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In this thesis, we study the interplay of phase separation and wetting in multicomponent systems. For this purpose, we have examined the phase separation pattern of a binary mixture (AB) in presence of stationary spherical particles (C)…

Soft Condensed Matter · Physics 2020-05-05 Supriyo Ghosh

We examine the symmetry-breaking effect of fixed constellations of particles on the surface-directed spinodal decomposition of binary blends in the presence of particles whose surfaces have a preferential affinity for one of the components.…

Chemical Physics · Physics 2020-06-16 Supriyo Ghosh , Arnab Mukherjee , Raymundo Arroyave , Jack F. Douglas

The ordering of particles in the drying process of a colloidal suspension is crucial in determining the properties of the resulting film. For example, microscopic inhomogeneities can lead to the formation of cracks and defects that can…

Soft Condensed Matter · Physics 2021-10-04 Maarten Wouters , Othmane Aouane , Marcello Sega , Jens Harting

We present molecular dynamics (MD) results to discuss wetting kinetics in binary fluid mixtures ($A:B=50:50$) undergoing surface-directed spinodal decomposition (SDSD) on an amorphous wall. Our simulations show the formation of a wetting…

Soft Condensed Matter · Physics 2025-12-09 Syed Shuja Hasan Zaidi , Madhu Priya , Sanjay Puri , Prabhat K. Jaiswal

We present a new numerical model to simulate settling trajectories of discretized individual or a mixture of particles of different geometrical shapes in a quiescent fluid and their flow trajectories in a flowing fluid. Simulations unveiled…

Computational Physics · Physics 2020-06-26 Hakan Başağaoğlu , Sauro Succi , Danielle Wyrick , Justin Blount

We present results from the molecular dynamics (MD) simulation of surface-directed spinodal decomposition (SDSD) in binary fluid mixtures ($A+B$) with off-critical compositions. The aim is to elucidate the role of composition ratio in the…

Soft Condensed Matter · Physics 2024-08-19 Syed Shuja Hasan Zaidi , Saumya Suvarna , Madhu Priya , Sanjay Puri , Prabhat K. Jaiswal

A partially miscible binary liquid mixture, composed of A and B particles, is considered theoretically under conditions for which a stable A-rich liquid phase is in thermal equilibrium with the vapor phase. The B-rich liquid is metastable.…

Soft Condensed Matter · Physics 2021-04-28 Hyojeong Kim , Lothar Schimmele , S. Dietrich

The surface directed spinodal decomposition of a binary liquid confined inside cylindrical pore is investigated using molecular dynamics simulation. One component of the liquid wets the pore surface while the other remains neutral. A…

Soft Condensed Matter · Physics 2023-09-19 Daniya Davis , Bhaskar Sen Gupta

Soft particles suspended in fluids flowing through microchannels are often encountered in biological flows such as cells in vessels. They can deform under flow or when subject to mechanical stresses as they interact with themselves.…

Soft Condensed Matter · Physics 2021-01-19 Danilo P. F. Silva , Rodrigo C. V. Coelho , Margarida M. Telo da Gama , Nuno A. M. Araújo

The accumulation of self-propelled particles on repulsive barriers is a widely observed feature in active matter. Despite being implicated in a broad range of biological processes, from biofilm formation to cytoskeletal movement, wetting of…

Statistical Mechanics · Physics 2025-12-12 Noah Grodzinski , Michael E. Cates , Robert L. Jack

The surface curvature of membranes, interfaces, and substrates plays a crucial role in shaping the self-assembly of particles adsorbed on these surfaces. However, little is known about the interplay between particle anisotropy and surface…

Soft Condensed Matter · Physics 2025-10-30 Gautam Bordia , Thomas P. Russell , Ahmad K. Omar

We carried out three-dimensional simulations, with about 1.4 million particles, of phase segregation in a low density binary fluid mixture, described mesoscopically by energy and momentum conserving Boltzmann-Vlasov equations. Using a…

patt-sol · Physics 2008-02-03 S. Bastea , J. L. Lebowitz

The self-assembly of binary nanoparticle superlattices from colloidal mixtures is a promising method for the fabrication of complex colloidal co-crystal structures. However, binary mixtures often form amorphous or metastable phases instead…

Soft Condensed Matter · Physics 2022-05-11 R. Allen LaCour , Timothy C. Moore , Sharon C. Glotzer

A binary mixture of particles interacting with spherically-symmetric potentials leading to microsegregation is studied by theory and molecular dynamics (MD) simulations. We consider spherical particles with equal diameters and volume…

Soft Condensed Matter · Physics 2020-11-20 O. Patsahan , M. Litniewski , A. Ciach

We investigate the behavior of colloidal suspensions with different volume fractions confined between parallel walls under a range of steady shears. We model the particles using molecular dynamics (MD) with full hydrodynamic interactions…

Soft Condensed Matter · Physics 2014-09-18 Frances E. Mackay , Kyle Pastor , Mikko Karttunen , Colin Denniston

Colloidal particles with appropriate wetting properties can become very strongly trapped at an interface between two immiscible fluids. We have harnessed this phenomenon to create a new class of soft materials with intriguing and…

Soft Condensed Matter · Physics 2009-11-13 K. A. White , A. B. Schofield , B. P. Binks , P. S. Clegg

The electrostatic interaction between pairs of spherical or macroscopically long, parallel cylindrical colloids trapped at fluid interfaces is studied theoretically for the case of small inter-particle separations. Starting from the…

Soft Condensed Matter · Physics 2018-11-30 Arghya Majee , Markus Bier , S. Dietrich

The evolution of the microstructure due to spinodal decomposition in phase separated mixtures has a strong impact on the final material properties. In the late stage of coarsening, the system is characterized by the growth of a single…

Soft Condensed Matter · Physics 2021-12-09 Björn König , Olivier J. J. Ronsin , Jens Harting

Motivated by observations of heterogeneous domain structure on the surface of cells, we consider a minimal model to describe the dynamics of phase separation on the surface of a spherical particle. Finite-size effects on the curved particle…

Soft Condensed Matter · Physics 2016-07-13 Matthias C. Bott , Joseph M. Brader

We consider the phase separation of binary fluids in contact with a surface which is preferentially wetted by one of the components of the mixture. We review the results available for this problem and present new numerical results obtained…

Statistical Mechanics · Physics 2007-05-23 Sorin Bastea , Sanjay Puri , Joel L. Lebowitz
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