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We report the first direct spectroscopic evidence for coherent electronic coupling between excitons and trions in atomically thin transition metal dichalcogenides, specifically monolayer MoSe2. Signatures of coupling appear as isolated…

Mesoscale and Nanoscale Physics · Physics 2014-09-30 Akshay Singh , Galan Moody , Sanfeng Wu , Yanwen Wu , Nirmal J. Ghimire , Jiaqiang Yan , David G. Mandrus , Xiaodong Xu , Xiaoqin Li

Screening due to surrounding dielectric medium reshapes the electron-hole interaction potential and plays a pivotal role in deciding the binding energies of strongly bound exciton complexes in quantum confined monolayers of transition metal…

Mesoscale and Nanoscale Physics · Physics 2017-08-16 Garima Gupta , Sangeeth Kallatt , Kausik Majumdar

The plasmon-mediated manipulation of light-matter interaction in two-dimensional atomically transition-metal dichalcogenides (TMDs) critically depends on the design of plasmonic nanostructures to achieve the maximum optical field in TMDs.…

Optics · Physics 2021-12-07 Wei Li , Ming Xin , Wenze Lan , Qinghu Bai , Shuo Du , Gang Wang , Baoli Liu , Changzhi Gu

Monolayer transition metal dichalcogenide semiconductors, with versatile experimentally accessible exciton species, offer an interesting platform for investigating the interaction between excitons and a Fermi sea of charges. Using hexagonal…

Mesoscale and Nanoscale Physics · Physics 2020-08-18 Thomas Goldstein , Yueh-Chun Wu , Shao-Yu Chen , Takashi Taniguchi , Kenji Watanabe , Kalman Varga , Jun Yan

Many of the fundamental optical and electronic properties of atomically thin transition metal dichalcogenides are dominated by strong Coulomb interactions between electrons and holes, forming tightly bound atom-like excitons. Here, we…

Atomically thin semiconductors such as transition metal dichalcogenide (TMD) monolayers exhibit a very strong Coulomb interaction, giving rise to a rich exciton landscape. This makes these materials highly attractive for efficient and…

Mesoscale and Nanoscale Physics · Physics 2022-11-02 Raul Perea-Causin , Daniel Erkensten , Jamie M. Fitzgerald , Joshua J. P. Thompson , Roberto Rosati , Samuel Brem , Ermin Malic

Monolayer transition metal dichalcogenides (TMDCs) are direct gap semiconductors with unique potential for ultrathin light emitters. Yet, their photoluminescence (PL) is not completely understood. We compute the radiative recombination rate…

Materials Science · Physics 2018-07-20 Hsiao-Yi Chen , Maurizia Palummo , Davide Sangalli , Marco Bernardi

We report a determination of the complex in-plane dielectric function of monolayers of four transition metal dichalcogenides: MoS2, MoSe2, WS2 and WSe2, for photon energies from 1.5 - 3 eV. The results were obtained from reflection spectra…

Monolayer transition-metal dichalcogenide (TMD) semiconductors exhibit strong excitonic effects and hold promise for optical and optoelectronic applications. Yet, electron doping of TMDs leads to the conversion of neutral excitons into…

We have investigated the exciton dynamics in transition metal dichalcogenide mono-layers using time-resolved photoluminescence experiments performed with optimized time-resolution. For MoSe2 monolayers, we measure $\tau_{rad}=1.8\pm0.2$ ps…

Materials Science · Physics 2016-05-18 C. Robert , D. Lagarde , F. Cadiz , G. Wang , B. Lassagne , T. Amand , A. Balocchi , P. Renucci , S. Tongay , B. Urbaszek , X. Marie

A monolayer of transition metal dichalcogenide (TMDC) is shown to be capable of supporting a guided optical mode below the exciton resonance, a two-dimensional exciton polariton. This visible or near IR mode is confined roughly within a…

Optics · Physics 2015-05-05 Jacob B. Khurgin

Monolayer transition metal dichalcogenide (TMD) semiconductors such as MoSe$_2$ host strongly bound excitons which are known to exhibit a strong resonant third-order nonlinear response. Although there have been numerous studies of the…

Transition metal dichalcogenides (TMD) monolayers, holding potential as good sunlight absorbers, are promising materials for next-generation optoelectronic devices. They may enable ultrathin photovoltaic(PV) devices thanks to their…

Materials Science · Physics 2022-11-28 C. Attaccalite , M. S. Prete , M. Palummo , O. Pulci

Developing novel techniques for depositing transition metal dichalcogenides is crucial for the industrial adoption of 2D materials in optoelectronics. In this work, the lateral growth of molybdenum disulfide (MoS2) over an insulating…

Monolayer transition metal dichalcogenides (1L-TMDs) have tremendous potential as atomically thin, direct bandgap semiconductors that can be used as convenient building blocks for quantum photonic devices. However, the short exciton…

The rise of quantum science and technologies motivates photonics research to seek new platforms with strong light-matter interactions to facilitate quantum behaviors at moderate light intensities. One promising platform to reach such strong…

The monolayers of semiconducting transition metal dichalcogenides host strongly bound excitonic complexes and are an excellent platform for exploring many-body physics. Here we demonstrate a controlled kinetic manipulation of the…

Mesoscale and Nanoscale Physics · Physics 2022-04-05 Suman Chatterjee , Sarthak Das , Garima Gupta , Kenji Watanabe , Takashi Taniguchi , Kausik Majumdar

The optical response of traditional semiconductors depends on the laser excitation power used in experiments. For two-dimensional (2D) semiconductors, laser excitation effects are anticipated to be vastly different due to complexity added…

In semiconductor physics, many essential optoelectronic material parameters can be experimentally revealed via optical spectroscopy in sufficiently large magnetic fields. For monolayer transition-metal dichalcogenide semiconductors, this…

Mesoscale and Nanoscale Physics · Physics 2020-08-20 M. Goryca , J. Li , A. V. Stier , T. Taniguchi , K. Watanabe , E. Courtade , S. Shree , C. Robert , B. Urbaszek , X. Marie , S. A. Crooker

Monolayer transition-metal dichalcogenides are direct gap semiconductors with great promise for optoelectronic devices. Although spatial correlation of electrons and holes plays a key role, there is little experimental information on such…

Materials Science · Physics 2015-06-23 A. T. Hanbicki , M. Currie , G. Kioseoglou , A. L. Friedman , B. T. Jonker
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