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Spin excitations are explored in the electron-doped spin-orbit Mott insulator (Sr$_{1-x}$La$_{x}$)$_3$Ir$_2$O$_7$. As this bilayer square lattice system is doped into the metallic regime, long-range antiferromagnetism vanishes, yet a…

Strongly Correlated Electrons · Physics 2016-09-14 Tom Hogan , Rebecca Dally , Mary Upton , J. P. Clancy , Kenneth Finkelstein , Young-June Kim , M. J. Graf , Stephen D. Wilson

A complete structural solution of the bilayer iridate compound Sr3Ir2O7 presently remains outstanding. Previously reported structures for this compound vary and all fail to explain weak structural violations observed in neutron scattering…

Strongly Correlated Electrons · Physics 2016-04-22 Tom Hogan , Lars Bjaalie , Liuyan Zhao , Carina Belvin , Xiaoping Wang , Chris G. Van de Walle , David Hsieh , Stephen D. Wilson

The electron-doping-driven collapse of the charge gap and staggered magnetization of the spin-orbit-assisted Mott insulator Sr$_{3}$Ir$_{2}$O$_{7}$ is explored via first-principles computational methods. In the antiferromagnetic phase, the…

Strongly Correlated Electrons · Physics 2018-08-15 Michael W. Swift , Zach Porter , Stephen D. Wilson , Chris G. Van de Walle

The path from a Mott insulating phase to high temperature superconductivity encounters a rich set of unconventional phenomena involving the insulator-to-metal transition (IMT) such as emergent electronic orders and pseudogaps that…

Strongly Correlated Electrons · Physics 2019-05-17 Zhenyu Wang , Daniel Walkup , Yulia Maximenko , Wenwen Zhou , Tom Hogan , Ziqiang Wang , Stephen D. Wilson , Vidya Madhavan

Layered perovskite iridates realize a rare class of Mott insulators that are predicted to be strongly spin-orbit coupled analogues of the parent state of cuprate high-temperature superconductors. Recent discoveries of pseudogap, magnetic…

Strongly Correlated Electrons · Physics 2017-04-25 H. Chu , L. Zhao , A. de la Torre , T. Hogan , S. D. Wilson , D. Hsieh

We have measured the doping and temperature dependence of lattice vibrations and magnetic excitations in the prototypical doped spin-orbit Mott insulator Sr$_{2-x}$La$_x$IrO$_4$ (x=0, 0.015, and 0.10). Our findings show that the…

Strongly Correlated Electrons · Physics 2017-09-27 H. Gretarsson , J. Sauceda , N. H. Sung , M. Höppner , M. Minola , B. J. Kim , B. Keimer , M. Le Tacon

A neutron scattering study of nonsuperconducting La$_{2-x}$Sr$_x$CaCu$_2$O$_6$ (x=0 and 0.2), a bilayer copper oxide without CuO chains, has revealed an unexpected tetragonal-to-orthorhombic transition with a doping dependent transition…

Superconductivity · Physics 2009-11-07 C. Ulrich , S. Kondo , M. Reehuis , H. He , C. Bernhard , C. Niedermayer , F. Bouree , P. Bourges , M. Ohl , H. M. Ronnow , H. Takagi , B. Keimer

The insulator to metal transition in LaTiO_3 induced by La substitution via Sr is studied within multi-band exact diagonalization dynamical mean field theory at finite temperatures. It is shown that weak hole doping triggers a large…

Strongly Correlated Electrons · Physics 2009-11-13 A. Liebsch

We investigated Ru-doped single-crystal 5$d$ iridiates, Sr$_2$Ir$_{1-x}$Ru$_x$O$_{4}$, at three different doping concentrations ($x =$ 0.01, 0.07 and 0.10) using optical spectroscopy. The undoped pristine compound (Sr$_2$IrO$_{4}$) is known…

Strongly Correlated Electrons · Physics 2021-10-06 Seokbae Lee , Yu-Seong Seo , Eilho Jung , Seulki Roh , Myounghoon Lee , Hwan Young Choi , Jong Hyuk Kim , Nara Lee , Young Jai Choi , Jungseek Hwang

