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We report the infrared dielectric properties of $\alpha$-quartz in the temperature range from $1.5\ \mathrm{K}$ to $200\ \mathrm{K}$. Using an infrared free-electron laser, far-infrared reflectivity spectra of a single crystal $y$-cut were…

Materials Science · Physics 2019-04-25 Christopher J. Winta , Martin Wolf , Alexander Paarmann

Recently, $\alpha$-$\textrm{RuCl}_3$ has attracted much attention as a possible material realization of the honeycomb Kitaev model, which may stabilize a quantum-spin-liquid state. Compared to extensive studies on its magnetic properties,…

In this paper we elucidate the optical response resulting from the interplay of charge distribution (ionicity) and Peierls instability (dimerization) in the neutral-ionic, ferroelectric phase transition of tetrathiafulvalene-chloranil…

Other Condensed Matter · Physics 2021-11-23 A. Girlando , M. Masino , A. Painelli , N. Drichko , M. Dressel , A. Brillante , R. G. Della Valle , E. Venuti

The interplay between electronic and lattice degrees of freedom is fundamental to charge density wave (CDW) formation, yet the microscopic origin often remains elusive. Here, we investigate the transient optical response of the…

Strongly Correlated Electrons · Physics 2026-01-27 Lei Wang , Mingwei Ma , Jiangxu Li , Liucheng Chen , Bingru Lu , Xiang Li , Feng Jin , Elbert E. M. Chia , Jianlin Luo , Rongyan Chen , Peitao Liu , Fang Hong , Xinbo Wang

Current phonon transport theory based on ground-state calculations has been successful in predicting thermal conductivity at room and medium temperatures but may misrepresent behavior at high temperatures. In this work, we predict the…

Materials Science · Physics 2023-12-20 Janak Tiwari , Tianli Feng

We report on the optical properties of undoped single crystal LaMnO_3, the parent compound of the colossal magneto-resistive manganites. Near-Normal incidence reflectance measurements are reported in the frequency range of 20-50,000 cm-1…

Strongly Correlated Electrons · Physics 2009-11-07 M. A. Quijada , J. R. Simpson , H. D. Drew , J. W. Lynn , L. Vasiliu-Doloc , Y. M. Mukovskii , S. G. Karabashev

The caged compound LaRu2Zn20 exhibits a structural transition at TS =150 K, whose driving mechanism remains elusive. We have investigated atomic dynamics by the measurements of specific heat C and inelastic X-ray scattering (IXS). The…

Strongly Correlated Electrons · Physics 2017-05-18 K. Wakiya , T. Onimaru , S. Tsutsui , K. T. Matsumoto , N. Nagasawa , A. Q. R. Baron , T. Hasegawa , N. Ogita , M. Udagawa , T. Takabatake

Critical behavior of the infrared reflectivity of RuSr_2GdCu_2O_8 ceramics is observed near the superconducting T_{SC} = 45 K and magnetic T_M = 133 K transition temperatures. The optical conductivity reveals the typical features of the…

Strongly Correlated Electrons · Physics 2009-10-31 A. V. Boris , P. Mandal , C. Bernhard , N. N. Kovaleva , K. Pucher , J. Hemberger , A. Loidl

We provide a detailed study of the reflectivity of multiferroic TbMnO_3 for wave numbers from 40 cm^{-1} to 1000 cm^{-1} and temperatures 5 K < T < 300 K. Excitations are studied for polarization directions E || a, the polarization where…

Strongly Correlated Electrons · Physics 2010-01-22 M. Schmidt , Ch. Kant , T. Rudolf , F. Mayr , A. A. Mukhin , A. M. Balbashov , J. Deisenhofer , A. Loidl

The thermal and electrical transport properties of single-crystalline LaBe$_{13}$ have been investigated by specific-heat ($C$) and electrical-resistivity ($\rho$) measurements. The specific-heat measurements in a wide temperature range…

Electric conductivity and structural details of the hole-doped polaron conductor La0.9Sr0.1FeO3 (LSF10) are reported. The conductivity of a single crystal shows an exponential increase with temperature with a maxi-mum of 100 S/cm at 700 K…

