Related papers: Coherence in Molecular Photoionization
We study strong field molecular ionization using few- (four to ten) cycle laser pulses. Employing a supercontinuum light source, we are able to tune the optical laser wavelength (photon energy) over a range of about $\sim$200 nm (500 meV).…
The advancement of the ultrafast pulse shaping and waveform synthesis allowed to coherently control the atomic and electronic motions in matter. The temporal resolution of the waveform synthesis is inversely proportional to the broadening…
Measuring the delay for an electron to emerge from different states is one of the major achievements of attosecond science. This delay can have two origins - the electron wave packet is reshaped during departure by the electrostatic field…
Bright squeezed light from parametric down-conversion in the infrared (IR) frequency range has triggered the emergence of attosecond quantum optics -- a new research field at the interface of quantum optics, strong-field physics, and…
The interaction of a short, few-cycle light pulse and an atom which is prepared initially in a superposition of two stationary states is shown to exhibit strong signatures of atomic coherence. For a given waveform of the laser pulse,…
The pursuit of ever-shorter time scales is a frontier in modern physics, exemplified by the synthesis of attosecond light pulses -- an achievement made possible by coherently superimposing a broad range of photon energies, as required by…
Recent technological advances allowed the coherent optical manipulation of high-energy electron wavepackets with attosecond precision. Here we theoretically investigate the collision of optically-modulated pulsed electron beams with atomic…
With the development of laser technology, pulse length enters the optical cycle regime and hence the interaction time between laser pulse and atoms becomes prominent. We investigate this problem in this Letter through the photoelectron…
The requirement of high space-time resolution and brightness is a great challenge for imaging atomic motion and making molecular movies. Important breakthroughs in ultrabright tabletop laser, x-ray and electron sources have enabled the…
In our model the electron dynamics are described by a two-state approximation. This might appear a rough approximation since it neglects coupling through excited electronic states and ionization channels. However at high intensity (laser…
The dynamics of atomic levels resonantly coupled by a coherent and intense short high-frequency laser pulse is discussed and it is advocated that this dynamics is sensitively probed by measuring the spectra of the particles emitted. It is…
We present the first direct experimental confirmation of attosecond pulse generation in the hard X-ray regime with a free-electron laser. Our experiment is based on measurements of a nonlinear optical phenomenon known as amplified…
Laser-induced electron diffraction is an evolving tabletop method, which aims to image ultrafast structural changes in gas-phase polyatomic molecules with sub-{\AA}ngstr\"om spatial and femtosecond temporal resolution. Here, we provide the…
We investigate how short and long electron trajectory contributions to high harmonic emission and their interferences give access to intra-molecular dynamics. In the case of unaligned molecules, we show experimental evidences that the long…
The generation of coherent light pulses in the extreme ultraviolet (XUV) spectral region with attosecond pulse durations constitutes the foundation of the field of attosecond science. Twenty years after the first demonstration of isolated…
The photoelectric effect, explained by Einstein in 1905, is often regarded as a one-electron phenomenon. However, in multi-electron systems, the interaction of the escaping electron with other electrons, referred to as electron correlation,…
We experimentally observe the action of multiple light pulses on the transverse motion of a continuous beam of fullerenes. The light potential is generated by non-resonant ultra-short laser pulses in perpendicular spatial overlap with the…
Controlling the wave function of free electrons is important to improve the spatial resolution of electron microscopes, the efficiency of electron interaction with sample modes of interest, and our ability to probe ultrafast materials…
Electron quantum path interferences in strongly laser-driven aligned molecules and their dependence on the molecular alignment is an essential open problem in strong-field molecular physics. Here, we demonstrate an approach which provides…
High harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, to date the shortest attosecond (as) pulses have been produced only in the extreme ultraviolet…