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We analyze the scaling laws for a set of two different species of long flexible polymer chains joined together at one of their extremities (copolymer stars) in space dimension D=2. We use a formerly constructed field-theoretic description…

Soft Condensed Matter · Physics 2009-11-07 Christian von Ferber , Yurij Holovatch

We study theoretically the entropic elasticity of a semi-flexible polymer, such as DNA, confined to two dimensions. Using the worm-like-chain model we obtain an exact analytical expression for the partition function of the polymer pulled at…

Soft Condensed Matter · Physics 2009-11-11 Ashok Prasad , Yuko Hori , Jane' Kondev

Polymer models describing the statistics of biomolecules under confinement have applications to a wide range of single molecule experimental techniques and give insight into biologically relevant processes {\em{in vivo}}. In this paper, we…

Biological Physics · Physics 2023-09-18 Joel Gard , Greg Morrison

The stretching of a polymer chain by a large scale chaotic flow is considered. The steady state which emerges as a balance of the turbulent stretching and anharmonic resistance of the chain is quantitatively described, i.e. the dependency…

chao-dyn · Physics 2009-10-31 Michael Chertkov

The interaction of polymers with small-scale velocity gradients can trigger a coil-stretch transition in the polymers. We analyze this transition within a direct numerical simulation of shear turbulence with an Oldroyd-B model for the…

Chaotic Dynamics · Physics 2009-11-07 Bruno Eckhardt , Jochen Kronjaeger , Joerg Schumacher

Motivated by recent DNA-pulling experiments, we revisit the Poland-Scheraga model of melting a double-stranded polymer. We include distinct bending rigidities for both the double-stranded segments, and the single-stranded segments forming a…

Soft Condensed Matter · Physics 2008-11-13 Sahand Jamal Rahi , Mark Peter Hertzberg , Mehran Kardar

We present a loop-opening model that accounts for the molecular details of the intrinsic fracture energy for fracturing polymer networks. This model includes not only the energy released from the scission of bridging chains but also the…

Materials Science · Physics 2024-01-31 Shu Wang , Chase M. Hartquist , Bolei Deng , Xuanhe Zhao

We propose an analytical method for understanding the problem of multi-channel electron transfer reaction in solution, modeled by a particle undergoing diffusive motion under the influence of one donor and several acceptor potentials. The…

Quantum Physics · Physics 2015-06-30 Aniruddha Chakraborty

The dynamic structure factor of semiflexible polymers in solution is derived from the wormlike chain model. Special attention is paid to the rigid constraint of an inextensible contour and to the hydrodynamic interactions. For the cases of…

Soft Condensed Matter · Physics 2009-10-28 Klaus Kroy , Erwin Frey

We study the dynamical response of a single semiflexible polymer chain based on the theory developed by Hallatschek et al. for the wormlike-chain model. The linear viscoelastic response under oscillatory forces acting at the two chain ends…

Soft Condensed Matter · Physics 2009-11-03 T. Hiraiwa , T. Ohta

We perform large scale three-dimensional molecular dynamics simulations of unlinked and unknotted ring polymers diffusing through a background gel, here a three-dimensional cubic lattice. Taking advantage of this architecture, we propose a…

Soft Condensed Matter · Physics 2014-07-01 D. Michieletto , D. Marenduzzo , E. Orlandini , G. P. Alexander , M. S. Turner

We investigate the multi-chain version of the Chemical Master Equation, when there are transitions between different states inside the long chains, as well as transitions between (a few) different chains. In the discrete version, such a…

Statistical Mechanics · Physics 2015-06-12 Vahe Galstyan , David B. Saakian

A polymer folding model on the square lattice is constructed with attractive contact interactions of strength 1/c^2, 0<c<1. The corresponding model on a dynamical random lattice, with freely fluctuating co-ordination number at each vertex,…

Condensed Matter · Physics 2016-08-31 S. Dalley

In this paper we consider in detail the connection between the problem of a polymer in a random medium and that of a quantum particle in a random potential. We are interested in a system of finite volume where the polymer is known to be…

Disordered Systems and Neural Networks · Physics 2009-10-31 Yohannes Shiferaw , Yadin Y. Goldschmidt

We investigate the crystallization of a single, flexible homopolymer chain using transition path sampling (TPS). The chain consists of N identical spherical monomers evolved according to Langevin dynamics. While neighboring monomers are…

Soft Condensed Matter · Physics 2016-08-17 Christian Leitold , Christoph Dellago

We develop a general analysis of the diffusive dynamics of polydisperse polymers in the presence of chemical potential gradients, within the context of the tube model (with all species entangled). We obtain a set of coupled dynamical…

Soft Condensed Matter · Physics 2009-11-07 I. Pagonabarraga , M. E. Cates

A model multilevel molecule described by two sets of rotational internal energy levels of different parity and degenerate ground states, coupled by a constant interaction, is considered, by assuming that the random collisions in a gas of…

Quantum Physics · Physics 2013-05-31 Filippo Giraldi , Francesco Petruccione

We propose and theoretically study an experiment designed to measure short time polymer reaction kinetics in melts or dilute solutions. The photolysis of groups centrally located along chain backbones, one group per chain, creates pairs of…

Soft Condensed Matter · Physics 2009-10-31 Oleg V. Bychuk , Ben O'Shaughnessy , Nicholas Turro

We study properties of dilute polymer solutions which are known to depend strongly on polymer elongation. The probability density function (PDF) of polymer end-to-end extensions $R$ in turbulent flows is examined. We demonstrate that if the…

chao-dyn · Physics 2009-10-31 E. Balkovsky , A. Fouxon , V. Lebedev

Within a nonperturbative dynamical two-body approach - based on coupled equations of motion for the one-body density matrix and the two-body correlation function - we study the distribution of occupation numbers in a correlated system close…

Nuclear Theory · Physics 2009-10-22 Andreas Peter , Wolfgang Cassing , Joern M. Haeuser , Alfred Pfitzner