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We demonstrate optical detection of a broad spectrum of ferromagnetic excitations using nitrogen-vacancy (NV) centers in an ensemble of nanodiamonds. Our recently developed approach exploits a straightforward CW detection scheme using…

Nuclear magnetic resonance (NMR) and magnetic resonance imaging (MRI) are well-established techniques that provide valuable information in a diverse set of disciplines but are currently limited to macroscopic sample volumes. Here we…

We present high-resolution optically detected magnetic resonance (ODMR) spectroscopy on single nitrogen-vacancy (NV) center spins in diamond at and around zero magnetic field. The experimentally observed transitions depend sensitively on…

Mesoscale and Nanoscale Physics · Physics 2019-11-22 Johannes Kölbl , Mark Kasperczyk , Beat Bürgler , Arne Barfuss , Patrick Maletinsky

Nuclear quadrupolar resonance (NQR) spectroscopy reveals chemical bonding patterns in materials and molecules through the unique coupling between nuclear spins and local fields. However, traditional NQR techniques require macroscopic…

Mesoscale and Nanoscale Physics · Physics 2025-01-14 S. Alex Breitweiser , Mathieu Ouellet , Tzu-Yung Huang , Tim H. Taminiau , Lee C. Bassett

Single nitrogen-vacancy (NV) centers are widely used as nanoscale sensors for magnetic and electric fields, strain and temperature. Nanoscale magnetometry using NV centers allows for example to quantitatively measure local magnetic fields…

Optically addressable solid-state spins have been proposed as robust radiofrequency (RF)-optical transducers sensitive to a specific RF frequency tuned by an external static magnetic field, but often require precise field alignment with the…

Amplification of a single spin state using nuclear magnetic resonance (NMR) techniques in a rotating frame is considered. The main aim is to investigate the efficient of various schemes for quantum detection. Results of numerical simulation…

Quantum Physics · Physics 2007-08-31 Gregory B. Furman , Victor M. Meerovich , Vladimir L. Sokolovsky

Nuclear magnetic resonance (NMR) spectroscopy usually requires high magnetic fields to create spectral resolution among different proton species. At low fields, chemical shift dispersion is insufficient to separate the species, and the…

Chemical Physics · Physics 2021-03-03 Stephen J. DeVience , Mason Greer , Soumyajit Mandal , Matthew S. Rosen

Nanodiamonds containing nitrogen vacancy (NV-) centers show promise for a number of emerging applications including targeted in vivo imaging and generating nuclear spin hyperpolarization for enhanced NMR spectroscopy and imaging. Here, we…

Magnetometers based on quantum mechanical processes enable high sensitivity and long-term stability without the need for re-calibration, but their integration into fieldable devices remains challenging. This paper presents a CMOS quantum…

Applied Physics · Physics 2020-07-23 Mohamed I. Ibrahim , Christopher Foy , Dirk R. Englund , Ruonan Han

We report a method for nanometer-scale pulsed nuclear magnetic resonance imaging and spectroscopy. Periodic radiofrequency pulses are used to create temporal correlations in the statistical polarization of a solid organic sample. The spin…

Mesoscale and Nanoscale Physics · Physics 2013-10-01 John M. Nichol , Tyler R. Naibert , Eric R. Hemesath , Lincoln J. Lauhon , Raffi Budakian

We report a systematic study of the hyperfine interaction between the electron spin of a single nitrogen-vacancy (NV) defect in diamond and nearby $^{13}$C nuclear spins, by using pulsed electron spin resonance spectroscopy. We isolate a…

Mesoscale and Nanoscale Physics · Physics 2015-06-04 A. Dréau , J. -R. Maze , M. Lesik , J. -F. Roch , V. Jacques

Magnetic resonance imaging (MRI) revolutionized diagnostic medicine and biomedical research by allowing a noninvasive access to spin ensembles. To enhance MRI resolution to the nanometer scale, new approaches including scanning probe…

Mesoscale and Nanoscale Physics · Physics 2019-10-23 Philip Willke , Kai Yang , Yujeong Bae , Andreas J. Heinrich , Christopher P. Lutz

The nitrogen-vacancy (NV) center in diamond has enabled studies of nanoscale nuclear magnetic resonance (NMR) and electron paramagnetic resonance with high sensitivity in small sample volumes. Most NV-detected NMR (NV-NMR) experiments are…

Mesoscale and Nanoscale Physics · Physics 2023-07-27 Yuhang Ren , Cooper Selco , Dylan Kawashiri , Michael Coumans , Benjamin Fortman , Louis S. Bouchard , Karoly Holczer , Susumu Takahashi

Recently, there have been significant developments to detect nuclear spins with an nitrogen vacancy (NV) center in diamond. However, due to the nature of the short range dipole-dipole interaction, it takes a long time to detect distant…

Quantum Physics · Physics 2021-08-11 Hideaki Hakoshima , Yuichiro Matsuzaki , Toyofumi Ishikawa

We report the detection and polarization of nuclear spins in diamond at room temperature by using a single nitrogen-vacancy (NV) center. We use Hartmann-Hahn double resonance to coherently enhance the signal from a single nuclear spin while…

Signal reception of nuclear magnetic resonance (NMR) usually relies on electrical amplification of the electromotive force caused by nuclear induction. Here, we report up-conversion of a radio-frequency NMR signal to an optical regime using…

While photoelectric detection of magnetic resonance (PDMR) can be applied to miniaturize nitrogen-vacancy (NV) center-based quantum sensors, real demonstration of PDMR-based magnetic field sensing remains as a distinctive challenge. To…

Quantum Physics · Physics 2026-02-13 Xuan-Ming Shen , Qilong Wu , Huihui Yu , Pei-Nan Ni , Qing Lou , Chao-Nan Lin , Xun Yang , Chong-Xin Shan , Yuan Zhang

Quantum entanglement has long been recognized as an important resource for quantum sensing. In this work, we demonstrate the use of multiple-quantum solid-state NMR for quantum sensing by creating, manipulating, and detecting large clusters…

Quantum Physics · Physics 2025-12-02 Conan Alexander , T S Mahesh

Advances in sensing devices that utilize nitrogen-vacancy (NV) center ensembles in diamond are driving progress in microscale nuclear magnetic resonance spectroscopy. Utilizing quantum sensing techniques in the high-field regime…

Quantum Physics · Physics 2025-10-22 Ainitze Biteri-Uribarren , Ana Martin , Jorge Casanova