paper presents the experimental realization of an ultrafast electron microscope operating at a repetition rate of 75 MHz based on a single compact resonant microwave cavity operating in dual mode. This elliptical cavity supports two…

Applied Physics · Physics 2019-01-29 J. F. M. van Rens , W. Verhoeven , E. R. Kieft , P. H. A. Mutsaers , O. J. Luiten

When an electromagnetic (EM) wave is propagating in a medium whose properties are varied abruptly in time, the wave experiences refractions and reflections known as "time-refractions" and "time-reflections", both manifesting spectral…

Applied Physics · Physics 2023-10-05 Thomas R. Jones , Alexander V. Kildishev , Mordechai Segev , Dimitrios Peroulis