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We report plasma-enhanced atomic layer deposition (ALD) to prepare conformal nickel thin films and nanotubes by using nickelocene as a precursor, water as the oxidant agent and an in-cycle plasma enhanced reduction step with hydrogen. The…

Materials with designed properties arises in a synergy between theoretical and experimental approaches. In this study we explore the set of Archimedean lattices forming a guidance to its electronic properties and topological phases. Within…

Mesoscale and Nanoscale Physics · Physics 2019-09-23 F. Crasto de Lima , Gerson J. Ferreira , R. H. Miwa

It has been widely accepted that planar boron structures, composed of triangular and hexagonal motifs are the most stable two dimensional (2D) phases and likely precursors for boron nanostructures. Here we predict, based on ab initio…

Materials Science · Physics 2014-02-28 Xiang-Feng Zhou , Xiao Dong , Artem R. Oganov , Qiang Zhu , Yongjun Tian , Hui-Tian Wang

Motivated by a recent experiment that reported the successful synthesis of hexagonal (h) AlN [Tsipas et al. Appl. Phys. Lett. 103, 251605 (2013)] we investigate structural, electronic and vibrational properties of bulk, bilayer and…

Materials Science · Physics 2015-03-03 C. Bacaksiz , H. Sahin , H. D. Ozaydin , S. Horzum , R. T. Senger , F. M. Peeters

We have investigated through fully atomistic reactive molecular dynamics and DFT simulations, the mechanical properties and fracture dynamics of novamene, a new 3D carbon allotrope structure recently proposed. Our results showed that…

Materials Science · Physics 2018-04-20 Eliezer F. Oliveira , Pedro A. S. Autreto , Cristiano F. Woellner , Douglas S. Galvao

Although 2D solids and their vdW heterostructures have garnered much attention recently, their amorphous forms have been less explored. We present a detailed analysis of the structural, electronic, and thermal properties of 2D amorphous…

Materials Science · Physics 2023-05-16 Emel Gürbüz , Biplab Sanyal

Lattice-matched heterovalent alloys and superlattices have some unique physical properties. For example, their band gap can change by a large amount without significant change in their lattice constants, thus they have great potential for…

Materials Science · Physics 2013-09-30 Hui-Xiong Deng , Bing Huang , Jingbo Li , Shu-Shen Li , Su-Huai Wei

The existence of two novel hybrid two-dimensional (2D) monolayers, 2D B3C2P3 and 2D B2C4P2, has been predicted based on the density functional theory calculations. It has been shown that these materials possess structural and thermodynamic…

We have investigated the possibility of using aluminum functionalized silicene trilayers (ABC-Si$_4$Al$_2$) as an anode material for alkali metal ion batteries (AMIBs). First, we studied the thermodynamic stability of ABC-Si$_4$Al$_2$ using…

Materials Science · Physics 2022-12-23 Bruno Ipaves , João F. Justo , Lucy V. C. Assali

Recent work on atomic-precision dopant incorporation technologies has led to the creation of both boron and aluminum $\delta$-doped layers in silicon with densities above the solid solubility limit. We use density functional theory to…

Materials Science · Physics 2023-08-23 Quinn T. Campbell , Shashank Misra , Andrew D. Baczewski

We generalize the construction of time-reversal symmetry-breaking triple-component semimetals, transforming under the pseudospin-1 representation, to arbitrary (anti-)monopole charge $2 n$, with $n=1,2,3$ in the crystalline environment. The…

Mesoscale and Nanoscale Physics · Physics 2019-12-09 Snehasish Nandy , Sourav Manna , Dumitru Calugaru , Bitan Roy

The three-dimensional topological semimetals represent a new quantum state of matter. Distinct from the surface state in the topological insulators that exhibits linear dispersion in two-dimensional momentum plane, the three-dimensional…

The abundant bonding possibilities of Carbon stimulate the design of numerous carbon allotropes, promising the foundation for exploring structure-functionality relationships. Herein, utilizing the space bending strategy, we successfully…

Atomic Physics · Physics 2024-01-25 Linfeng Yu , Yi Zhang , Jianzhou Lin , Kexin Dong , Xiong Zheng , Zhenzhen Qin , Guangzhao Qin

The energy landscape of carbon is exceedingly complex, hosting diverse and important metastable phases, including diamond, fullerenes, nanotubes and graphene. Searching for structures, especially those with large unit cells, in this…

Materials Science · Physics 2018-11-14 Chaoyu He , Xizhi Shi , S. J. Clark , Jin Li , Chris J. Pickard , Tao Ouyang , Chunxiao Zhang , Chao Tang , Jianxin Zhong

Cadmium arsenide ($\rm Cd_3As_2$) is known for its inverted band structure and ultra-high electron mobility. It has been theoretically predicted and also confirmed by ARPES experiments to exhibit a 3D Dirac semimetal phase containing…

Mesoscale and Nanoscale Physics · Physics 2016-06-14 Shih-Ting Guo , R. Sankar , Yung-Yu Chien , Tay-Rong Chang , Horng-Tay Jeng , Guang-Yu Guo , F. C. Chou , Wei-Li Lee

A new set of lattice-models based on the hexagonal $\sqrt{N}\times\sqrt{N}$ super-cells of the well-known honeycomb lattice with single-hole defect (HL-D-1/2N) are proposed to realize the nontrivial isolated flat-bands. Through performing…

Materials Science · Physics 2022-08-15 Chaoyu He , Yujie Liao , Tao Ouyang , Huimin Zhang , Hongjun Xiang , Jianxin Zhong

Due to the flexibility of C and N atoms in forming different types of bonds, the prediction of new two-dimensional (2D) carbon nitrides is a hot topic in the field of carbon-based materials. Using first-principles calculations, we propose…

Materials Science · Physics 2024-01-09 Linyang Li , Jialei Li , Yawei Yu , Yuxuan Song , Jia Li , Xiaobiao Liu , François M. Peeters , Xin Chen , Guodong Liu

Electronic structures of carbides with the rocksalt structure were calculated by full potential electronic codes solving the Kohn-Sham equation. Bonding characters were analyzed by constructing tight-binding Hamiltonian based on…

Materials Science · Physics 2012-11-09 Wenxu Zhang , Zhida Song , Bin Peng , Wanli Zhang

In this paper, density functional theory calculations are used to explore the electronic and atomic reconstruction at interfaces between III-III/I-V oxides. In particular, at these interfaces, two dimensional electron gases (2DEGs) with…

Materials Science · Physics 2012-06-06 Valentino R. Cooper

The isolation of graphene and transition metal dichalcongenides has opened a veritable world to a great number of layered materials which can be exfoliated, manipulated, and stacked or combined at will. With continued explorations expanding…