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The Green-Kubo theory of thermal transport has long be considered incompatible with modern simulation methods based on electronic-structure theory, because it is based on such concepts as energy density and current, which are ill-defined at…

Statistical Mechanics · Physics 2018-08-20 Stefano Baroni , Riccardo Bertossa , Loris Ercole , Federico Grasselli , Aris Marcolongo

Transport coefficients, such as the diffusion coefficient and shear viscosity, are important material properties that are calculated in computer simulations. In this study, the criterion for the best estimation of viscosity, as an example…

Computational Physics · Physics 2023-06-05 Xin Liu , Xuhong Guo , Qi Liao

The thermal conductivity of classical multi-component fluids is seemingly affected by the intrinsic arbitrariness in the definition of the atomic energies and it is ill-conditioned numerically, when evaluated from the Green-Kubo theory of…

Statistical Mechanics · Physics 2019-09-30 Riccardo Bertossa , Federico Grasselli , Loris Ercole , Stefano Baroni

Molecular dynamics (MD) simulations are used to calculate transport coefficients in a two-component plasma interacting through a repulsive Coulomb potential. The thermal conductivity, electrical conductivity, electrothermal coefficient,…

Plasma Physics · Physics 2025-11-14 Briggs Damman , Jarett LeVan , Scott Baalrud

Quantum simulation methods based on density-functional theory are currently deemed unfit to cope with atomic heat transport within the Green-Kubo formalism, because quantum-mechanical energy densities and currents are inherently ill-defined…

Materials Science · Physics 2016-01-20 Aris Marcolongo , Paolo Umari , Stefano Baroni

We present a method, based on the classical Green-Kubo theory of linear response, to compute the heat conductivity of extended systems, leveraging energy-density, rather than energy-current, fluctuations, thus avoiding the need to devise an…

Materials Science · Physics 2024-02-01 Enrico Drigo , Maria Grazia Izzo , Stefano Baroni

The transport coefficient of shear viscosity is studied for a hadron matter through microscopic transport model, the Ultra--relativistic Quantum Molecular Dynamics (UrQMD), using the Green--Kubo formulas. Molecular--dynamical simulations…

Nuclear Theory · Physics 2009-11-10 Azwinndini Muronga

Equilibrium molecular dynamics simulations are used to calculate the thermal conductivity of the one component plasma (OCP) via the Green-Kubo formalism over a broad range of Coulomb coupling strength, $0.1\le\Gamma\le180$. These…

Plasma Physics · Physics 2019-10-30 Brett Scheiner , Scott D. Baalrud

We herein present a first-principles formulation of the Green-Kubo method that allows the accurate assessment of the non-radiative thermal conductivity of solid semiconductors and insulators in equilibrium ab initio molecular dynamics…

Materials Science · Physics 2017-05-03 Christian Carbogno , Rampi Ramprasad , Matthias Scheffler

Under many conditions, macroscopic grains flow like a fluid; kinetic theory pred icts continuum equations of motion for this granular fluid. In order to test the theory, we perform event driven molecular simulations of a two-dimensional gas…

Statistical Mechanics · Physics 2009-10-31 C. Bizon , M. D. Shattuck , J. B. Swift , Harry L. Swinney

Atomistic simulations of heat transport in complex materials are costly and hard to converge. This has led to the development of several noise-reduction techniques applicable to equilibrium molecular-dynamics (MD) simulations. We analyze…

Materials Science · Physics 2025-11-19 Sandro Wieser , YuJie Cen , Georg K. H. Madsen , Jesús Carrete

The calculation of thermal conductivity in insulating solids at temperatures below the Debye temperature is problematic, due to the breakdown of classical and semi-classical approaches. In this work, we present a fully quantum methodology…

Statistical Mechanics · Physics 2026-02-19 Vladislav Efremkin , Stefano Mossa , Jean-Louis Barrat , Markus Holzmann

Thermal conductivity of hadron matter is studied using a microscopic transport model, which will be used to simulate ultra-relativistic heavy ion collisions at different energy densities, namely the Ultra-relativistic Quantum Molecular…

Nuclear Theory · Physics 2016-04-27 T. E Nemakhavhani , A. Muronga

Equilibrium molecular dynamics simulations, in combination with the Green-Kubo (GK) method, have been extensively used to compute the thermal conductivity of liquids. However, the GK method relies on an ambiguous definition of the…

Computational Physics · Physics 2020-09-30 Bingqing Cheng , Daan Frenkel

Ab initio Green-Kubo (aiGK) simulations of heat transport in solids allow for assessing lattice thermal conductivity in anharmonic or complex materials from first principles. In this work, we present a detailed account of their practical…

Materials Science · Physics 2023-06-14 Florian Knoop , Matthias Scheffler , Christian Carbogno

Molecular dynamics simulations play an important role in studying heat transport in complex materials. The lattice thermal conductivity can be computed either using the Green-Kubo formula in equilibrium MD (EMD) simulations or using…

Computational Physics · Physics 2018-05-02 Haikuan Dong , Zheyong Fan , Libin Shi , Ari Harju , Tapio Ala-Nisilla

Using Kubo's linear response theory, we derive expressions for the frequency-dependent electrical conductivity (Kubo-Greenwood formula), thermopower, and thermal conductivity in a strongly correlated electron system. These are evaluated…

Plasma Physics · Physics 2012-05-04 Bastian Holst , Martin French , Ronald Redmer

The purpose of this study is to provide a reproducible framework in the use of the Green-Kubo formalism to extract transport coefficients. More specifically, in the case of shear viscosity, we investigate the limitations and technical…

Nuclear Theory · Physics 2018-07-04 J. -B. Rose , J. M. Torres-Rincon , D. Oliinychenko , A. Schäfer , H. Petersen

The vast amount of computational studies on electrical conduction in solid-state electrolytes is not mirrored by comparable efforts addressing thermal conduction, which has been scarcely investigated despite its relevance to thermal…

Materials Science · Physics 2024-06-18 Davide Tisi , Federico Grasselli , Lorenzo Gigli , Michele Ceriotti

The Green-Kubo (GK) method is a rigorous framework for heat transport simulations in materials. However, it requires an accurate description of the potential-energy surface and carefully converged statistics. Machine-learning potentials can…

Materials Science · Physics 2023-10-12 Marcel F. Langer , Florian Knoop , Christian Carbogno , Matthias Scheffler , Matthias Rupp
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