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We report the first experimental demonstration of stimulated Raman adiabatic passage (STIRAP) in nuclear-spin transitions of $^{14}$N within nitrogen-vacancy (NV) color centers in diamond. It is shown that the STIRAP technique suppresses…

Accurate control of a quantum system is a fundamental requirement in many areas of modern science ranging from quantum information processing to high-precision measurements. A significantly important goal in quantum control is to prepare a…

The use of the nuclear spins surrounding electron spin qubits as quantum registers and long-lived memories opens the way to new applications in quantum information and biological sensing. Hence, there is a need for generic and robust forms…

Quantum Physics · Physics 2021-07-06 O. T. Whaites , J. Randall , T. H. Taminiau , T. S. Monteiro

Quantum adiabatic passages can be greatly accelerated by a suitable control field, called a counter-diabatic field, which varies during the scan through resonance. Here, we implement this technique on the electron spin of a single…

Nuclear spins in certain solids couple weakly to their environment, making them attractive candidates for quantum information processing and inertial sensing. When coupled to the spin of an optically-active electron, nuclear spins can be…

Quantum Physics · Physics 2022-11-11 Alexander A. Wood , Russell M. Goldblatt , Robert E. Scholten , Andy M. Martin

Detecting and controlling nuclear spin nano-ensembles is crucial for the further development of nuclear magnetic resonance (NMR) spectroscopy and for the emerging solid state quantum technology. Here we present the fabrication of a…

High-fidelity multi-qubit initialization is vital for quantum simulation, quantum information processing (QIP), and quantum sensing. In diamond platforms, nuclear spin registers can be initialized through polarization transfer from a nearby…

Quantum Physics · Physics 2026-03-02 Soham Pal , Oliver T. Whaites , Wolfgang Knolle , Tania S. Monteiro , Helena S. Knowles

Stimulated Raman Adiabatic Passage, a very efficient technique for manipulating a quantum system based on the adiabatic theorem, is analyzed in the case where the manipulated physical system is interacting with a spin bath. Exploitation of…

Quantum Physics · Physics 2023-11-21 Benedetto Militello , Anna Napoli

We experimentally isolate, characterize and coherently control up to six individual nuclear spins that are weakly coupled to an electron spin in diamond. Our method employs multi-pulse sequences on the electron spin that resonantly amplify…

Mesoscale and Nanoscale Physics · Physics 2012-10-23 T. H. Taminiau , J. J. T. Wagenaar , T. van der Sar , F. Jelezko , V. V. Dobrovitski , R. Hanson

We demonstrate a novel method for coherent optical manipulation of individual nuclear spins in the solid state, mediated by the electronic states of a proximal quantum emitter. Specifically, using the nitrogen-vacancy (NV) color center in…

Quantum Physics · Physics 2020-04-22 M. L. Goldman , T. L. Patti , D. Levonian , S. F. Yelin , M. D. Lukin

Significant aspects of advanced quantum technology today rely on rapid control of atomic matterwaves with hyperfine Raman transitions. Unfortunately, efficient Raman excitations are usually accompanied by uncompensated dynamic phases and…

Atomic Physics · Physics 2023-05-29 Liyang Qiu , Lingjing Ji , Jiangyong Hu , Yizun He , Yuzhuo Wang , Saijun Wu

Spin defects in solids, such as the nitrogen-vacancy (NV) center in diamond, have emerged as a key tool for detecting nuclear spins at the nanoscale. While active nuclear spin control via radio-frequency (RF) irradiation is often…

Isolated nuclear spins offer a promising building block for quantum information processing systems, but their weak interactions often impede preparation, control, and detection. Hyperfine coupling to a proximal electronic spin can enhance…

Quantum Physics · Physics 2013-05-29 Benjamin Smeltzer , Jean McIntyre , Lilian Childress

Reaching a given target quantum state with high fidelity and fast operation speed close to the quantum limit represents an important goal in quantum information science. Here, we experimentally demonstrate superadiabatic quantum driving to…

Quantum Physics · Physics 2024-04-05 Musang Gong , Min Yu , Yaoming Chu , Wei Chen , Qingyun Cao , Ning Wang , Jianming Cai , Ralf Betzholz , Luigi Giannelli

Squeezing ensemble of spins provides a way to surpass the standard quantum limit (SQL) in quantum metrology and test the fundamental physics as well, and therefore attracts broad interest. Here we propose an experimentally accessible…

Quantum Physics · Physics 2021-04-07 Keyu Xia

This work theoretically investigates possibilities of using the Stimulated Raman Adiabatic Passage (STIRAP) and its variants to control a coherent superposition of quantum states. We present a generalization of the so-called fractional…

Quantum Physics · Physics 2026-01-14 Miguel A. Alarcón , Karl Hauser , Nikolay V. Golubev

Nuclear spins in the solid state environment of diamond are highly coherent, but difficult to rapidly control due to the small nuclear gyromagnetic ratio. Here we demonstrate a more than 50-fold enhancement of the effective nuclear…

Mesoscale and Nanoscale Physics · Physics 2016-08-05 S. Sangtawesin , J. R. Petta

In a solid-state spin system, we experimentally demonstrate a protocol for quantum-state population transfer with an improved efficiency compared to traditional stimulated Raman adiabatic passage (STIRAP). Using the ground-state triplet of…

Quantum Physics · Physics 2023-05-03 Musang Gong , Min Yu , Ralf Betzholz , Yaoming Chu , Pengcheng Yang , Zhenyu Wang , Jianming Cai

Precise coherent control of the individual electronic spins associated with atom-like impurities in the solid state is essential for applications in quantum information processing and quantum metrology. We demonstrate all-optical…

Quantum Physics · Physics 2015-03-05 Yiwen Chu , Matthew Markham , Daniel J. Twitchen , Mikhail D. Lukin

Spin impurities in diamond have emerged as a promising building block in a wide range of solid-state-based quantum technologies. The negatively charged silicon-vacancy centre combines the advantages of its high-quality photonic properties…

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