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Previous studies have suggested a conundrum in the relaxation dynamics of polydisperse supercooled liquids. It has been shown that in two dimensions, the relative relaxation times of particles of different sizes become more similar as the…

Soft Condensed Matter · Physics 2025-03-06 Ilian Pihlajamaa , Lotte van Gessel , Corentin Laudicina , Luc van Burik , Liesbeth Janssen

We study Harmonic Soft Spheres as a model of thermal structural glasses in the limit of infinite dimensions. We show that cooling, compressing and shearing a glass lead to a Gardner transition and, hence, to a marginally stable amorphous…

Disordered Systems and Neural Networks · Physics 2018-05-02 Giulio Biroli , Pierfrancesco Urbani

Ice growth has attracted great attention for its capability of fabricating hierarchically porous microstructure. However, the formation of tilted lamellar microstructure during freezing needs to be reconsidered due to the limited control of…

Materials Science · Physics 2020-12-09 Tongxin Zhang , Lilin Wang , Zhijun Wang , Junjie Li , Jincheng Wang

We present a simple model for an associating liquid in which polymorphism and density anomaly are connected. Our model combines a two dimensional lattice gas with particles interacting through a soft core potential and orientational degrees…

Statistical Mechanics · Physics 2009-11-10 Vera B. Henriques , Marcia C Barbosa

We investigate the behavior of amorphous silicon under hydrostatic compression using molecular simulations. During compression, amorphous silicon undergoes a discontinuous nonequilibrium transition from a low-density to a high-density…

Soft Condensed Matter · Physics 2023-05-31 Jan Grießer , Gianpietro Moras , Lars Pastewka

All liquids are topologically disordered materials; however, the degree of disorder can vary as a result of internal fluctuations in structure and topology. These fluctuations depend on both the composition and temperature of the system.…

Statistical Mechanics · Physics 2018-08-15 Katelyn A. Kirchner , Seong H. Kim , John C. Mauro

All phase transitions can be categorised into two different types: continuous and discontinuous phase transitions. Discontinuous phase transitions are normally accompanied with significant structural changes, and nearly all of them have the…

Soft Condensed Matter · Physics 2024-02-20 Yusheng Lei , Ran Ni

Topological data analysis (TDA) is a new emerging and powerful tool to understand the medium range structure ordering of multi-scale data. This study investigates the density anomalies observed during cooling of liquid silica from…

Materials Science · Physics 2023-10-05 Andrea Tirelli , Kousuke Nakano

Pressure induced structural modifications in vitreous Ge$_{x}$Se$_{100-x}$ (where 10 $\leq$ x $\leq$ 25)are investigated using X-ray absorption spectroscopy (XAS) along with supplementary X-ray diffraction (XRD) experiments and ab initio…

Glasses derive their functional properties from complex relaxation dynamics that remain enigmatic under extreme conditions. While the temperature dependence of these relaxation processes is well-established, their behavior under…

Thermodynamic properties of liquid water as well as hexagonal (Ih) and cubic (Ic) ice are predicted based on density functional theory at the hybrid-functional level, rigorously taking into account quantum nuclear motion, anharmonic…

Materials Science · Physics 2025-10-06 Bingqing Cheng , Edgar A. Engel , Jörg Behler , Christoph Dellago , Michele Ceriotti

Heterogeneous ice growth exhibits a maximum in freezing rate arising from the competition between kinetics and the thermodynamic driving force between the solid and liquid states. Here, we use molecular dynamics simulations to elucidate the…

Soft Condensed Matter · Physics 2013-12-31 Razvan A. Nistor , Thomas E. Markland , B. J. Berne

Using computer simulations of an atomistic glass-forming liquid, we investigate the fluctuations of the overlap between a fluid configuration and a quenched reference system. We find that large fluctuations of the overlap develop as…

Statistical Mechanics · Physics 2015-05-29 Ludovic Berthier , Robert L. Jack

Using two dimensional simulations, we study the formation of structures with a high-density contrast by magnetohydrodynamic waves in regions in which the ratio of thermal to magnetic pressure is small. The initial state is a uniform…

Astrophysics · Physics 2009-11-11 S. Van Loo , S. A. E. G. Falle , T. W. Hartquist

The relaxation dynamics of glass-forming systems shows a multitude of features that are absent in normal liquids, such as non-exponential relaxation and a strong temperature-dependence of the relaxation time. Connecting these dynamic…

Disordered Systems and Neural Networks · Physics 2019-04-03 Zhen Wei Wu , Walter Kob , Wei-Hua Wang , Limei Xu

We propose and numerically implement a local probe of the static self-induced heterogeneity characterizing glass-forming liquids. The method relies on the equilibrium statistics of the overlap between pairs of configurations measured in…

Soft Condensed Matter · Physics 2022-05-23 Benjamin Guiselin , Gilles Tarjus , Ludovic Berthier

The dynamical glass transition is typically taken to be the temperature at which a glassy liquid is no longer able to equilibrate on experimental timescales. Consequently, the physical properties of these systems just above or below the…

Soft Condensed Matter · Physics 2017-03-08 Samuel S. Schoenholz , Ekin D. Cubuk , Efthimios Kaxiras , Andrea J. Liu

Wavy pattern of ice with a specific wavelength occurs during ice growth from a thin layer of undercooled water flowing down the surface of icicles or inclined plane. In the preceding paper [K. Ueno, Phys. Rev. E {\bf 68}, 021603 (2003)], we…

Materials Science · Physics 2009-11-10 K. Ueno

When an ensemble of particles interact hydrodynamically, they generically display large-scale transient structures such as swirls in sedimenting particles [1], or colloidal strings in sheared suspensions [2]. Understanding these…

Soft Condensed Matter · Physics 2013-01-24 Nicolas Desreumaux , Jean-Baptiste Caussin , Raphael Jeanneret , Eric Lauga , Denis Bartolo

Thermal motions in the 2D Lennard-Jones liquid near solidification are studied at equilibrium and under shear flow conditions. At the temperatures of the study, the liquid is significantly aggregated. On times of few to few tens of…

Mesoscale and Nanoscale Physics · Physics 2017-03-03 Alexander Z. Patashinski , Rafal Orlik , Mark A. Ratner
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