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This work presents a detailed analysis of the photothermionic-photovoltaic hybrid solar device. The electrons in this hybrid device gain energy from both the solar photons and thermophotons generated within the device, and hence the device…

Applied Physics · Physics 2022-09-23 Ehsanur Rahman , Alireza Nojeh

Miniaturized photodetectors are becoming increasingly sought-after components for a range of next generation technologies, such as autonomous vehicles, integrated wearable devices, or gadgets embedded in the Internet of Things. A major…

Carbon materials are excellent candidates for photovoltaic solar cells: they are Earth-abundant, possess high optical absorption, and superior thermal and photostability. Here we report on solar cells with active layers made solely of…

Defects trap photocarriers and hinder solar water splitting. The nanoscale photocarrier transport, trapping, and recombination mechanisms are usually inferred from ensemble-averaged measurements and remain elusive. Because an individual…

In this work, using a hybrid density functional theory (DFT) based calculation, we propose a new two-dimensional (2D) B-C-N material, $g-B_{3}C_{2}N_{3}$, with the promising prospect of metal-free photocatalysis. A comprehensive…

Materials Science · Physics 2022-07-14 Sreejani Karmakar , Souren Adhikary , Sudipta Dutta

Perovskite photoelectrodes are being extensively studied in search for photocatalytic materials that can produce hydrogen through water splitting. The solar-to-hydrogen efficiency of these materials is critically dependent on the…

Applied Physics · Physics 2019-06-26 Yihuang Xiong , Ismaila Dabo

Multifunctional three-dimensional (3-D) nano-architectures, integrating all device components within tens of nanometers, offer great promise for next generation electrical energy storage applications, but have remained challenging to…

Chemical Physics · Physics 2017-06-08 Jörg G. Werner , Gabriel G. Rodríguez-Calero , Héctor D. Abruña , Ulrich Wiesner

Graphene like 2D materials have attracted tremendous attention in the field of photocatalytic water splitting. Indium Selenide (InSe) is one such potential material. Here, we report the effect of Tellurium on InSe monolayer for the…

Materials Science · Physics 2016-10-04 M. R. Ashwin Kishore , P. Ravindran

We report the results of density functional theory (DFT) based calculations on monolayer and bilayer green phosphorene and their heterostructures with MoSe2. Both monolayer and bilayer green phosphorene are direct band gap semiconductors…

Materials Science · Physics 2018-11-26 Sumandeep Kaur , Ashok Kumar , Sunita Srivastava , K. Tankeshwar , Ravindra Pandey

Regio-regular poly(3-hexylthiophene-2,5-diyl) (rr-P3HT), the work-horse of organic photovoltaics, has been recently exploited in bulk heterojunction (BHJ) configuration with phenyl-C61-butyric acid methyl ester (PCBM) for solution-processed…

Indium phosphide and derived compound semiconductors are materials often involved in high-efficiency solar water splitting due to their versatile opto-electronic properties. Surface corrosion, however, typically deteriorates the performance…

Chemical Physics · Physics 2022-11-16 Mario Löw , Margot Guidat , Jongmin Kim , Matthias M. May

The photocatalytic splitting of water into molecular hydrogen and molecular oxygen with sunlight is the dream reaction for solar energy conversion. Since decades, transition-metal-oxide semiconductors and supramolecular organometallic…

Chemical Physics · Physics 2018-07-10 Wolfgang Domcke , Johannes Ehrmaier , Andrzej L. Sobolewski

Electrochemical water splitting technology for producing "green hydrogen" is important for the global mission of carbon neutrality. Electrocatalysts with decent performance at high current densities play a central role in the industrial…

Chemical Physics · Physics 2022-02-16 Yuting Luo , Zhiyuan Zhang , Manish Chhowalla , Bilu Liu

Narrow-bandgap III-V semiconductor nanowires (NWs) with a suitable band structure and strong light-trapping ability are ideal for high-efficiency low-cost solar water-splitting systems. However, due to their nanoscale dimension, they suffer…

Titanium dioxide (TiO$_2$) plays a central role in the study of artificial photosynthesis, owing to its ability to perform photocatalytic water splitting. Despite over four decades of intense research efforts in this area, there is still…

Materials Science · Physics 2016-07-28 Christopher E. Patrick , Feliciano Giustino

We report the development of graphite-based solar cells using a simple method and low cost materials. Suspension of graphite powder in mineral water was simply dropped onto the surface of fluorine-doped tin oxide glass (FTO) to form a thick…

A well-established procedure for the photoelectrochemical (PEC) splitting of water relies on using porous electrodes of WO3 sensitized with BiVO4 as a visible scavenger photoanode semiconductor. In this work, we propose an evolved…

The active layer microstructure of organic solar cells is critical to efficiency. By studying the photovoltaic properties of organic solar cell's microstructure, it is possible to increase the efficiency of the solar cell. A graph-based…

Neural and Evolutionary Computing · Computer Science 2019-10-29 Caine Ardayfio

Successful synthesis of the nitrogenated holey two-dimensional structures C2N (Nat. Commun. 2015, 6, 6486) using simply wet-chemical reaction offer a cost-effective way to generate other 2D materials with novel optical and electronic…

Materials Science · Physics 2015-06-17 Ruiqi Zhang , Jinlong Yang

Converting solar energy into chemical energy by splitting water is a promising means to generate a sustainable and renewable solution without detrimental environmental impact. The two-dimensional semiconductors serve as potential catalysts…

Mesoscale and Nanoscale Physics · Physics 2019-09-18 Srilatha Arra , Rohit Babar , Mukul Kabir