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Hot-exciton relaxation in semiconductor nanocrystals (NCs) is often described using perturbative theories, but their accuracy is difficult to assess for realistic exciton--phonon Hamiltonians. Here, we benchmark the perturbative quantum…

Thermoresponsive microgels are soft colloids that find widespread use as model systems for soft matter physics. Their complex internal architecture, made of a disordered and heterogeneous polymer network, has been so far a major challenge…

The in-plane coefficient of thermal expansion (CTE) for CdSe nanoplatelets with the zinc-blende structure containing from two to five monolayers is calculated from first principles within the quasiharmonic approximation. A comparison of the…

Materials Science · Physics 2019-08-14 Alexander I. Lebedev

Point polarizable molecules at fixed spatial positions have solvable electrostatic properties in classical approximation, the most familiar being the Clausius-Mossotti (CM) formula. This paper generalizes the model and imagines various…

Materials Science · Physics 2009-11-10 Philip B. Allen

Semiconductor Bi$_2$O$_2$Se nanolayers of high crystal quality have been realized via epitaxial growth. These two-dimensional (2D) materials possess excellent electron transport properties with potential application in nanoelectronics. It…

Mesoscale and Nanoscale Physics · Physics 2018-02-12 Mengmeng Meng , Shaoyun Huang , Congwei Tan , Jinxiong Wu , Yumei Jing , Hailin Peng , H. Q. Xu

Atomistically detailed computational studies of nanocrystals, such as those derived from the promising lead-halide perovskites, are challenging due to the large number of atoms and lack of symmetries to exploit. Here, focusing on…

Materials Science · Physics 2022-10-05 Giulia Biffi , Yeongsu Cho , Roman Krahne , Timothy C. Berkelbach

Quantum computation strongly relies on the realisation, manipulation and control of qubits. A central method for realizing qubits is by creating a double-well potential system with a significant gap between the first two eigenvalues and the…

Quantum Physics · Physics 2016-09-01 Ariel Landau , Yakir Aharonov , Eliahu Cohen

We investigate the ground state of a balanced electron-hole system in the quantum Hall regime using mean-field theory and obtain a rich phase diagram as a function of interlayer distance d and the filling factor within a layer. We identify…

Mesoscale and Nanoscale Physics · Physics 2007-12-03 C. -H. Zhang , Yogesh N. Joglekar

Understanding the physics of light emitter in quantum nanostructure regarding scalability, geometry, structure of the system and coupling between different degrees of freedom is important as one can improve the design and further provide…

Mesoscale and Nanoscale Physics · Physics 2019-01-25 Chen-Yen Lai , S. A. Trugman , Jian-Xin Zhu

One-dimensional (1D) confinement has been revealed to effectively tune the properties of materials in homogeneous states. The 1D physics can be further enriched by electronic inhomogeneity, which unfortunately remains largely unknown. Here…

Strongly Correlated Electrons · Physics 2021-08-11 Kaixuan Zhang , Lin Li , Hui Li , Qiyuan Feng , Nan Zhang , Long Cheng , Xiaodong Fan , Yubin Hou , Qingyou Lu , Zhenyu Zhang , Changgan Zeng

Solid-state nanopores offer a powerful platform for nanoscale analysis of individual analytes, including biomolecules and functionalized nanoparticles, by confining them within a precisely defined sensing region. However, their inherently…

Deciphering the three-dimensional atomic structure of solid-solid interfaces in core-shell nanomaterials is the key to understand their remarkable catalytical, optical and electronic properties. Here, we probe the three-dimensional atomic…

Materials Science · Physics 2023-06-21 Zezhou Li , Zhiheng Xie , Yao Zhang , Xilong Mu , Hai-jing Yin , Ya-wen Zhang , Colin Ophus , Jihan Zhou

We report on polarization-resolved resonant photoluminescence (PL) spectroscopy of bright (spin-1) and dark (spin-2) excitons in colloidal CdSe nanocrystal quantum dots. Using high magnetic fields to 33 T, we resonantly excite (and…

Materials Science · Physics 2009-11-11 M. Furis , H. Htoon , M. A. Petruska , T. Barrick , V. I. Klimov , S. A. Crooker

Overcoming the limitations of current nanofabrication techniques to achieve nanoscale feature sizes is essential for achieving new regimes of light-matter interactions at extreme frequencies and length scales. Here, we demonstrate a…

We perform computational investigations of electrolyte-mediated interactions of charged colloidal particles confined within nanochannels. We investigate the role of discrete ion effects, valence, and electrolyte strength on colloid-wall…

Soft Condensed Matter · Physics 2023-02-28 Inderbir S. Sidhu , Amalie L. Frischknecht , Paul J. Atzberger

The shape of crystalline nanoparticles (NP) can often be described by polyhedra with flat facet surfaces. Thus, structural studies of polyhedral bodies can help to describe geometric details of NPs. Here we consider compact polyhedra of…

Mesoscale and Nanoscale Physics · Physics 2023-07-24 Klaus E. Hermann

Intermittent photoluminescence of colloidal core/shell semiconductor nanocrystals of spherical and branched shape was studied under CW-laser excitation. Luminescent multichannel registration system was applied for the fluorescence detection…

Optics · Physics 2011-12-13 A. G. Vitukhnovsky , M. M. Kovalev , V. V. Lidsky , E. M. Khokhlov

Lipid nanoparticles own a remarkable potential in nanomedicine, only partially disclosed. While the clinical use of liposomes and cationic lipid-nucleic acid complexes is well-established, liquid lipid nanoparticles (nanoemulsions), solid…

Voltage control of ferromagnetism on the nanometer scale is highly appealing for the development of novel electronic devices. Here a key challenge is to implement and combine low power consumption, high operation speed, reliable…

The energy and photoluminescence (PL) spectra of a two-dimensional electron gas (2DEG) interacting with a valence-band hole are studied in the high-magnetic-field limit as a function of the filling factor nu and the separation $d$ between…

Mesoscale and Nanoscale Physics · Physics 2009-10-31 John J. Quinn , Arkadiusz Wojs , Kyung-Soo Yi , Izabela Szlufarska
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