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Related papers: Understanding reversible looping kinetics of a lon…

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A diffusion theory for intramolecular reactions of polymer chain in dilute solution is formulated. We give a detailed analytical expression for calculation of rate of polymer looping in solution. The physical problem of looping can be…

Statistical Mechanics · Physics 2017-06-07 Moumita Ganguly , Anirudhha Chakraborty

We present a theoretical model for understanding the kinetics of a long polymer in solution. A Smoluchowski-like equation has been used to model the problem of polymer looping with a Dirac delta function sink of finite strength. The results…

Statistical Mechanics · Physics 2017-04-25 Moumita Ganguly , Anirudhha Chakraborty

We investigate theoretically the end-to-end looping time of a long chain polymer molecule immersed in a solvent. The dynamics of the end-to-end distance is governed by a Smoluchowski-like equation of a particle moving under the influence of…

Soft Condensed Matter · Physics 2018-03-20 Moumita Ganguly , Aniruddha Chakraborty

A simple analytical method for solving intra-molecular reactions of polymer chain in dilute solution is formulated. The physical problem of looping can be modeled mathematically with the use of a Smoluchowski-like equation with a Dirac…

Statistical Mechanics · Physics 2018-04-25 Moumita Ganguly , Aniruddha Chakraborty

The fundamental understanding of loop formation of long polymer chains in solution has been an important thread of research for several theoretical and experimental studies. Loop formations are important phenomenological parameters in many…

Statistical Mechanics · Physics 2017-01-17 Moumita Ganguly , Anirudhha Chakraborty

A diffusion-like theory for real time end-to-end distance of a long polymer chain in dilute solution is formulated. We give a detailed analytical expression for the end-to-end distance auto-correlation function of a long chain polymer in…

Soft Condensed Matter · Physics 2018-02-28 Moumita Ganguly , Aniruddha Chakraborty

The dynamics of loop formation by linear polymer chains has been a topic of several theoretical/experimental studies. Formation of loops and their opening are key processes in many important biological processes. Loop formation in flexible…

Soft Condensed Matter · Physics 2015-05-14 K. P. Santo , K. L. Sebastian

We study the reaction kinetics of end-functionalized polymer chains dispersed in an unreactive polymer melt. Starting from an infinite hierarchy of coupled equations for many-chain correlation functions, a closed equation is derived for the…

Soft Condensed Matter · Physics 2009-10-31 Ben O'Shaughnessy , Dimitrios Vavylonis

A theory of diffusion-controlled intramolecular reactions of polymer chain in dilute solution is formulated. Our model is based on the widely used diffusion-reaction formalism of Wilemski and Fixman (J. Chem. Phys. 60, 866 (1974). Our model…

Soft Condensed Matter · Physics 2016-06-02 Aniruddha Chakraborty

Although the stretching of polymers and biomolecules is important in numerous settings, their response when confined to two-dimensions is relatively poorly-studied. In this paper, we derive closed-form analytical expressions for the…

Soft Condensed Matter · Physics 2013-05-28 Sara Iliafar , Dmitri Vezenov , Anand Jagota

Loop formation between monomers in the interior of semiflexible chains describes elementary events in biomolecular folding and DNA bending. We calculate analytically the interior distance distribution function for semiflexible chains using…

Soft Condensed Matter · Physics 2009-11-11 Changbong Hyeon , D. Thirumalai

Molecular dynamics simulation methods are used to study the folding of polymer chains into packed cubic states. The polymer model, based on a chain of linked sites moving in the continuum, includes both excluded volume and torsional…

Soft Condensed Matter · Physics 2009-11-10 D. C. Rapaport

We study two cross-linked polymer systems in the strong stretching regime. The first consists of two polymers sharing one endpoint, with the other two endpoints coupled by a harmonic potential. Within the weakly bending approximation, we…

Soft Condensed Matter · Physics 2026-03-30 Geunho Noh , Panayotis Benetatos

Dynamics of a discrete polymer in time-dependent external potentials is studied with the master equation approach. We consider both stochastic and deterministic switching mechanisms for the potential states and give the essential equations…

Statistical Mechanics · Physics 2008-06-25 Janne Kauttonen , Juha Merikoski , Otto Pulkkinen

We study energy relaxation in a phenomenological model for polymer built from rheological considerations: a one dimensional nonlinear lattice with dissipative couplings. These couplings are well known in polymer's community to be possibly…

Statistical Mechanics · Physics 2009-11-07 F. Gobet , S. Ciliberto , T. Dauxois

We investigate the kinetics of loop formation in flexible ideal polymer chains (Rouse model), and polymers in good and poor solvents. We show for the Rouse model, using a modification of the theory of Szabo, Schulten, and Schulten, that the…

Soft Condensed Matter · Physics 2007-11-13 Ngo Minh Toan , Greg Morrison , Changbong Hyeon , D. Thirumalai

We present results of Monte Carlo study of the monomer-monomer correlation functions, static structure factor and asphericity characteristics of a single homopolymer in the coil and globular states for three distinct architectures of the…

Soft Condensed Matter · Physics 2009-11-07 Edward G. Timoshenko , Yuri A. Kuznetsov , Ronan Connolly

The process of polymer condensation, i.e. the formation of bonds between reactive end-groups, is ubiquitous in both industry and biology. Here we study generic systems undergoing polymer condensation in competition with cyclisation. Using a…

We analyze the probability of a single loop formation in a long flexible polymer chain in disordered environment in $d$ dimensions. The structural defects are considered to be correlated on large distances $r$ according to a power law $\sim…

Soft Condensed Matter · Physics 2016-04-14 K. Haydukivska , V. Blavatska

The mechanical properties of molecules are today captured by single molecule manipulation experiments, so that polymer features are tested at a nanometric scale. Yet devising mathematical models to get further insight beyond the commonly…

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