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Related papers: Radio Frequency Magneto-Optical Trapping of CaF wi…

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Recent experiments have demonstrated direct cooling and trapping of diatomic and triatomic molecules in magneto-optical traps (MOTs). However, even the best molecular MOTs to date still have density $10^{-5}$ times smaller than in typical…

Atomic Physics · Physics 2023-04-19 Thomas K. Langin , David DeMille

We report magneto-optical trapping (MOT) of a polyatomic molecule, calcium monohydroxide (CaOH). The MOT contains $2.0(5)\times 10^4$ CaOH molecules at a peak density of $3.0(8)\times10^{6}$ cm$^{-3}$. CaOH molecules are further sub-Doppler…

We report the experimental realization of a conveyor-belt magneto-optical trap for calcium monofluoride (CaF) molecules. The obtained highly-compressed cloud has a mean radius of 64(5) $\mu$m and a peak number density of $3.6(5) \times…

Laser slowing of CaF molecules down to the capture velocity of a magneto-optical trap (MOT) for molecules is achieved. Starting from a two-stage buffer gas beam source, we apply frequency-broadened "white-light" slowing and observe…

A key method to produce trapped and laser-cooled molecules is the magneto-optical trap (MOT), which is conventionally created using light red-detuned from an optical transition. In this work, we report a MOT for CaF molecules created using…

Atomic Physics · Physics 2024-06-18 Samuel J. Li , Connor M. Holland , Yukai Lu , Lawrence W. Cheuk

Direct laser cooling and trapping of molecules to temperature below Doppler limit and density exceeding $10^8$ are challenging due to the sub-Doppler heating effects of molecular magneto-optical trap (MOT). In our previous paper [1], we…

Atomic Physics · Physics 2023-05-29 S. Xu , R. Li , Y. Zhai , Y. Xia , M. Siercke , S. Ospelkaus

We present the properties of a magneto-optical trap (MOT) of CaF molecules. We study the process of loading the MOT from a decelerated buffer-gas-cooled beam, and how best to slow this molecular beam in order to capture the most molecules.…

Atomic Physics · Physics 2017-12-06 H. J. Williams , S. Truppe , M. Hambach , L. Caldwell , N. J. Fitch , E. A. Hinds , B. E. Sauer , M. R. Tarbutt

Molecular magneto-optical traps (MOTs) typically capture orders of magnitude fewer particles than their atomic counterparts due in part to their significantly lower capture velocities. Here, we employ a Stochastic Schr\"odinger Equation…

Current dual-frequency magneto-optical traps for ultracold molecules are plagued by sub-Doppler heating effects, making them vastly inferior to standard atomic MOTs. Here we demonstrate theoretically that the sub-Doppler effects in such a…

Atomic Physics · Physics 2023-04-06 S. Xu , P. Kaebert , M. Stepanova , T. Poll , M. Siercke , S. Ospelkaus

We demonstrate with a RF-MOT the one dimensional, transverse magneto-optical compression of a cold beam of calcium monofluoride (CaF). By continually alternating the magnetic field direction and laser polarizations of the magneto-optical…

Calcium monofluoride (CaF) molecules are loaded into an optical dipole trap (ODT) and subsequently laser cooled within the trap. Starting with magneto-optical trapping, we sub-Doppler cool CaF and then load $150(30)$ CaF molecules into an…

We report optical trapping of laser-cooled molecules at sufficient density to observe molecule-molecule collisions for the first time in a bulk gas. SrF molecules from a red-detuned magneto-optical trap (MOT) are compressed and cooled in a…

Atomic Physics · Physics 2024-05-09 Varun Jorapur , Thomas K. Langin , Qian Wang , Geoffrey Zheng , David DeMille

Diatomic molecules are promising systems for quantum science applications due to their complex energy structures and strong dipole-dipole interactions. Achieving ultracold temperatures is essential for these applications, but the complexity…

Atomic Physics · Physics 2025-11-21 Dongkyu Lim , Eunmi Chae

We demonstrate a three-dimensional magneto-optical trap (MOT) of a metal hydride molecule, CaH. We are able to scatter $\sim$$10^{4}$ photons with vibrational loss covered up to vibrational quantum number $\nu=2$. This allows us to laser…

Atomic Physics · Physics 2025-12-30 Jinyu Dai , Benjamin Riley , Qi Sun , Debayan Mitra , Tanya Zelevinsky

We demonstrate rapid loading of a magneto-optical trap (MOT) of cadmium atoms from a pulsed cryogenic helium buffer gas beam, overcoming strong photoionization losses. Using the $ ^1S_0 \rightarrow{} ^1P_1 $ transition at 229 nm, we capture…

Direct laser cooling of molecules has reached a phase space density exceeding 10$^{-6}$ in optical traps, but with rather small molecular numbers. To progress towards quantum degeneracy, a mechanism is needed that combines sub-Doppler…

Atomic Physics · Physics 2023-05-24 Justin J. Burau , Parul Aggarwal , Kameron Mehling , Jun Ye

Magneto-optical trapping forces for molecules are far weaker than for alkali atoms because the photon scattering rate is reduced when there are multiple ground states, and because of optical pumping into dark states. The force is further…

Atomic Physics · Physics 2021-12-14 M. R. Tarbutt , T. C. Steimle

Calcium monofluoride (CaF) is magnetically slowed and trapped using optical pumping. Starting from a collisionally cooled slow beam, CaF with an initial velocity of ~ 30 m/s is slowed via magnetic forces as it enters a 800 mK deep magnetic…

Atomic Physics · Physics 2014-03-26 Hsin-I Lu , Ivan Kozyryev , Boerge Hemmerling , Julia Piskorski , John M. Doyle

We experimentally and theoretically study the continuous accumulation of cold atoms from a magneto-optical trap (MOT) into a finite depth trap, consisting in a magnetic quadrupole trap dressed by a radiofrequency (RF) field. Chromium atoms…

Magneto-optical traps are central to atomic and molecular quantum technologies and precision tests of fundamental physics, where both sensitivity and bandwidth scale strongly with atom number and loading rate. We demonstrate that employing…

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