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Related papers: Doppler-free Fourier transform spectroscopy

200 papers

We report a photonic microwave and RF fractional Hilbert transformer based on an integrated Kerr micro-comb source. The micro-comb source has a free spectral range (FSR) of 50GHz, generating a large number of comb lines that serve as a…

Dual-comb interferometry utilizes two optical frequency combs to map the optical field's spectrum to a radio-frequency signal without using moving parts, allowing improved speed and accuracy. However, the method is compounded by the…

Mid-infrared microscopy is an important tool for biological analyses, allowing a direct probe of molecular bonds in their low energy landscape. In addition to the label-free extraction of spectroscopic information, the application of…

We have developed a hyperspectral imaging scheme that involves a combination of dual-comb spectroscopy and Hadamard-transform-based single-pixel imaging. The scheme enables us to obtain 12,000 hyperspectral images of amplitude and phase at…

The common approach for producing Rydberg atoms in warm vapor cells is with lasers arranged in a counter-propagating, collinear configuration. Doppler effects in these configurations reduce the efficiency of excitation to the Rydberg state…

We present the development and performance of a Fourier transformation (FT) based Raman spectrometer working with visible laser (532 nm) excitation. It is generally thought that FT-Raman spectrometers are not viable in the visible range…

We study the two-photon laser excitation to the 5D$_{5/2}$ energy level of $^{85}$Rb atoms contained in the interstices of a porous material made from sintered ground glass with typical pore dimensions in the 10 - 100 $\mu$m range. The…

Atomic Physics · Physics 2017-10-18 Lucía Amy , Lorenzo Lenci , Santiago Villalba , Horacio Failache , Arturo Lezama

We present a novel approach to cavity ring-down spectroscopy utilizing an optical frequency comb as the direct probe of the Fabry-Perot cavity, coupled with a time-resolved Fourier transform spectrometer for parallel retrieval of ring-down…

Precision laser spectroscopy in the extreme ultraviolet of the 1S-2S two-photon transition in singly-ionized helium is a promising route for tests of fundamental physics. We demonstrate laser excitation of this transition in an atomic beam…

Ultrabroadband electro-optic sampling with few-cycle optical pulses is known to be an extremely sensitive technique to detect electric field amplitudes. By combining this method with dual-comb spectroscopy and with a new class of ultrafast…

We have carried out dual-comb spectroscopy and observed in a simultaneous acquisition a 140-THz-wide spectrum from 1.0 to 1.9 {\mu}m using two fiber-based frequency combs phase-locked to each other. This ultra-broad wavelength bandwidth is…

Rapid characterization of optical and vibrational spectra with high resolution can identify species in cluttered environments and is important for assays and early alerts. In this regard, dual-comb spectroscopy has emerged as a powerful…

Optics · Physics 2016-12-21 Myoung-Gyun Suh , Qi-Fan Yang , Ki Youl Yang , Xu Yi , Kerry Vahala

In this paper we show that the discrete Fourier transform can be performed by scattering a coherent particle or laser beam off a two-dimensional potential that has the shape of rings or peaks. After encoding the initial vector into the…

Mesoscale and Nanoscale Physics · Physics 2016-08-31 Michael N. Leuenberger , Daniel Loss , Michael E. Flatte , D. D. Awschalom

Optical-optical double-resonance (OODR) spectroscopy using a narrow-linewidth pump and a frequency comb probe has previously been used to measure and assign sub-Doppler transitions in the 3${\nu}$${_3}$ ${\Leftarrow}$ ${\nu}$${_3}$ spectral…

Chemical Physics · Physics 2025-12-08 Kevin K. Lehmann , Isak Silander , Adrian Hjältén , Michael Rey , Aleksandra Foltynowicz

Nonlinear optical effects can be enhanced in tapered optical fibers with diameters less than the wavelength of the propagating light. Here we report on the observation of two-photon absorption using tapered fibers in rubidium vapor at power…

Quantum Physics · Physics 2010-10-22 S. M. Hendrickson , M. M. Lai , T. B. Pittman , J. D. Franson

Two frequency combs can be used to measure the full complex response of a sample in a configuration which can be alternatively viewed as the equivalent of a dispersive Fourier transform spectrometer, infrared time domain spectrometer, or a…

Optics · Physics 2015-05-18 I. Coddington , W. C. Swann , N. R. Newbury

We demonstrate a simple system for dual-comb spectroscopy based on two inherently coherent optical frequency combs generated via seeded parametric down-conversion. The inbuilt coherence is established by making the two combs share a common…

Optics · Physics 2024-08-13 Mikhail Roiz , Santeri Larnimaa , Touko Uotila , Mikko Narhi , Markku Vainio

The phase information provided by the beat note between frequency combs and two continuous-wave lasers is used to extrapolate the phase evolution of comb modes found in a spectral region obtained via nonlinear broadening. This thereafter…

We have demonstrated Doppler-free intermodulated fluorescence spectroscopy of helium $2^3P-3^{1,3}D$ transitions in an rf discharged sealed-off cell using a compact laser system at 588 nm. An external cavity diode laser at 1176 nm was…

Atomic Physics · Physics 2015-06-11 Pei-Ling Luo , Jinmeng Hu , Yan Feng , Li-Bang Wang , Jow-Tsong Shy

A femtosecond frequency comb provides a vast number of equidistantly spaced narrow band laser modes that can be simultaneously tuned and frequency calibrated with 15 digits accuracy. Our Vernier spectrometer utilizes all of theses modes in…