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Using data obtained from first-principles calculations, we show that the position of the morphotropic phase boundary (MPB) and transition temperature at MPB in ferroelectric perovskite solutions can be predicted with quantitative accuracy…

Materials Science · Physics 2009-11-11 Ilya Grinberg , Matthew R. Suchomel , P. K. Davies , Andrew M. Rappe

A key challenge for the practical application of metal halide perovskites (MHPs) is the instability of the desired perovskite phase relative to the optically non-active $\delta$ phase. To determine the phase stability, we previously…

Three first order magnetic phase transitions (FOMT) have been detected at TCPr, TNinter and TCinter over the temperature range from 5 K to 340 K at fields up to 9 T in PrMn1.4Fe0.6Ge2, and the magnetocaloric effect (MCE) around these…

Materials Science · Physics 2008-09-01 R. Zeng , J. L Wang , L. Lu , W. X. Li , S. J. Campbell , S. X. Dou

Despite extensive research interests in perovskite oxides, low energy consumption, non-destructive and maneuverable methods for phase transition in perovskite oxides are still the under its exploration, and the underlying mechanisms remain…

Materials Science · Physics 2023-08-10 Cong Zhou , Jian Zhou

The thermopower and thermal conductivity of superconducting perovskite $MgCNi_3$ ($T_c \approx$ 8 K) have been studied. The thermopower is negative from room temperature to 10 K. Combining with the negative Hall coefficient reported…

Superconductivity · Physics 2009-11-07 S. Y. Li , W. Q. Mo , M. Yu , W. H. Zheng , C. H. Wang , Y. M. Xiong , R. Fan , H. S. Yang , B. M. Wu , L. Z. Cao , X. H. Chen

We describe magneto-, baro- and elastocaloric effects (MCEs, BCEs and eCEs) in materials which possess both discontinuous (first-order) and continuous (second-order) magnetic phase transitions. Our ab initio theory of the interacting…

Materials Science · Physics 2020-06-03 Eduardo Mendive-Tapia , Julie B. Staunton

We have studied the electrocaloric response of the archetypal antiferroelectric PbZrO3 as a function of voltage and temperature in the vicinity of its antiferroelectric-paraelectric phase transition. Large electrocaloric effects of opposite…

Piezoelectric PZT solid solutions were studied as a function of pressure and temperature. Moderate pressure is found to induce phase transitions to monoclinic phases (Cm,Cc) for Ti-rich PZT, which are the same ferroelectric phases…

Materials Science · Physics 2009-05-14 Jérôme Rouquette , Julien Haines , Véronique Bornand , Philippe Papet

The thermoelectric properties of halide perovskites $\mathrm{CsMI_3}$ (M=Sn and Pb) are investigated from a combination of first-principles calculations and semiclassical Boltzmann transport theory by considering both the electron and…

Materials Science · Physics 2016-05-31 San-Dong Guo , Jian-Li Wang

Antiferroelectrics have been recently sparking interest due to their potential use in energy storage and electrocaloric cooling. Their main distinctive feature is antiferroelectric switching, i.e. the possibility to induce a phase…

The phase diagram of a quantum paraelectric antiferromagnet EuTiO3 under an external electric field was calculated using Landau-Ginzburg-Devonshire theory. It was shown that the application of an external electric field E leads to the…

The perovskite crystal BaTiO3 is modeled using a first-principles based effective Hamiltonian and molecular dynamics simulations are performed to estimate the pyroelectric response. The electrocaloric temperature change, \DeltaT, is…

Materials Science · Physics 2012-08-30 S. P. Beckman , L. F. Wan , Jordan A. Barr , Takeshi Nishimatsu

A comparative study of the dielectric properties and electric polarization of multiferroics GdMn2O5 and Gd0.8Ce0.2Mn2O5 has been carried out in the temperature range from 5 up to 300 K. The polarization properties in the ferroelectric state…

Materials Science · Physics 2018-04-18 V. A. Sanina , B. Kh. Khannanov , E. I. Golovenchits , M. P. Shcheglov

Perovskite-type Ba0.9Sr0.1Ti0.9Sn0.1O3(BSTSn) ceramic was synthesized by the sol gel method. The P E hysteresis loops were recorded at different temperatures to investigate the ferroelectric and energy storage properties of BSTSn ceramic.…

Materials Science · Physics 2023-06-13 S. Khardazi , H. Zaitouni , S. Belkhadir , D. Mezzane , M. Amjoud , Y. Gagou , B. Asbani , I. Lukyanchuk , S. Terenchuk

The ground state properties of the pure perovskite compounds PrMnO$_3$ and NdMnO$_3$ were investigated by magnetization, magnetic AC susceptibility and specific heat measurements. A strongly anisotropic behavior has been detected for…

Condensed Matter · Physics 2007-05-23 J. Hemberger , M. Brando , R. Wehn , V. Yu. Ivanov , A. A. Mukhin , A. M. Balbashov , A. Loidl

We have studied the temperature dependence of the photoemission spectra of Pr$_{1-x}$Ca$_x$MnO$_3$ (PCMO) with $x=0.25$, 0.3 and 0.5. For $x=0.3$ and 0.5, we observed a gap in the low-temperature CE-type charge-ordered (CO) phase and a…

Strongly Correlated Electrons · Physics 2009-11-13 K. Ebata , M. Hashimoto , K. Tanaka , A. Fujimori , Y. Tomioka , Y. Tokura

Crystal-field excitations, for example in transition-metal oxides where a rare-earth element is used as a spacer between the transition-metal-oxide tetrahedra and octahedra, are assumed to be extremely robust with respect to external…

Strongly Correlated Electrons · Physics 2021-10-12 Joel O'Brien , Guochu Deng , Dehong Yu , Xiaoxuan Ma , Zhenjie Feng , Wei Ren , Shixun Cao , Robert A. Robinson , Garry J. McIntyre , Clemens Ulrich

Pyro-current measurements have been widely used to study ferroelectric properties in multiferroic materials. However, determination of intrinsic polarization by this method is not straightforward because of leakage current and trapped…

Materials Science · Physics 2015-01-06 Chandan De , Somnath Ghara , A. Sundaresan

Organic-inorganic hybrid perovskite architecture could serve as a robust platform for materials design to realize functionalities beyond photovoltaic applications. We explore caloric effects in organometal halide perovskites, taking…

Materials Science · Physics 2016-04-21 Shi Liu , Ronald E. Cohen

Electrostatic dielectric capacitors are foundational to advance the electronics and electric power devices due to their ultrafast charging/discharging capability and high-power density. However, the low energy density limits the potential…

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