Related papers: Second-order Nonlinear Optical Microscopy of Spide…
Charge transport processes at interfaces which are governed by complex interfacial electronic structure play a crucial role in catalytic reactions, energy storage, photovoltaics, and many biological processes. Here, the first soft X-ray…
Nonlinear optical generation has been a well-established way to realize frequency conversion in nonlinear optics, whereas previous studies were just focusing on the scalar light fields. Here we report a concise yet efficient experiment to…
We report a direct observation on the unique laterally emitted surface second harmonic generation (SHG) in a single ZnTe nanowire. The highly directional surface SHG signal that polarizes along the direction vertical to the nanowire growth…
Integrating 2D materials onto on-chip photonic devices holds significant potential for nonlinear frequency conversion across various applications. The lack of inversion symmetry in monolayers of transition metal dichalcogenides (TMDs),…
We analyze second-harmonic generation (SHG) at a thin effectively quadratic nonlinear interface between two linear optical media. We predict multistability of SHG for both plane and localized waves, and also describe two-color localized…
Described experimental conditions, reproducibility and optimization for the nonlinear optical effects (SHG, THG) for the diagnostic of functionalization of vertically aligned mesoporous silica thin films activated by silver and copper ions.…
Parametric oscillation is a fundamental concept that underlies nonlinear wave-matter interactions, leading to generation or amplification of new frequency components. Using a temporal modulation generated by the heterodyne interference of a…
The response functions of a material characterize its behavior under external stimuli, such as electromagnetic radiation. Such responses may grow linearly with the amplitude of the incident radiation, as is the case of absorption, or may be…
In this paper, the detection of a small reflector in a randomly heterogenous medium using second-harmonic generation is investigated. The medium is illuminated by a time-harmonic plane wave at frequency omega. It is assumed that the…
High complexity, dense integrated nanophotonic circuits possessing strong nonlinearities are desirable for a breadth of applications in classical and quantum optics. In this work, we study natural phase matching via modal engineering in…
Metallic nanostructures exhibit strong nonlinear-optical response at surface plasmon resonances, where the light-matter coupling efficiency is enhanced. An active modulation of this response can be realized by means of an external magnetic…
A first-principles study of the birefringence and the frequency dependent second harmonic generation (SHG) coefficients of the ternary pnictide semiconductors with formula ABC$_2$ (A = Zn, Cd; B = Si, Ge; C = As, P) with the chalcopyrite…
The solid-state harmonic generation (SSHG) derives from photocurrent coherence. The crystal symmetry, including point-group symmetry and time-reversal symmetry, constrains the amplitude and phase of the photocurrent, thus manipulates the…
Optical-field sampling using second-harmonic generation (SHG) from strong-field ionization enables ultrabroadband terahertz detection, but the microscopic origin of the SHG signal and its ultrabroadband response have been unclear. Here we…
Although massless Dirac fermions in graphene constitute a centrosymmetric medium for in-plane excitations, their second-order nonlinear optical response is nonzero if the effects of spatial dispersion are taken into account. Here we present…
Second harmonic generation (SHG) with a material of large transparency is an attractive way of generating coherent light sources at exotic wavelength range such as VUV, UV and visible light. It is of critical importance to improve nonlinear…
Spectroscopy of the centrosymmetric magnetic semiconductors EuTe and EuSe reveals spin-induced optical second harmonic generation (SHG) in the band gap vicinity at 2.1-2.4eV. The magnetic field and temperature dependence demonstrates that…
We study the dynamical response function relevant for two-dimensional coherent nonlinear optical spectroscopy of the antiferromagnetic frustrated $J_{1}$-$J_{3}$ Heisenberg model on the square lattice within its long-range ordered,…
LMTO calculations are presented for the frequency dependent second harmonic generation (SHG) in the polytypes 2H, 4H, 6H, 15R and 3C of SiC. All independent tensor components are calculated. The spectral features and the ratios of the 333…
Ferroelectric nematic liquid crystals exhibit unique non-linear optical properties, with the potential to become transformative materials for photonic applications. A promising direction relies on the fabrication of tailored polar…