We explore the effects of disordered charged defects on the electronic excitations observed in the photoemission spectra of doped transition metal oxides in the Mott insulating regime by the example of the $R_{1-x}$Ca$_x$VO$_3$ perovskites,…

Strongly Correlated Electrons · Physics 2018-04-09 Adolfo Avella , Andrzej M. Oleś , Peter Horsch

Motivated by experiments on the carrier-doped bilayer iridate $(\text{Sr}_{1-x}\text{La}_x)_3\text{Ir}_2\text{O}_7$, we study the dynamics of a single doped electron in a bilayer magnet in the presence of spin-orbit coupling, taking into…

Strongly Correlated Electrons · Physics 2018-12-20 Shouryya Ray , Matthias Vojta

We use single-crystal neutron diffraction to determine the crystal structure symmetry and the magnetic evolution in the rhodium doped iridates $\rm Sr_2Ir_{1-x}Rh_{x}O_4$ ($0\leq x \leq 0.16$). Throughout this doping range, the crystal…

The evolution of the electronic properties of electron-doped (Sr{1-x}La{x})2IrO4 is experimentally explored as the doping limit of La is approached. As electrons are introduced, the electronic ground state transitions from a spin-orbit Mott…

We propose and study theoretically a new mechanism of electron-impurity scattering in doped seminconductors with large dielectric constant. It is based upon the idea of \textit{vector} character of deformations caused in the crystalline…

Mesoscale and Nanoscale Physics · Physics 2022-09-26 Khachatur G. Nazaryan , Mikhail Feigel'man

TM-doped IrTe2(TM=Mn, Fe, Co, Ni) compounds were synthesized by solid state reaction. Single crystal x-ray diffraction experiments indicate that part of the doped TM ions (TM=Fe, Co, and Ni) substitute for Ir, and the rest intercalate into…

Superconductivity · Physics 2013-10-18 J. -Q. Yan , B. Saparov , A. S. Sefat , H. Yang , H. B. Cao , H. D. Zhou , B. C. Sales , D. G. Mandrus

Doping the distorted-perovskite Mott insulators LaTiO$_3$ and GdTiO$_3$ with a single SrO layer along the [001] direction gives rise to a rich correlated electronic structure. A realistic superlattice study by means of the charge…

Materials Science · Physics 2015-05-08 Frank Lechermann , Michael Obermeyer

The electronic phase diagram of the weak spin-orbit Mott insulator (Sr(1-x)Lax)3Ir2O7 is determined via an exhaustive experimental study. Upon doping electrons via La substitution, an immediate collapse in resistivity occurs along with a…

Strongly Correlated Electrons · Physics 2015-07-07 Tom Hogan , Z. Yamani , D. Walkup , Xiang Chen , Rebecca Dally , Thomas Z. Ward , John Hill , Z. Islam , Vidya Madhavan , Stephen D. Wilson

Neutron diffraction measurements are presented exploring the magnetic and structural phase behaviors of the candidate J$_{eff}=1/2$ Mott insulating iridate Sr$_2$IrO$_4$. Comparisons are drawn between the correlated magnetism in this single…

Strongly Correlated Electrons · Physics 2013-04-09 Chetan Dhital , Tom Hogan , Z. Yamani , Clarina de la Cruz , Xiang Chen , Sovit Khadka , Zhensong Ren , Stephen D. Wilson

The effect of isoelectronic substitution within single crystals of (Sr1-xCax)2-yIrO4+z is explored. The nominal n=1 Ruddlesden-Popper phase with y=0, z=0 remains stable from x=0 until x=0.11, where the antiferromagnet spin-orbit Mott…

Materials Science · Physics 2016-11-23 Xiang Chen , Stephen D. Wilson

The ground state of a double-exchange model for orbitally degenerate $e_g$ electrons with Jahn-Teller lattice coupling and weak disorder is found to be spatially inhomogeneous near half filling. Using a real space Monte-Carlo method we show…

Disordered Systems and Neural Networks · Physics 2009-11-11 Sanjeev Kumar , Arno P. Kampf , Pinaki Majumdar
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