Strongly Correlated Electrons · Physics 2011-06-07 A. Braun , J. Richter , A. S. Harvey , A. Infortuna , A. Frei , E. Pomjakushina , Bongjin S. Mun , P. Holtappels , U. Vogt , K. Conder , L. J. Gauckler , T. Graule

We report results on the electrodynamic response of $TiOCl$, a low-dimensional spin-1/2 quantum magnet that shows a spin gap formation for T$<T_{c1}$= 67 $K$. The Fano-like shape of a few selected infrared active phonons suggests an…

Strongly Correlated Electrons · Physics 2009-11-10 G. Caimi , L. Degiorgi , N. N. Kovaleva , P. Lemmens , F. C. Chou

The infrared reflectivity of a $\rm La_{0.67}Ca_{0.33}MnO_3$ single crystal is studied over a broad range of temperatures (78-340 K), magnetic fields (0-16 T), and wavenumbers (20-9000 cm$^{-1}$). The optical conductivity gradually changes…

Strongly Correlated Electrons · Physics 2019-08-17 A. V. Boris , N. N. Kovaleva , A. V. Bazhenov , P. J. M. van Bentum , Th. Rasing , S-W. Cheong , A. V. Samoilov , N. -C. Yeh

High-frequency dielectric studies of Bi_0.85Nd_0.15FeO_3 ceramics performed betweeen 100 and 900 K reveal hardening of most polar phonons on cooling below antiferroelectric phase transition, which occurs near 600 K. Moreover, a strong THz…

Materials Science · Physics 2011-10-18 V. Goian , S. Kamba , S. Greicius , D. Nuzhnyy , S. Karimi , I. M. Reaney

A maximum superconductive transition temperature $T_\textrm{C}$ = 203.5 K has recently been reported for a sample of the binary compound tri-hydrogen sulfide (H$_\textrm{3}$S) prepared at high pressure and with room temperature annealing.…

Superconductivity · Physics 2017-03-14 Dale R. Harshman , Anthony T. Fiory

We use time-domain terahertz spectroscopy to measure the low energy conductivity and magnons in RuCl$_3$ under external magnetic field. At zero field, an oscillation with a frequency of 0.62 THz is clearly observed in time-domain spectrum…

Strongly Correlated Electrons · Physics 2018-09-19 L. Y. Shi , Y. Q. Liu , T. Lin , M. Y. Zhang , S. J. Zhang , L. Wang , Y. G. Shi , T. Dong , N. L. Wang

Temperature-dependent FAR-infrared reflectivity spectra of partially ordered magnetodielectric La2CoMnO6 is presented, from room temperature up to 675 K. A clear first-ordered structural phase transition (SPT) from a monoclinic structure…

Materials Science · Physics 2018-02-22 R. X. Silva , A. Nonato , R. L. Moreira , R. M. Almeida , C. W. A. Paschoal

Optical properties of single-crystal monoclinic CuO in the range 70 - 6000 \cm were studied at temperatures from 7 to 300 K. Normal reflection spectra were obtained from the (001) and (010) crystal faces thus giving for the first time…

Strongly Correlated Electrons · Physics 2009-10-31 A. B. Kuz'menko , D. van der Marel , P. J. M. van Bentum , E. A. Tishchenko , C. Presura , A. A. Bush

Terahertz and far-infrared electric and magnetic responses of hexagonal piezomagnetic YMnO3 single crystals are investigated. Antiferromagnetic resonance is observed in the spectra of magnetic permeability mu_a [H(omega) oriented within the…

Materials Science · Physics 2012-02-13 C. Kadlec , V. Goian , K. Z. Rushchanskii , P. Kuzel , M. Lezaic , K. Kohn , R. V. Pisarev , S. Kamba

Recent experiments on K$_3$C$_{60}$ and layered copper-oxide materials have reported substantial changes in the optical response following application of an intense THz pulse. These data have been interpreted as the stimulation of a…

Mesoscale and Nanoscale Physics · Physics 2019-01-02 Giuliano Chiriacò , Andrew J. Millis , Igor L. Aleiner