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Results from four different approximations to the phonon-assisted quantum adsorption rate for cold atoms on a 2D material are compared and contrasted: (1) a loop expansion (LE) based on the atom-phonon coupling, (2) non-crossing…

Mesoscale and Nanoscale Physics · Physics 2018-12-18 Sanghita Sengupta , Dennis P. Clougherty

The phonon-assisted sticking rate of slow moving atoms impinging on an elastic membrane at nonzero temperature is studied analytically using a model with linear atom-phonon interactions, valid in the weak coupling regime. A perturbative…

Mesoscale and Nanoscale Physics · Physics 2017-12-06 Dennis P. Clougherty

We study the infrared dynamics of low-energy atoms interacting with a sample of suspended graphene at finite temperature. The dynamics exhibits severe infrared divergences order by order in perturbation theory as a result of the singular…

Mesoscale and Nanoscale Physics · Physics 2016-06-22 Sanghita Sengupta , Valeri N. Kotov , Dennis P. Clougherty

A continuum model for low-energy physisorption on a membrane under tension is proposed and studied with variational mean-field theory. A discontinuous change in the energy-dependent sticking coefficient is predicted under certain…

Mesoscale and Nanoscale Physics · Physics 2014-12-08 Dennis P. Clougherty

Crystalline membranes at finite temperatures have an anomalous behavior of the bending rigidity that makes them more rigid in the long wavelength limit. This issue is particularly relevant for applications of graphene in nano- and…

Materials Science · Physics 2010-09-22 K. V. Zakharchenko , R. Roldan , A. Fasolino , M. I. Katsnelson

Two approximations used by Sengupta [Phys. Rev. B {\bf 100}, 075429 (2019)] in numerically computing the adsorption rate of cold hydrogen atoms on suspended graphene are critically examined. The independent boson model approximation (IBMA)…

Mesoscale and Nanoscale Physics · Physics 2020-06-12 Dennis P. Clougherty

We devise a theory of adsorption of low-energy atoms on suspended graphene membranes maintained at 10 K based on a model of atom-acoustic phonon interactions. Our primary technique includes a non-perturbative method which treats the…

Mesoscale and Nanoscale Physics · Physics 2020-01-06 Sanghita Sengupta

Adsorption of hydrogen atoms on a single graphite sheet (graphene) has been investigated by first-principles electronic structure means, employing plane-wave based, periodic density functional theory. A reasonably large 5x5 surface unit…

Materials Science · Physics 2009-11-13 Simone Casolo , Ole Martin Lovvik , Rocco Martinazzo , Gian Franco Tantardini

Based on a new self-energy for atom-phonon interaction, preceding Comment argues about the insufficiency of the mathematical techniques within the Independent Boson Model (IBM) to study physisorption in graphene membranes. In this Reply, we…

Materials Science · Physics 2020-07-15 Sanghita Sengupta

Graphene plasmonic resonators have been broadly studied in the terahertz and mid-infrared ranges because of their electrical tunability and large confinement factors which can enable dramatic enhancement of light-matter coupling. In this…

We perform a detailed analysis of electronic polarizability of graphene with different theoretical approaches. From Kubo's linear response formalism, we give a general expression of frequency and wave-vector dependent polarizability within…

Mesoscale and Nanoscale Physics · Physics 2021-03-31 Tao Zhu , Mauro Antezza , Jian-Sheng Wang

Free-standing graphene is inherently crumpled in the out-of-plane direction due to dynamic flexural phonons and static wrinkling. We explore the consequences of this crumpling on the effective mechanical constants of graphene. We develop a…

We demonstrate that a key elastic parameter of a suspended crystalline membrane---the Poisson ratio (PR) $\nu$---is a non-trivial function of the applied stress $\sigma$ and of the system size $L$, i.e., $\nu=\nu_L(\sigma)$. We consider a…

Mesoscale and Nanoscale Physics · Physics 2018-05-01 I. S. Burmistrov , I. V. Gornyi V. Yu. Kachorovskii , M. I. Katsnelson , J. H. Los , A. D. Mirlin

Graphene is the nature's thinnest elastic membrane, with exceptional mechanical and electrical properties. We report the direct observation and creation of one-dimensional (1D) and 2D periodic ripples in suspended graphene sheets, using…

Mesoscale and Nanoscale Physics · Physics 2009-07-28 Wenzhong Bao , Feng Miao , Zhen Chen , Hang Zhang , Wanyoung Jang , Chris Dames , Chun Ning Lau

Quasi free-standing monolayer graphene can be produced by intercalating species like oxygen or hydrogen between epitaxial graphene and the substrate crystal. If the graphene is indeed decoupled from the substrate, one would expect the…

We present a detailed calculation of intensities of two-phonon and four-phonon Raman peaks in graphene. Writing the low-energy hamiltonian of the interaction of electrons with the crystal vibrations and the electromagnetic field from pure…

Materials Science · Physics 2009-11-13 D. M. Basko

The smearing of the graphene/graphane interface due to the thermally activated migration of hydrogen atoms is studied by the molecular dynamics method. Contrary to expectations, it is found that the fast spontaneous regeneration of this…

Mesoscale and Nanoscale Physics · Physics 2015-05-14 L. A. Openov , A. I. Podlivaev

Graphene is the extreme material for molecular sensory and hydrogen storage applications because of its two-dimensional geometry and unique structure-property relationship. In this Letter, hydrogenation of graphene is discussed in the…

Materials Science · Physics 2010-02-10 Zhiping Xu , Kun Xue

Two-magnon Raman scattering provides important information about electronic correlations in the insulating parent compounds of high-$T_c$ materials. Recent experiments have shown a strong dependence of the Raman signal in $B_{1g}$ geometry…

Strongly Correlated Electrons · Physics 2009-10-30 Dirk K. Morr , Andrey V. Chubukov

Density functional calculations are employed to study the molecular dissociation of hydrogen on graphene, the diffusion of chemisorbed atomic species, and the electronic properties of the resulting hydrogen on graphene system. Our results…

Materials Science · Physics 2011-06-03 Hayley McKay , David J. Wales , S. J. Jenkins , J. A. Verges , P. L. de Andres
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