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Because molecules can have their orientation locked when embedded into a solid rare-gas matrix, their hyperfine structure is strongly perturbed relative to the freely rotating molecule. The addition of an electric field further perturbs the…

Atomic Physics · Physics 2018-10-03 A. C. Vutha , M. Horbatsch , E. A. Hessels

In atoms spin-orbit coupling (SOC) cannot raise the angular momentum above a maximum value or lower it below a minimum. Here we show that this need not be the case in materials built from nanoscale structures including multi-nuclear…

Strongly Correlated Electrons · Physics 2017-03-15 A. L. Khosla , A. C. Jacko , J. Merino , B. J. Powell

In this article we present a concrete proposal for spin squeezing the ultracold ground state polar paramagnetic molecule OH, a system currently under fine control in the laboratory. In contrast to existing work, we consider a single,…

Quantum Physics · Physics 2016-01-20 M. Bhattacharya

Beams of neutral polar molecules in a low-field seeking quantum state can be slowed down using a Stark decelerator, and can subsequently be loaded and confined in electrostatic quadrupole traps. The efficiency of the trap loading process is…

We demonstrate loading of SrF molecules into an optical dipole trap (ODT) via in-trap $\Lambda$-cooling. We find that this cooling can be optimized by a proper choice of relative ODT and $\Lambda$ beam polarizations. In this optimized…

Atomic Physics · Physics 2021-10-27 Thomas K. Langin , Varun Jorapur , Yuqi Zhu , Qian Wang , David DeMille

In contrast to a "single particle table-top trap", an essential feature of a storage ring "trap" is that $10^{10}$ or more particles can have their spins aligned in a polarized beam. This is a nunber of polarized particles large enough for…

Accelerator Physics · Physics 2021-09-22 Richard M Talman

Artificial molecules containing just one or two electrons provide a powerful platform for studies of orbital and spin quantum dynamics in nanoscale devices. A well-known example of these dynamics is tunneling of electrons between two…

We demonstrate that ultracold symmetric top molecules loaded into an optical lattice can realize highly tunable and unconventional models of quantum magnetism, such as an XYZ Heisenberg spin model. We show that anisotropic dipole-dipole…

Quantum Gases · Physics 2015-03-20 M. L. Wall , K. Maeda , L. D. Carr

In weakly bound diatomic molecules, energy levels are closely spaced and thus more susceptible to mixing by magnetic fields than in the constituent atoms. We use this effect to control the strengths of forbidden optical transitions in…

Atomic Physics · Physics 2015-12-22 B. H. McGuyer , M. McDonald , G. Z. Iwata , W. Skomorowski , R. Moszynski , T. Zelevinsky

Dipolar interactions are ubiquitous in nature and rule the behavior of a broad range of systems spanning from energy transfer in biological systems to quantum magnetism. Here, we study magnetization-conserving dipolar induced spin-exchange…

Quantum Gases · Physics 2020-04-22 A. Patscheider , B. Zhu , L. Chomaz , D. Petter , S. Baier , A. M. Rey , F. Ferlaino , M. J. Mark

Formation of a magnetic hysteresis loop with respect to a bias voltage is investigated theoretically in a spin-valve device based on a single magnetic molecule. We consider a device consisting of two ferromagnetic electrodes bridged by a…

Mesoscale and Nanoscale Physics · Physics 2018-05-09 Anna Płomińska , Maciej Misiorny , Ireneusz Weymann

Strongly interacting spins underlie many intriguing phenomena and applications ranging from magnetism to quantum information processing. Interacting spins combined with motion display exotic spin transport phenomena, such as superfluidity…

We demonstrate long rotational coherence of individual polar molecules in the motional ground state of an optical trap. In the present, previously unexplored regime, the rotational eigenstates of molecules are dominantly quantized by…

We provide a theoretical framework for the electric field control of the electron spin in systems with diffusive electron motion. The approach is valid in the experimentally important case where both intrinsic and extrinsic spin-orbit…

Mesoscale and Nanoscale Physics · Physics 2009-09-10 R. Raimondi , P. Schwab

We consider a spin-orbit coupled system of particles in an external trap that is represented by a deformed harmonic oscillator potential. The spin-orbit interaction is a Rashba interaction that does not commute with the trapping potential…

Quantum Gases · Physics 2013-06-25 O. V. Marchukov , A. G. Volosniev , D. V. Fedorov , A. S. Jensen , N. T. Zinner

We describe a dynamic magneto-optical trap (MOT) suitable for the use with vacuum systems in which optical access is limited to a single window. This technique facilitates the long-standing desire of producing integrated atom chips, many of…

Atomic Physics · Physics 2016-11-28 Jo Rushton , Ritayan Roy , James Bateman , Matt Himsworth

Spin-flips are one of the limiting factors for spin-based information processing. We demonstrate a transport approach for determining the spin-flip rates of a self-assembled InAs double quantum dot occupied by a single electron. In such…

Mesoscale and Nanoscale Physics · Physics 2024-03-18 Olfa Dani , Robert Hussein , Johannes C. Bayer , Klaus Pierz , Sigmund Kohler , Rolf J. Haug

We consider cold collisions of OH molecules in the $^2\Pi_{3/2}$ grounds state, under the influnce of a magnetic field. We find that modest fields of several thousand gauss can act to suppress inelastic collisions of weak-field seeking…

Atomic Physics · Physics 2009-11-10 Christopher Ticknor , John L. Bohn

We present rigorous solution of problems of tunneling with dissipation and decoherence for a spin of an atom or a molecule in an isotropic solid matrix. Our approach is based upon switching to a rotating coordinate system coupled to the…

Materials Science · Physics 2009-11-07 E. M. Chudnovsky , X. Martinez-Hidalgo

Simultaneous two-dimensional trapping of neutral dipolar molecules in low- and high-field seeking states is analyzed. A trapping potential of the order of 20 mK can be produced for molecules like ND3 with time-dependent electric fields. The…

Chemical Physics · Physics 2009-11-10 T. Junglen , T. Rieger , S. A. Rangwala , P. W. H. Pinkse , G. Rempe