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The bursting of bubbles at an air/liquid interface is a familiar occurrence important to foam stability, cell cultures in bioreactors and mass transfer between the sea and atmosphere. Here we document the hitherto unreported formation and…

Droplet formation in oiling-out crystallization has important implication for separation and purification of pharmaceutical active ingredients by using an antisolvent. In this work, we report the crystallization processes of oiling-out…

Soft Condensed Matter · Physics 2020-09-14 Xuehua Zhang , Zixiang Wei , Howon Choi , Hao Hao , Huaiyu Yang

Biphasic chemical reactions compartmentalized in small droplets offer advantages, such as streamlined procedures for chemical analysis, enhanced chemical reaction efficiency and high specificity of conversion. In this work, we…

Soft Condensed Matter · Physics 2020-07-10 Zhengxin Li , Akihito Kiyama , Hongbo Zeng , Detlef Lohse , Xuehua Zhang

An aqueous suspension of silica nanoparticles or nanofluid can alter the wettability of surfaces, specifically by making them hydrophilic and oil-repellent under water. Wettability alteration by nanofluids have important technological…

Applied Physics · Physics 2021-08-13 Shidong Li , Anqi Sng , Dan Daniel , Hon Chung Lau , Ole Torsæter , Ludger P. Stubbs

Solvent exchange is a process involving mixing between a good solvent with dissolved solute and a poor solvent. The process creates local oversaturation which causes the nucleation of minute solute droplets. Such ternary systems on a…

Fluid Dynamics · Physics 2022-06-07 You-An Lee , Chao Sun , Sander G. Huisman , Detlef Lohse

Classical hydrodynamic models predict that infinite work is required to move a three-phase contact line, defined here as the line where a liquid/vapor interface intersects a solid surface. Assuming a slip boundary condition, in which the…

Droplet-based microfluidics has emerged as a powerful technology for the miniaturization and automation of biochemical assays. The replacement of surfactants by nanoparticles as interfacial stabilizers has gained increasing interest.…

Soft Condensed Matter · Physics 2019-06-21 Laura Andreina Chacon Orellana , Jean-Christophe Baret

Droplet-based interphase synthesis provides means to produce nanoparticles with low polydispersity by controlling mass transport through droplet dynamics. An experimentally validated model, based on coupled computational fluid dynamics with…

Fluid Dynamics · Physics 2023-04-17 Vivekananda Bal , Rajdip Bandyopadhyaya

We introduce a model of chemically active particles of a multi-component fluid that can change their interactions with other particles depending on their state. Since such switching of interactions can only be maintained by the input of…

Soft Condensed Matter · Physics 2019-05-01 Dino Osmanovic , Yitzhak Rabin

Jumping of coalescing condensate droplets from superhydrophobic surfaces is an interesting phenomenon which yields marked heat transfer enhancement over the more explored gravity-driven droplet removal mode in surface condensation, a phase…

Nanodroplets on chemically structured substrates move under the action of disjoining pressure induced forces. A detailed analysis of them shows that even in the absence of long-ranged lateral variations of the effective interface potential,…

Soft Condensed Matter · Physics 2009-11-13 A. Moosavi , M. Rauscher , S. Dietrich

We present three-dimensional numerical simulations, employing the well-established lattice Boltzmann method, and investigate similarities and differences between surfactants and nanoparticles as additives at a fluid-fluid interface. We…

Soft Condensed Matter · Physics 2012-07-26 Stefan Frijters , Florian Günther , Jens Harting

The compartmentalization of chemical reactions within droplets has advantages in low costs, reduced consumption of reagents and increased throughput. Reactions in small droplets have also been shown to greatly accelerate the rate of many…

Soft Condensed Matter · Physics 2020-07-27 Brendan P. Dyett , Xuehua Zhang

The surface impact and collisions of particle-laden nanodrops are studied using molecular dynamics computer simulations. The drops are composed of Lennard- Jones dimers and the particles are rigid spherical sections of a cubic lattice, with…

Soft Condensed Matter · Physics 2015-09-02 Joel Koplik

The impact of nanometer sized drops on solid surfaces is studied using molecular dynamics simulations. Equilibrated floating drops consisting of short chains of Lennard-Jones liquids with adjustable volatility are directed normally onto an…

Soft Condensed Matter · Physics 2015-06-11 Joel Koplik , Rui Zhang

In this paper we study the formation of nanodrops on curved surfaces (both convex and concave) by means of molecular dynamics simulations, where the particles interact via a Lennard-Jones potential. We find that the contact angle is not…

Fluid Dynamics · Physics 2017-07-14 Shantanu Maheshwari , Martin van der Hoef , Detlef Lohse

Microdrop impact and spreading phenomena are explored as an interface formation process using a recently developed computational framework. The accuracy of the results obtained from this framework for the simulation of high deformation…

Fluid Dynamics · Physics 2015-06-04 J. E. Sprittles , Y. D. Shikhmurzaev

An evaporating droplet is a dynamic system in which flow is spontaneously generated to minimize the surface energy, dragging particles to the borders and ultimately resulting in the so-called "coffee-stain effect". The situation becomes…

Fluid Dynamics · Physics 2015-11-24 Alvaro Marin , Robert Liepelt , Massimiliano Rossi , Christian J. Kähler

Preparation of nanoemulsions of triglyceride oils in water usually requires high mechanical energy and sophisticated equipment. Recently, we showed that alpha-to-beta (viz. gel-to-crystal) phase transition, observed with most lipid…

Soft Condensed Matter · Physics 2021-07-07 Diana Cholakova , Desislava Glushkova , Slavka Tcholakova , Nikolai Denkov

The occurrence of concentration and temperature gradients in saline microdroplets evaporating directly in air makes them unsuitable for nucleation studies where homogeneous composition is required. This can be addressed by immersing the…

Materials Science · Physics 2021-11-24 Ruel Cedeno , Romain Grossier , Nadine Candoni , Adrian Flood , Stéphane Veesler